Abstract
Sea salt aerosols play a dual role in affecting the atmospheric radiative balance. Directly, sea salt particles scatter the incoming solar radiation and absorb the outgoing terrestrial radiation. By acting as cloud condensation nuclei, sea salt aerosols indirectly modulate the atmospheric radiative budget through their effective contribution to cloud formation. Using the Canadian Aerosol Module (CAM)–Canadian Centre for Climate Modelling and Analysis (CCCma) GCM, version 3 (GCM3) framework, the direct as well as the indirect shortwave (SW) radiative effects of sea salt aerosols are simulated. The model results herein suggest that sea salt aerosols exert a significant direct radiative effect over oceanic regions, with seasonal means in the range from −2 to −3 W m−2 over the Southern Ocean. Globally, sea salt’s SW indirect effect (annual mean −0.38 W m−2) is found to be less than its direct effect (annual mean −0.65 W m−2). However, sea salt’s indirect effect is found to be far stronger over the Southern Hemisphere than over the Northern Hemisphere, especially over the Southern Ocean with seasonal means around −4 W m−2, which exceed its direct effect. The model results herein suggest that sea salt aerosols significantly modulate the atmospheric radiation budget over oceanic regions and need to be accounted for in global climate models.
Corresponding author address: Tarek Ayash, Dept. of Chemical Engineering and Applied Chemistry, University of Toronto, 200 College Street, Toronto, ON M5S 3E5, Canada. Email: tarek.ayash@utoronto.ca
