Abstract
In this paper, accurate UV polarization measurements are performed on a volcanic ash cloud after long-range transport at Lyon, France (45.76°N, 4.83°E). The volcanic particles are released from the mid-April 2010 eruption of the Eyjafjallajökull Icelandic volcano (63.63°N, 19.62°W). The aerosol UV depolarization, which arises from nonspherical volcanic ash particles, serves as an independent means to discriminate ash from nonash particles in the volcanic cloud. This discrimination is only feasible if the intrinsic ash particle depolarization ration δash is accurately determined. In this paper, the δash value [δash = (40.5 ± 2.0)%] is derived from literature laboratory measurements on a scattering matrix to ensure ash particle specificity. It is shown that traditional approaches, based on direct lidar depolarization ratio δa measurements, are only valid very close to the source region, because δa may be very different from δash, when nonash particles are present. For the first time, observed lidar depolarization ratios, in the range from a few percent to 40%, are hence interpreted in comparison with δash taken as a reference. It is then shown how to use the sensitive and accurate UV polarization measurements to access to the size-averaged number concentration vertical profile of volcanic ash particles in the troposphere. Vertical profiles of the backscattering coefficient specific to volcanic ash particles, providing altitude-resolved ash particle number concentrations, are presented in the troposphere after optical scattering computation. This new methodology can be applied to other aerosols events and for other optical remote sensing experiments.
