The Atmospheric Radiation Measurement (ARM) Climate Research Facility (www.arm.gov) provides atmospheric observations from diverse climatic regimes around the world. Because it is a U.S. Department of Energy (DOE) user facility, ARM data are freely available to anyone through the ARM Data Archive. With 20 years of operations, the facility recently added two mobile facilities and an aerial facility to its network of fixed-location sites. Research using ARM data has led to advances in areas ranging from radiative transfer to cloud microphysics. The American Recovery and Reinvestment Act of 2009 allowed ARM to enhance its observational capabilities with a broad array of new instruments at its fixed and mobile sites and the aerial facility. Instruments include scanning radars; water vapor, cloud/aerosol extinction, and Doppler lidars; aerosol instruments for measuring optical, physical, and chemical properties; and aircraft probes for measuring cloud and aerosol properties. Taking full advantage of these instruments will involve the development of complex data products. This work is underway but will benefit from engagement with the broader scientific community. This article describes the current status of the ARM research capabilities with an emphasis on developments over the past eight years since ARM was designated a DOE scientific user facility, reviews some of scientific advances made using the ARM Facility over the past two decades, and describes the new measurement capabilities and adaptations of the ARM facility to make effective use of these capabilities.