Seasonal Simulation of Tropospheric Ozone over the Midwestern and Northeastern United States: An Application of a Coupled Regional Climate and Air Quality Modeling System

Ho-Chun Huang Illinois State Water Survey, Champaign, Illinois

Search for other papers by Ho-Chun Huang in
Current site
Google Scholar
PubMed
Close
,
Xin-Zhong Liang Illinois State Water Survey, Champaign, Illinois

Search for other papers by Xin-Zhong Liang in
Current site
Google Scholar
PubMed
Close
,
Kenneth E. Kunkel Illinois State Water Survey, Champaign, Illinois

Search for other papers by Kenneth E. Kunkel in
Current site
Google Scholar
PubMed
Close
,
Michael Caughey Illinois State Water Survey, Champaign, Illinois

Search for other papers by Michael Caughey in
Current site
Google Scholar
PubMed
Close
, and
Allen Williams Illinois State Water Survey, Champaign, Illinois

Search for other papers by Allen Williams in
Current site
Google Scholar
PubMed
Close
Restricted access

Abstract

The impacts of air pollution on the environment and human health could increase as a result of potential climate change. To assess such possible changes, model simulations of pollutant concentrations need to be performed at climatic (seasonal) rather than episodic (days) time scales, using future climate projections from a general circulation model. Such a modeling system was employed here, consisting of a regional climate model (RCM), an emissions model, and an air quality model. To assess overall model performance with one-way coupling, this system was used to simulate tropospheric ozone concentrations in the midwestern and northeastern United States for summer seasons between 1995 and 2000. The RCM meteorological conditions were driven by the National Centers for Environmental Prediction/Department of Energy global reanalysis (R-2) using the same procedure that integrates future climate model projections. Based on analyses for several urban and rural areas and regional domains, fairly good agreement with observations was found for the diurnal cycle and for several multiday periods of high ozone episodes. Even better agreement occurred between monthly and seasonal mean quantities of observed and model-simulated values. This is consistent with an RCM designed primarily to produce good simulations of monthly and seasonal mean statistics of weather systems.

Corresponding author address: Ho-Chun Huang, Illinois State Water Survey, 2204 Griffith Dr., Champaign, IL 61820. Email: huang2@uiuc.edu

This article included in the NOAA/EPA Golden Jubilee special collection.

Abstract

The impacts of air pollution on the environment and human health could increase as a result of potential climate change. To assess such possible changes, model simulations of pollutant concentrations need to be performed at climatic (seasonal) rather than episodic (days) time scales, using future climate projections from a general circulation model. Such a modeling system was employed here, consisting of a regional climate model (RCM), an emissions model, and an air quality model. To assess overall model performance with one-way coupling, this system was used to simulate tropospheric ozone concentrations in the midwestern and northeastern United States for summer seasons between 1995 and 2000. The RCM meteorological conditions were driven by the National Centers for Environmental Prediction/Department of Energy global reanalysis (R-2) using the same procedure that integrates future climate model projections. Based on analyses for several urban and rural areas and regional domains, fairly good agreement with observations was found for the diurnal cycle and for several multiday periods of high ozone episodes. Even better agreement occurred between monthly and seasonal mean quantities of observed and model-simulated values. This is consistent with an RCM designed primarily to produce good simulations of monthly and seasonal mean statistics of weather systems.

Corresponding author address: Ho-Chun Huang, Illinois State Water Survey, 2204 Griffith Dr., Champaign, IL 61820. Email: huang2@uiuc.edu

This article included in the NOAA/EPA Golden Jubilee special collection.

Save
  • Aw, J., and M. J. Kleeman, 2003: Evaluating the first-order effect of intraannual temperature variability on urban air pollution. J. Geophys. Res., 108 .4365, doi:10.1029/2002JD002688.

    • Search Google Scholar
    • Export Citation
  • Berkowitz, C. M., J. D. Fast, S. Springston, R. Larson, C. Spicer, and P. Doskey, 1998: Formation mechanisms and chemical characteristics of elevated photochemical layers over the United States. J. Geophys. Res., 103 , 1063110647.

    • Search Google Scholar
    • Export Citation
  • Berkowitz, C. M., J. D. Fast, and R. C. Easter, 2000: Boundary-layer vertical exchange processes and the mass budget of ozone: Observations and model results. J. Geophys. Res., 105 , 1478914805.

    • Search Google Scholar
    • Export Citation
  • Bouchet, V. S., R. Laprise, E. Torlaschi, and J. C. McConnell, 1999a: Studying ozone climatology with a regional climate model, 1, Model description and evaluation. J. Geophys. Res., 104 , 3035130371.

    • Search Google Scholar
    • Export Citation
  • Bouchet, V. S., R. Laprise, E. Torlaschi, J. C. McConnell, and D. A. Plummer, 1999b: Studying ozone climatology with a regional climate model, 2, Climatology. J. Geophys. Res., 104 , 3037330385.

    • Search Google Scholar
    • Export Citation
  • Carter, W. P. L., 1990: A detailed mechanism for the gas-phase atmospheric reactions of organic compounds. Atmos. Environ., 24A , 481518.

    • Search Google Scholar
    • Export Citation
  • Chang, J. S., R. A. Brost, I. S. A. Isaksen, S. Madronich, P. Middleton, W. R. Stockwell, and C. J. Walcek, 1987: A three dimensional Eulerian acid deposition model: Physical concepts and formulation. J. Geophys. Res., 92 , 1468114700.

    • Search Google Scholar
    • Export Citation
  • Chang, J. S., S. Jin, Y. Li, M. Beauharnois, C-H. Lu, H-C. Huang, S. Tanrikulu, and J. Damassa, 1997: The SARMAP Air Quality Model final report. Air Resource Board, California Environmental Protection Agency.

  • Cressman, G., 1959: An operational objective analysis system. Mon. Wea. Rev., 87 , 367374.

  • Doran, J. C., C. M. Berkowitz, R. L. Coulter, W. J. Shaw, and C. W. Spicer, 2003: The 2001 Phoenix Sunrise experiment: Vertical mixing and chemistry during the morning transition in Phoenix. Atmos. Environ., 37 , 23652377.

    • Search Google Scholar
    • Export Citation
  • Dudhia, J., D. Gill, Y-R. Guo, K. Manning, W. Wang, and J. Chriszar, 2000: PSU/NCAR Mesoscale Modeling System tutorial class notes and user’s guide: MM5 Modeling System Version 3. [Available online at http://www.mmm.ucar.edu/mm5/documents/MM5_tut_Web_notes/tutorialTOC.htm.].

  • Fast, J. D., and W. E. Heilman, 2003: The effect of lake temperatures and emissions on ozone exposure in the western Great Lakes region. J. Appl. Meteor., 42 , 11971217.

    • Search Google Scholar
    • Export Citation
  • Fast, J. D., and W. E. Heilman, 2005: Simulated sensitivity of seasonal ozone exposure in the Great Lakes region to changes in anthropogenic emissions in the presence of interannual variability. Atmos. Environ., 39 , 52915306.

    • Search Google Scholar
    • Export Citation
  • Fast, J. D., J. C. Doran, W. J. Shaw, R. L. Coulter, and T. J. Martin, 2000: The evolution of the boundary layer and its effect on air chemistry in the Phoenix area. J. Geophys. Res., 105 , 2283322848.

    • Search Google Scholar
    • Export Citation
  • Fast, J. D., R. A. Zaveri, X. Bian, E. G. Chapman, and R. C. Easter, 2002: Effect of regional-scale transport on oxidants in the vicinity of Philadelphia during the 1999 NE-OPS field campaign. J. Geophys. Res., 107 .4307, doi:10.1029/2001JD000980.

    • Search Google Scholar
    • Export Citation
  • Gery, M. W., G. Z. Whitten, J. P. Killus, and M. C. Dodge, 1989: A photochemical kinetics mechanism for urban and regional scale computer modeling. J. Geophys. Res., 94 , 1292512956.

    • Search Google Scholar
    • Export Citation
  • Guenther, A., P. Zimmerman, and M. Wildermuth, 1994: Natural volatile organic compound emissions rate estimates for U.S woodland landscapes. Atmos. Environ., 28 , 11971210.

    • Search Google Scholar
    • Export Citation
  • Hogrefe, C., S. T. Rao, P. Kasibhatla, W. Hao, G. Sistla, R. Mathur, and J. McHenry, 2001: Evaluating the performance of regional-scale photochemical modeling systems: Part II— Ozone predictions. Atmos. Environ., 35 , 41754188.

    • Search Google Scholar
    • Export Citation
  • Hogrefe, C., and Coauthors, 2004a: Simulating regional-scale ozone climatology over the eastern United States: Model evaluation results. Atmos. Environ., 38 , 26272638.

    • Search Google Scholar
    • Export Citation
  • Hogrefe, C., and Coauthors, 2004b: Simulating changes in regional air pollution over the eastern United States due to changes in global and regional climate and emissions. J. Geophys. Res., 109 .D22301, doi:10.1029/2004JD004690.

    • Search Google Scholar
    • Export Citation
  • Houghton, J. T., Y. Ding, D. J. Griggs, M. Noguer, P. J. van der Linden, X. Dai, K. Maskell, and C. A. Johnson, 2001: Climate Change 2001: The Scientific Basis. Cambridge University Press, 881 pp.

    • Search Google Scholar
    • Export Citation
  • Houyoux, M. R., J. M. Vukovich Jr., C. J. Coats, N. J. M. Wheeler, and P. S. Kasibhatla, 2000: Emission inventory development and processing for the Seasonal Model for Regional Air Quality (SMRAQ) project. J. Geophys. Res., 105 , 90799090.

    • Search Google Scholar
    • Export Citation
  • Huang, H-C., 2002: Modeling study on the importance of biogenic VOCs in tropospheric ozone formations over the U.S. Proc. Int. Workshop on Biogenic Volatile Organic Compounds and Ozone Pollution, Taipei, Taiwan, National Yunlin University of Science and Technology, 65–90.

  • Huang, H-C., and J. S. Chang, 2001: On the performance of numerical solvers for chemistry submodel in three-dimensional air quality models, 1. Box-model simulations. J. Geophys. Res., 106 , 2017520188.

    • Search Google Scholar
    • Export Citation
  • Kanamitsu, M., W. Ebisuzaki, J. Woolen, S-K. Yang, J. J. Hnilo, M. Fiorino, and G. L. Potter, 2002: The NCEP-DOE AMIP-II reanalysis (R-2). Bull. Amer. Meteor. Soc., 83 , 16311643.

    • Search Google Scholar
    • Export Citation
  • Kunkel, K. E., S. A. Changnon, B. C. Reinke, and R. W. Arritt, 1996: The July 1995 heat wave in the Midwest: A climatic perspective and critical weather factors. Bull. Amer. Meteor. Soc., 77 , 15071518.

    • Search Google Scholar
    • Export Citation
  • Liang, X-Z., K. E. Kunkel, and A. N. Samel, 2001: Development of a regional climate model for U.S. Midwest applications. Part I: Sensitivity to buffer zone treatment. J. Climate, 14 , 43634378.

    • Search Google Scholar
    • Export Citation
  • Liang, X-Z., L. Li, K. E. Kunkel, M. Ting, and J. X. L. Wang, 2004: Regional climate model simulation of U.S. precipitation during 1982–2002. Part I: Annual cycle. J. Climate, 17 , 35103528.

    • Search Google Scholar
    • Export Citation
  • Liang, X-Z., J. Pan, J. Zhu, K. E. Kunkel, J. X. L. Wang, and A. Dai, 2006: Regional climate model downscaling of the U.S. summer climate and future change. J. Geophys. Res., 111 .D10108, doi:10.1029/2005JD006685.

    • Search Google Scholar
    • Export Citation
  • Lu, R., C. Lin, R. Turco, and A. Arakawa, 2000: Cumulus transport of chemical tracers, 1, Cloud-resolving model simulations. J. Geophys. Res., 105 , 1000110021.

    • Search Google Scholar
    • Export Citation
  • Middleton, P., W. R. Stockwell, and W. P. L. Carter, 1990: Aggregation and analysis of volatile organic compound emissions for regional modeling. Atmos. Environ., 24A , 11071133.

    • Search Google Scholar
    • Export Citation
  • NRC, 1991: Rethinking the Ozone Problem in Urban and Regional Air Pollution. National Academy Press, 500 pp.

  • Ranzieri, A. J., and R. Thuillier, 1991: San Joaquin Valley Air Quality Study (SJVAQS) and Atmospheric Utility Signatures, Predictions and Experiments (AUSPEX): A collaborative modeling program. Proc. 84th Annual Meeting of the Air & Waste Management Association, Vancouver, BC, Canada, Air and Waste Management Association, Paper 91-70.5.

  • Sander, S. P., and Coauthors, 2003: Chemical kinetics and photochemical data for use in atmospheric studies. Evaluation Number 14, NASA JPL Publication 02-25, 334 pp.

  • Seaman, N. L., 2000: Meteorological modeling for air-quality assessments. Atmos. Environ., 34 , 22312259.

  • Seinfeld, J. H., and S. N. Pandis, 1998: Atmospheric Chemistry and Physics: From Air Pollution to Climate Change. Wiley-Interscience, 1326 pp.

    • Search Google Scholar
    • Export Citation
  • Stockwell, W. R., P. Middleton, J. S. Chang, and X. Tang, 1990: The second generation Regional Acid Deposition Model chemical mechanism for regional air quality modeling. J. Geophys. Res., 95 , D10. 1634316367.

    • Search Google Scholar
    • Export Citation
  • Tao, Z., S. M. Larson, D. J. Wuebbles, A. Williams, and M. Caughey, 2003: A summer simulation of biogenic contribution to ground-level ozone over the continental United States. J. Geophys. Res., 108 .4404, doi:10.1029/2002JD002945.

    • Search Google Scholar
    • Export Citation
  • Williams, A., M. Caughey, H-C. Huang, X-Z. Liang, K. E. Kunkel, Z. Tao, S. Larson, and D. J. Wuebbles, 2001: Comparison of emissions processing by EMS95 and SMOKE over the Midwestern U.S. 10th Int. Emission Inventory Conf. “One Atmosphere, One Inventory, Many Challenges,” Denver, CO, U.S. EPA.

  • Zhu, J., and X-Z. Liang, 2006: Regional climate model simulation of U.S. soil temperature and moisture during 1982–2002. J. Geophys. Res., 110 .D24110, doi:10.1029/2005JD006472.

    • Search Google Scholar
    • Export Citation
All Time Past Year Past 30 Days
Abstract Views 0 0 0
Full Text Views 364 144 6
PDF Downloads 105 34 5