On Estimating Dry Deposition Rates in Complex Terrain

Bruce B. Hicks Air Resources Laboratory, National Oceanic and Atmospheric Administration, Silver Spring, Maryland

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Abstract

In complex terrain, horizontal advection and filtration through a canopy can add substantially to the vertical diffusion component assumed to be the dominant transfer mechanism in conventional deposition velocity formulations. To illustrate this, three separate kinds of terrain complexity are addressed here: 1) a horizontal landscape with patches of forest, 2) a uniformly vegetated gentle hill, and 3) a mountainous area. In flat areas with plots of trees, the elevation of the standard area-weighted dry deposition velocity will likely depend on the product hn1/2, where h is the tree height and n is the number of plots per unit area. For the second case, it is proposed that the standard “flat earth” deposition velocity might need to be increased by a factor like [1 + Ra/(Rb + Rc)]1/2. For mountainous ecosystems, where no precise estimate of local dry deposition appears attainable, the actual dry deposition rate is probably bounded by the extremes associated with 1) the flat earth assumption involving aerodynamic, quasi-boundary layer, and canopy resistances as in conventional formulations, and 2) an alternative assumption that the aerodynamic resistance is zero. Such issues are of particular importance in the context of atmospheric loadings to sensitive ecosystems, where the concepts of critical loads and deposition forecasting are now of increasing relevance. They are probably of less importance if the emphasis is on air quality alone, because air quality responds slowly to changes in deposition rates. The issues addressed here are mainly appropriate in the context of air surface exchange that is not controlled by surface resistance (e.g., for deposition of easily captured chemicals such as nitric acid vapor, and perhaps for atmospheric momentum) and for chemicals that have no local sources. It is argued that dry deposition rates derived from classical applications of deposition velocities are often underestimates.

Corresponding author address: Bruce Hicks, Metcorps, P.O. Box 1510, Norris, TN 37828. Email: hicks.metcorps@gmail.com

This article included in the NOAA/EPA Golden Jubilee special collection.

Abstract

In complex terrain, horizontal advection and filtration through a canopy can add substantially to the vertical diffusion component assumed to be the dominant transfer mechanism in conventional deposition velocity formulations. To illustrate this, three separate kinds of terrain complexity are addressed here: 1) a horizontal landscape with patches of forest, 2) a uniformly vegetated gentle hill, and 3) a mountainous area. In flat areas with plots of trees, the elevation of the standard area-weighted dry deposition velocity will likely depend on the product hn1/2, where h is the tree height and n is the number of plots per unit area. For the second case, it is proposed that the standard “flat earth” deposition velocity might need to be increased by a factor like [1 + Ra/(Rb + Rc)]1/2. For mountainous ecosystems, where no precise estimate of local dry deposition appears attainable, the actual dry deposition rate is probably bounded by the extremes associated with 1) the flat earth assumption involving aerodynamic, quasi-boundary layer, and canopy resistances as in conventional formulations, and 2) an alternative assumption that the aerodynamic resistance is zero. Such issues are of particular importance in the context of atmospheric loadings to sensitive ecosystems, where the concepts of critical loads and deposition forecasting are now of increasing relevance. They are probably of less importance if the emphasis is on air quality alone, because air quality responds slowly to changes in deposition rates. The issues addressed here are mainly appropriate in the context of air surface exchange that is not controlled by surface resistance (e.g., for deposition of easily captured chemicals such as nitric acid vapor, and perhaps for atmospheric momentum) and for chemicals that have no local sources. It is argued that dry deposition rates derived from classical applications of deposition velocities are often underestimates.

Corresponding author address: Bruce Hicks, Metcorps, P.O. Box 1510, Norris, TN 37828. Email: hicks.metcorps@gmail.com

This article included in the NOAA/EPA Golden Jubilee special collection.

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  • Beier, C., P. Gundersen, and L. Rasmussen, 1992: A new method for estimation of dry deposition of particles based on throughfall measurements in a forest edge. Atmos. Environ., 26A , 15531559.

    • Search Google Scholar
    • Export Citation
  • Bradley, E. F., 1980: An experimental study of the profiles of wind speed, shearing stress and turbulence at the crest of a large hill. Quart. J. Roy. Meteor. Soc., 106 , 101124.

    • Search Google Scholar
    • Export Citation
  • Crawford, T. L., R. J. Dobosy, R. T. McMillen, C. A. Vogel, and B. B. Hicks, 1996: Air-surface exchange measurements in heterogeneous regions: Extending tower observations with spatial structure observed from small aircraft. Global Change Biol., 2 , 275285.

    • Search Google Scholar
    • Export Citation
  • Desjardins, R. L., and Coauthors, 1997: Scaling up flux measurements for the boreal forest using aircraft-tower combinations. J. Geophys. Res., 102 , 2912529134.

    • Search Google Scholar
    • Export Citation
  • Finnigan, J. J., and S. E. Belcher, 2004: Flow over a hill covered with a plant canopy. Quart. J. Roy. Meteor. Soc., 130 , 129.

  • Hicks, B. B., 1995: On the determination of total deposition to remote areas. Acid Rain Research: Do We Have Enough Answers, G. J. Heij and J. W. Erisman, Eds., Elsevier Press, 163–173.

    • Search Google Scholar
    • Export Citation
  • Hicks, B. B., 2001: Areal measurements of ozone, water, and heat fluxes over land with different surface complexity, using aircraft. Water Air Soil Pollut. Focus, 1 , 213222.

    • Search Google Scholar
    • Export Citation
  • Hicks, B. B., D. D. Baldocchi, T. P. Meyers, D. R. Matt, and R. P. Hosker Jr., 1987: A preliminary multiple resistance routine for deriving dry deposition velocities from measured quantities. Water Air Soil Pollut., 36 , 311330.

    • Search Google Scholar
    • Export Citation
  • Jackson, P. S., and J. C. R. Hunt, 1975: Turbulent wind flow over a low hill. Quart. J. Roy. Meteor. Soc., 101 , 929955.

  • Katul, G. G., J. J. Finnegan, D. Poggi, R. Leuning, and S. E. Belcher, 2006: The influence of hilly terrain on canopy–atmosphere carbon dioxide exchange. Bound.-Layer Meteor., 118 , 189216.

    • Search Google Scholar
    • Export Citation
  • Langan, S. J., J. Hall, B. Reynolds, M. Broadmeadow, M. Hornung, and M. S. Cresser, 2004: The development of an approach to assess critical loads of acidity for woodland habitats in Great Britain. Hydrol. Earth System Sci., 8 , 355365.

    • Search Google Scholar
    • Export Citation
  • Lenschow, D. H., R. Pearson, and B. B. Stankov, 1982: Measurements of ozone vertical flux to ocean and forest. J. Geophys. Res., 87 , 88338837.

    • Search Google Scholar
    • Export Citation
  • Lindberg, S. E., and C. T. Garten, 1989: Sources of sulphur in forest canopy throughfall. Nature, 336 , 148151.

  • Lovett, G. M., and S. E. Lindberg, 1984: Dry deposition and canopy exchange in a mixed oak forest as determined by analysis of throughfall. J. Appl. Ecol., 21 , 10131027.

    • Search Google Scholar
    • Export Citation
  • Ma, J., and S. M. Daggupaty, 2000: Effective dry deposition velocities for gases and particles over heterogeneous terrain. J. Appl. Meteor., 39 , 13791390.

    • Search Google Scholar
    • Export Citation
  • Mason, P. J., and J. C. King, 1984: Atmospheric flow over a succession of nearly two-dimensional ridges and valleys. Quart. J. Roy. Meteor. Soc., 110 , 821845.

    • Search Google Scholar
    • Export Citation
  • McMillen, R. T., 1990: Estimating the spatial variability of trace gas deposition velocities. NOAA Tech. Memo. ERL-ARL-181, 37 pp.

  • Meroney, R. N., 1980: Wind-tunnel simulation of the flow over hills and complex terrain. J. Indust. Aerodyn., 5 , 297321.

  • Meyers, T. P., W. T. Luke, and J. L. Meisinger, 2006: Fluxes of ammonia and sulfate over maize using relaxed eddy accumulation. Agric. For. Meteor., 136 , 203213.

    • Search Google Scholar
    • Export Citation
  • Monti, P., H. J. S. Fernando, M. Princevac, W. C. Chan, T. A. Kowalewski, and E. R. Pardyiak, 2002: Observations of flow and turbulence in the nocturnal boundary layer over a slope. J. Atmos. Sci., 59 , 25132534.

    • Search Google Scholar
    • Export Citation
  • Ohba, R., N. Ukeguchi, S. Kakishima, and B. Lamb, 1990: Wind tunnel experiment of gas diffusion in stably stratified flow over a complex terrain. Atmos. Environ., 24 , 19872001.

    • Search Google Scholar
    • Export Citation
  • Ross, A. N., and S. B. Vosper, 2005: Neutral turbulent flow over forested hills. Quart. J. Roy. Meteor. Soc., 131 , 18411862.

  • Sheih, C. M., M. L. Wesely, and B. B. Hicks, 1979: Estimated dry deposition velocities of sulfur over the eastern United States and surrounding regions. Atmos. Environ., 13 , 13611368.

    • Search Google Scholar
    • Export Citation
  • Slinn, W. G. N., 1982: Predictions for particle deposition to vegetative surfaces. Atmos. Environ., 16 , 17851794.

  • Snyder, W. H., 1990: Fluid modeling applied to atmospheric diffusion in complex terrain. Atmos. Environ., 24A , 20712088.

  • Weathers, K. C., G. M. Lovett, and P. Lathrop, 2000: The effect of landscape features on deposition to Hunter Mountain, Catskill Mountains, New York. Ecol. Appl., 10 , 528540.

    • Search Google Scholar
    • Export Citation
  • Wood, N., 1995: The onset of separation in neutral, turbulent flow over hills. Bound.-Layer Meteor., 76 , 137164.

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