Droplets to Drops by Turbulent Coagulation

N. Riemer Department of Mechanical and Aeronautical Engineering, University of California, Davis, Davis, California

Search for other papers by N. Riemer in
Current site
Google Scholar
PubMed
Close
and
A. S. Wexler Department of Mechanical and Aeronautical Engineering, Department of Civil and Environmental Engineering, and Department of Land, Air, and Water Resources, University of California, Davis, Davis, California

Search for other papers by A. S. Wexler in
Current site
Google Scholar
PubMed
Close
Restricted access

Abstract

This study addresses two central problems in cloud microphysics. The first is the source of large droplets, which initiates the rapid production of warm rain. The second is the broadening of the cloud droplet spectrum at both tails of the spectrum. The study explores how in-cloud turbulence can help to close the gaps in our understanding. With box model simulations, the development of cloud droplet spectra is calculated using a coagulation kernel that recently has been derived from direct numerical simulations. This kernel includes both the effect of turbulence on the relative velocities of the droplets and on the local increases in droplet concentration, the so-called accumulation effect. Under the assumption that this kernel can be extrapolated to atmospheric Reynolds numbers, the results show that for typical atmospheric conditions, the turbulent coagulation kernel is several orders of magnitude larger than the sedimentation kernel for droplets smaller then 100 μm. While for calm air after 30-min simulation time, only 7% of the total mass is found in droplets with sizes over 100 μm, this increases to 79% for a dissipation rate of 100 cm2 s−3 and 96% for 300 cm2 s−3 if a combined sedimentation and turbulent kernel is employed that assumes that the sedimentation and turbulent kernel can be added. Hence, moderate turbulence can enhance significantly the formation of large droplets. Furthermore, a time-scale analysis shows that broadening at the upper end of the spectrum is caused by turbulent coagulation whereas thermodynamic effects are responsible for broadening at the lower end.

* Current affiliation: Center for Turbulence Research, Stanford University, Stanford, California

Corresponding author: A. S. Wexler, University of California, Davis, One Shields Avenue, Davis, CA 95616. Email: aswexler@ucdavis.edu

Abstract

This study addresses two central problems in cloud microphysics. The first is the source of large droplets, which initiates the rapid production of warm rain. The second is the broadening of the cloud droplet spectrum at both tails of the spectrum. The study explores how in-cloud turbulence can help to close the gaps in our understanding. With box model simulations, the development of cloud droplet spectra is calculated using a coagulation kernel that recently has been derived from direct numerical simulations. This kernel includes both the effect of turbulence on the relative velocities of the droplets and on the local increases in droplet concentration, the so-called accumulation effect. Under the assumption that this kernel can be extrapolated to atmospheric Reynolds numbers, the results show that for typical atmospheric conditions, the turbulent coagulation kernel is several orders of magnitude larger than the sedimentation kernel for droplets smaller then 100 μm. While for calm air after 30-min simulation time, only 7% of the total mass is found in droplets with sizes over 100 μm, this increases to 79% for a dissipation rate of 100 cm2 s−3 and 96% for 300 cm2 s−3 if a combined sedimentation and turbulent kernel is employed that assumes that the sedimentation and turbulent kernel can be added. Hence, moderate turbulence can enhance significantly the formation of large droplets. Furthermore, a time-scale analysis shows that broadening at the upper end of the spectrum is caused by turbulent coagulation whereas thermodynamic effects are responsible for broadening at the lower end.

* Current affiliation: Center for Turbulence Research, Stanford University, Stanford, California

Corresponding author: A. S. Wexler, University of California, Davis, One Shields Avenue, Davis, CA 95616. Email: aswexler@ucdavis.edu

Save
  • Abrahamson, J., 1975: Collision rates of small particles in a vigorously turbulent fluid. Chem. Eng. Sci., 30 , 13711379.

  • Arenberg, D., 1939: Turbulence as the major factor in the growth of cloud drops. Bull. Amer. Meteor. Soc., 20 , 444448.

  • Beard, K. V., and H. T. Ochs, 1993: Warm-rain initiation: An overview of microphysical mechanisms. J. Appl. Meteor., 32 , 608625.

  • Belin, F., J. Maurer, P. Tabeling, and H. Willaime, 1997: Velocity gradient distributions in fully developed turbulence: An experimental study. Phys. Fluids, 9 , 38433850.

    • Search Google Scholar
    • Export Citation
  • Berry, E. X., 1967: Cloud droplet growth by collection. J. Atmos. Sci., 24 , 688700.

  • Bott, A., 1998: A flux method for the numerical solution of the stochastic collection equation. J. Atmos. Sci., 55 , 22842293.

  • Brenguier, J-L., and L. Chaumat, 2001: Droplet spectra broadening in cumulus clouds. Part I: Broadening in adiabatic cores. J. Atmos. Sci., 58 , 628641.

    • Search Google Scholar
    • Export Citation
  • Butuirat, F., and M. Kielkiewicz, 1996: On additivity of coagulation kernels. Ann. Nucl. Energy, 23 , 10911096.

  • de Almeida, F. C., 1976: The collisional problem of cloud droplets moving in a turbulent environment—Part I: A method of solution. J. Atmos. Sci., 33 , 15711578.

    • Search Google Scholar
    • Export Citation
  • Friedlander, S. K., 1977: Smoke, Dust, and Haze. Wiley, 317 pp.

  • Grabowski, W. W., and P. Vaillancourt, 1999: Comments on “Preferential concentration of cloud droplets by turbulence: Effects of the early evolution of cumulus cloud droplet spectra.”. J. Atmos. Sci., 56 , 14331436.

    • Search Google Scholar
    • Export Citation
  • Grover, S. N., and H. R. Pruppacher, 1985: The effect of vertical turbulent fluctuations in the atmosphere on the collection of aerosol particles by cloud droplets. J. Atmos. Sci., 42 , 23052318.

    • Search Google Scholar
    • Export Citation
  • Hall, W. D., 1980: A detailed microphysical model within a two-dimensional dynamic framework: Model description and preliminary results. J. Atmos. Sci., 37 , 24862507.

    • Search Google Scholar
    • Export Citation
  • Jonas, P. R., and P. Goldsmith, 1972: The collection efficiencies of small droplets falling through a sheared air flow. J. Fluid Mech., 52 , 593608.

    • Search Google Scholar
    • Export Citation
  • Kerminen, V-M., and A. S. Wexler, 1995: Growth laws for atmospheric aerosol particles: An examination of the bimodality of the accumulation mode. Atmos. Environ., 29 , 32623275.

    • Search Google Scholar
    • Export Citation
  • Khain, A. P., and M. B. Pinsky, 1995: Drop inertia and its contribution to turbulent coalescence in convective clouds. Part I: Drop fall in the flow with random horizontal velocity. J. Atmos. Sci., 52 , 196206.

    • Search Google Scholar
    • Export Citation
  • Khain, A. P., and M. B. Pinsky, 1997: Turbulence effects on the collision kernel. II: Increase of the swept volume of colliding drops. Quart. J. Roy. Meteor. Soc., 123 , 15431560.

    • Search Google Scholar
    • Export Citation
  • Khain, A., M. Ovtchinnikov, M. Pinsky, A. Pokrovsky, and H. Krugliak, 2000: Notes of the state-of-the-art numerical modeling of cloud microphysics. Atmos. Res., 55 , 159224.

    • Search Google Scholar
    • Export Citation
  • Kostinski, A. B., and R. A. Shaw, 2001: Scale-dependent droplet clustering in turbulent clouds. J. Fluid Mech., 434 , 389398.

  • Kruis, F. E., and K. A. Kusters, 1997: The collision rate of particles in turbulent flow. Chem. Eng. Commun., 158 , 201230.

  • Lee, I. Y., and H. R. Pruppacher, 1977: A comparative study on the growth of cloud drops by condensation using an air parcel model with and without entrainment. Pure Appl. Geophys., 115 , 523545.

    • Search Google Scholar
    • Export Citation
  • MacPherson, J. I., and G. A. Isaac, 1977: Turbulent characteristics of some Canadian cumulus clouds. J. Appl. Meteor., 16 , 8190.

  • Majeed, M. A., and A. S. Wexler, 2001: Microphysics of aqueous droplets in clouds and fogs as applied to PM-fine modeling. Atmos. Environ., 35 , 16391653.

    • Search Google Scholar
    • Export Citation
  • Maxey, M. R., 1987: The gravitational settling of particles in homogeneous turbulence and random flow fields. J. Fluid Mech., 174 , 441465.

    • Search Google Scholar
    • Export Citation
  • Neizvestny, A. I., and A. G. Kobzunenko, 1986: Effect of small-scale turbulence on the coagulation growth rate of cloud droplets. Izv. Akad. Nauk SSSR, Fiz. Atmos. Okeana, 22 , 626633.

    • Search Google Scholar
    • Export Citation
  • Park, S. H., F. E. Kruis, K. W. Lee, and H. Fissan, 2002: Evolution of particle size distributions due to turbulent and Brownian coagulation. Aerosol Sci. Technol., 36 , 419432.

    • Search Google Scholar
    • Export Citation
  • Pinsky, M. B., and A. Khain, 1996: Simulations of drop fall in a homogeneous isotropic turbulent flow. Atmos. Res., 40 , 223259.

  • Pinsky, M., and A. Khain, 1997a: Formation of inhomogeneity in drop concentration induced by the inertia of drops falling in a turbulent flow, and the influence of the inhomogeneity on the drop-spectrum broadening. Quart. J. Roy. Meteor. Soc., 123 , 165186.

    • Search Google Scholar
    • Export Citation
  • Pinsky, M., and A. Khain, 1997b: Turbulence effect on the collision kernel. I: Formation of velocity deviations of drops falling within a turbulent three-dimensional flow. Quart. J. Roy. Meteor. Soc., 123 , 15171542.

    • Search Google Scholar
    • Export Citation
  • Pinsky, M. B., and A. P. Khain, 1997c: Turbulence effects on droplet growth and size distribution in clouds—A review. J. Aerosol Sci., 28 , 11771214.

    • Search Google Scholar
    • Export Citation
  • Pinsky, M., and A. P. Khain, 2001: Fine structure of cloud droplet concentration as seen from the Fast-FSSP measurements. Part I: Method of analysis and preliminary results. J. Appl. Meteor., 40 , 15151537.

    • Search Google Scholar
    • Export Citation
  • Pinsky, M., A. Khain, and M. Shapiro, 1999: Collisions of small drops in a turbulent flow. Part I: Collision efficiency. Problem formulation and preliminary results. J. Atmos. Sci., 56 , 25852600.

    • Search Google Scholar
    • Export Citation
  • Pinsky, M., A. Khain, and M. Shapiro, 2000: Stochastic effects of cloud droplet hydrodynamic interaction in a turbulent flow. Atmos. Res., 53 , 131169.

    • Search Google Scholar
    • Export Citation
  • Pruppacher, H. R., and J. D. Klett, 1997: Microphysics of Clouds and Precipitation. 2d ed. Kluwer Academic, 954 pp.

  • Reade, W. C., and L. R. Collins, 2000: Effect of preferential concentration on turbulent collision rates. Phys. Fluids, 12 , 25302540.

    • Search Google Scholar
    • Export Citation
  • Rogers, R. R., and M. K. Yau, 1989: A Short Course in Cloud Physics. 3d ed. Butterworth-Heinemann, 290 pp.

  • Saffman, P. G., and J. S. Turner, 1956: On the collision of drops in turbulent clouds. J. Fluid Mech., 1 , 1630.

  • Shaw, R. A., 2000: Supersaturation intermittency in turbulent clouds. J. Atmos. Sci., 57 , 34523456.

  • Shaw, R. A., 2003: Particle–turbulence interactions in atmospheric clouds. Annu. Rev. Fluid Mech., 35 , 183227.

  • Squires, K. D., and J. K. Eaton, 1991: Preferential concentration of particles by turbulence. Phys. Fluids, A3 , 11691179.

  • Sundaram, S., and L. R. Collins, 1996: Numerical considerations in simulating a turbulent suspension of finite-volume particles. J. Comput. Phys., 124 , 337350.

    • Search Google Scholar
    • Export Citation
  • Sundaram, S., and L. R. Collins, 1997: Collision statistics in an isotropic, particle-laden turbulent suspension. I. Direct numerical simulations. J. Fluid Mech., 335 , 75110.

    • Search Google Scholar
    • Export Citation
  • Vaillancourt, P. A., and M. K. Yau, 2000: Review of particle–turbulence interactions and consequences for cloud physics. Bull. Amer. Meteor. Soc., 81 , 285298.

    • Search Google Scholar
    • Export Citation
  • Vaillancourt, P. A., M. K. Yau, P. Bartello, and W. W. Grabowski, 2002: Microscopic approach to cloud droplet growth by condensation. Part II: Turbulence, clustering and condensational growth. J. Atmos. Sci., 59 , 34213435.

    • Search Google Scholar
    • Export Citation
  • Vohl, O., S. K. Mitra, S. C. Wurzler, and H. R. Pruppacher, 1999: A wind tunnel study of the effects of turbulence on the growth of cloud drops by collision and coalescence. J. Atmos. Sci., 56 , 40884099.

    • Search Google Scholar
    • Export Citation
  • Wang, L-P., and M. R. Maxey, 1993: Settling velocity and concentration distribution of heavy particles in homogeneous isotropic turbulence. J. Fluid Mech., 335 , 2768.

    • Search Google Scholar
    • Export Citation
  • Wang, L-P., A. S. Wexler, and Y. Zhou, 1998: Statistical mechanical description of turbulent coagulation. Phys. Fluids, 10 , 26472651.

    • Search Google Scholar
    • Export Citation
  • Wang, L-P., A. S. Wexler, and Y. Zhou, 2000: Statistical mechanical description and modelling of turbulent collision of inertial particles. J. Fluid Mech., 415 , 117153.

    • Search Google Scholar
    • Export Citation
  • Warner, J., 1969: The microstructure of cumulus cloud. Part I. General features of the droplet spectrum. J. Atmos. Sci., 26 , 10491065.

    • Search Google Scholar
    • Export Citation
  • Williams, J. J. E., and R. I. Crane, 1983: Particle collision rate in turbulent flow. Int. J. Multiphase Flow, 9 , 421435.

  • Woods, J. D., P. Goldsmith, and J. C. Drake, 1972: Coalescence in a turbulent cloud. Quart. J. Roy. Meteor. Soc., 98 , 135149.

  • Yin, Y., Z. Levin, T. Reisin, and S. Tzivion, 2000: The effects of giant cloud condensation nuclei on the development of precipitation in convective clouds: A numerical study. Atmos. Res., 53 , 91116.

    • Search Google Scholar
    • Export Citation
  • Zhou, Y., A. S. Wexler, and L-P. Wang, 2001: Modelling turbulent collision of bidisperse inertial particles. J. Fluid Mech., 433 , 77104.

    • Search Google Scholar
    • Export Citation
All Time Past Year Past 30 Days
Abstract Views 0 0 0
Full Text Views 252 76 5
PDF Downloads 241 72 7