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- Author or Editor: Zhanqing Li x
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Abstract
Global datasets of surface radiation budget (SRB) have been obtained from satellite programs. These satellite-based estimates need validation with ground-truth observations. This study validates the estimates of monthly mean surface insolation contained in two satellite-based SRB datasets with the surface measurements made at worldwide radiation stations from the Global Energy Balance Archive (GEBA). One dataset was developed from the Earth Radiation Budget Experiment (ERBE) using the algorithm of Li et al. (ERBE/SRB), and the other from the International Satellite Cloud Climatology Project (ISCCP) using the algorithm of Pinker and Laszlo and that of Staylor (GEWEX/SRB). Since the ERBE/SRB data contain the surface net solar radiation only, the values of surface insolation were derived by making use of the surface albedo data contained in the GEWEX/SRB product. The resulting surface insolation has a bias error near zero and a root-mean-square error (RMSE) between 8 and 28 W m−2. The RMSE is mainly associated with poor representation of surface observations within a grid cell. When the number of surface observations are sufficient, the random error is estimated to be about 5 W m−2 with present satellite-based estimates. In addition to demonstrating the strength of the retrieving method, the small random error demonstrates how well the ERBE derives the monthly mean fluxes at the top of the atmosphere (TOA). A larger scatter is found for the comparison of transmissivity than for that of insolation. Month to month comparison of insolation reveals a weak seasonal trend in bias error with an amplitude of about 3 W m−2. As for the insolation data from the GEWEX/SRB, larger bias errors of 5–10 W m−2 are evident with stronger seasonal trends and almost identical RMSEs.
Abstract
Global datasets of surface radiation budget (SRB) have been obtained from satellite programs. These satellite-based estimates need validation with ground-truth observations. This study validates the estimates of monthly mean surface insolation contained in two satellite-based SRB datasets with the surface measurements made at worldwide radiation stations from the Global Energy Balance Archive (GEBA). One dataset was developed from the Earth Radiation Budget Experiment (ERBE) using the algorithm of Li et al. (ERBE/SRB), and the other from the International Satellite Cloud Climatology Project (ISCCP) using the algorithm of Pinker and Laszlo and that of Staylor (GEWEX/SRB). Since the ERBE/SRB data contain the surface net solar radiation only, the values of surface insolation were derived by making use of the surface albedo data contained in the GEWEX/SRB product. The resulting surface insolation has a bias error near zero and a root-mean-square error (RMSE) between 8 and 28 W m−2. The RMSE is mainly associated with poor representation of surface observations within a grid cell. When the number of surface observations are sufficient, the random error is estimated to be about 5 W m−2 with present satellite-based estimates. In addition to demonstrating the strength of the retrieving method, the small random error demonstrates how well the ERBE derives the monthly mean fluxes at the top of the atmosphere (TOA). A larger scatter is found for the comparison of transmissivity than for that of insolation. Month to month comparison of insolation reveals a weak seasonal trend in bias error with an amplitude of about 3 W m−2. As for the insolation data from the GEWEX/SRB, larger bias errors of 5–10 W m−2 are evident with stronger seasonal trends and almost identical RMSEs.
Abstract
Measurements of radiation budgets, both at the top of the atmosphere (TOA) and at the surface, are essential to understanding the earth's climate. The TOA budgets can, in principle, be measured directly from satellites, while on a global scale surface budgets need to be deduced from TOA measurements. Most methods of inferring surface solar-radiation budgets from satellite measurements are applicable to particular scene types or geographic locations, and none is valid over highly reflective surfaces such as ice or snow. In addition, the majority of models require inputs such as cloud-optical thickness that are usually not known.
Extensive radiative transfer modeling for different surface, atmospheric, and cloud conditions suggests a linear relationship between the TOA-reflected flux and the flux absorbed at the surface for a fixed solar zenith angle (SZA). The linear relationship is independent of cloud-optical thickness and surface albedo. Sensitivity tests show that the relationship depends strongly on SZA and moderately on precipitable water and cloud type. The linear relationship provides a simple parameterization to estimate surface-absorbed flux from satellite-measured reflected flux at the TOA. Unlike other models, the present model makes explicit use of the SZA. Precipitable water is included as a secondary parameter. Surface-absorbed fluxes deduced from this simple parameterized model generally agree to within 10 W m−2 with the absorbed fluxes determined from detailed radiative transfer calculations, without including information on the presence or absence of cloud, cloud type, optical thickness, or surface type.
Abstract
Measurements of radiation budgets, both at the top of the atmosphere (TOA) and at the surface, are essential to understanding the earth's climate. The TOA budgets can, in principle, be measured directly from satellites, while on a global scale surface budgets need to be deduced from TOA measurements. Most methods of inferring surface solar-radiation budgets from satellite measurements are applicable to particular scene types or geographic locations, and none is valid over highly reflective surfaces such as ice or snow. In addition, the majority of models require inputs such as cloud-optical thickness that are usually not known.
Extensive radiative transfer modeling for different surface, atmospheric, and cloud conditions suggests a linear relationship between the TOA-reflected flux and the flux absorbed at the surface for a fixed solar zenith angle (SZA). The linear relationship is independent of cloud-optical thickness and surface albedo. Sensitivity tests show that the relationship depends strongly on SZA and moderately on precipitable water and cloud type. The linear relationship provides a simple parameterization to estimate surface-absorbed flux from satellite-measured reflected flux at the TOA. Unlike other models, the present model makes explicit use of the SZA. Precipitable water is included as a secondary parameter. Surface-absorbed fluxes deduced from this simple parameterized model generally agree to within 10 W m−2 with the absorbed fluxes determined from detailed radiative transfer calculations, without including information on the presence or absence of cloud, cloud type, optical thickness, or surface type.
Abstract
Several observational datasets were used to assess the quality of the radiative characteristics of the Canadian Climate Centre (CCC) second-generation GCM. The GCM data were obtained from the Atmospheric Model Intercomparison Project (AMIP) simulation. Data corresponding to the period January 1985 through December 1988 were examined since this period of the AMIP simulation overlaps with the Earth Radiation Budget Experiment (ERBE) and the International Satellite Cloud Climatology Project (ISCCP) datasets. Attention was given to mean January and July conditions. Optical properties of surfaces, clear skies, and cloudy skies were examined.
Ocean albedos are too high in the Tropics and too low in the polar regions relative to surface observations and theoretical estimates. Compared to a satellite-derived dataset, however, they are slightly underestimated. Throughout much of the Sahara and Saudi Deserts surface albedos are too low, while for much of Western Australia they are too high. Excessive amounts of snow in Southeast Asia seem to have been sustained by a localized snow albedo feedback related to inappropriate snow albedo specification and a weak masking effect by vegetation. Neglect of freshwater lakes in the Canadian Shield leads to negative and positive albodo anomalies in winter and summer, respectively.
Like many GCMS, the CCC model has too little atmospheric H20 vapor. This results in too much outgoing longwave radiation from clear skies, especially in the Tropics. Neglect of all trace gases except for C02 and weak H20 vapor absorption exacerbate this bias.
Assessment of the radiative properties of clouds was done very generally at this stage due to lack of confidence in available observational data. Total and high cloud fractions were compared to ISCCP estimates. Warm tropical oceans appear to have too much high cloud. Evaluation of low cloud fraction is less straightforward but it is clear that due to lack of a shallow convection scheme and coarse vertical resolution, the GCM is almost devoid of low clouds over cool oceans.
Cloud radiative forcing CRF from the GCM was compared to CRF obtained from ERBE data. Globally averaged, net CRF is in excellent accord with observations but shortwave and longwave CRFs are too strong. Zonal averages, however, reveal biases in which clouds act to cool the Tropics too much and cool the high latitudes too little during summer, yet they warm polar regions too much during winter. Regional examination shows that these biases are confined largely to oceans. Tropical oceans have excessive shortwave CRF despite good total cloud amounts. This may be due to neglect of cloud geometry effects on solar radiative transfer.
Abstract
Several observational datasets were used to assess the quality of the radiative characteristics of the Canadian Climate Centre (CCC) second-generation GCM. The GCM data were obtained from the Atmospheric Model Intercomparison Project (AMIP) simulation. Data corresponding to the period January 1985 through December 1988 were examined since this period of the AMIP simulation overlaps with the Earth Radiation Budget Experiment (ERBE) and the International Satellite Cloud Climatology Project (ISCCP) datasets. Attention was given to mean January and July conditions. Optical properties of surfaces, clear skies, and cloudy skies were examined.
Ocean albedos are too high in the Tropics and too low in the polar regions relative to surface observations and theoretical estimates. Compared to a satellite-derived dataset, however, they are slightly underestimated. Throughout much of the Sahara and Saudi Deserts surface albedos are too low, while for much of Western Australia they are too high. Excessive amounts of snow in Southeast Asia seem to have been sustained by a localized snow albedo feedback related to inappropriate snow albedo specification and a weak masking effect by vegetation. Neglect of freshwater lakes in the Canadian Shield leads to negative and positive albodo anomalies in winter and summer, respectively.
Like many GCMS, the CCC model has too little atmospheric H20 vapor. This results in too much outgoing longwave radiation from clear skies, especially in the Tropics. Neglect of all trace gases except for C02 and weak H20 vapor absorption exacerbate this bias.
Assessment of the radiative properties of clouds was done very generally at this stage due to lack of confidence in available observational data. Total and high cloud fractions were compared to ISCCP estimates. Warm tropical oceans appear to have too much high cloud. Evaluation of low cloud fraction is less straightforward but it is clear that due to lack of a shallow convection scheme and coarse vertical resolution, the GCM is almost devoid of low clouds over cool oceans.
Cloud radiative forcing CRF from the GCM was compared to CRF obtained from ERBE data. Globally averaged, net CRF is in excellent accord with observations but shortwave and longwave CRFs are too strong. Zonal averages, however, reveal biases in which clouds act to cool the Tropics too much and cool the high latitudes too little during summer, yet they warm polar regions too much during winter. Regional examination shows that these biases are confined largely to oceans. Tropical oceans have excessive shortwave CRF despite good total cloud amounts. This may be due to neglect of cloud geometry effects on solar radiative transfer.
Abstract
A parameterization that relates the reflected solar flux at the top of the atmosphere to the net solar flux at the surface in terms of only the column water vapor amount and the solar zenith angle was tested against surface observations. Net surface fluxes deduced from coincidental collocated satellite-measured radiances and from measurements from towers in Boulder during summer and near Saskatoon in winter have mean differences of about 2 W m−2, regardless of whether the sky is clear or cloudy. Furthermore, comparisons between the net
Abstract
A parameterization that relates the reflected solar flux at the top of the atmosphere to the net solar flux at the surface in terms of only the column water vapor amount and the solar zenith angle was tested against surface observations. Net surface fluxes deduced from coincidental collocated satellite-measured radiances and from measurements from towers in Boulder during summer and near Saskatoon in winter have mean differences of about 2 W m−2, regardless of whether the sky is clear or cloudy. Furthermore, comparisons between the net
Abstract
It has been widely recognized that aerosols can modify cloud properties, but it remains uncertain how much the changes and associated variations in cloud radiative forcing are related to aerosol loading. Using 4 yr of A-Train satellite products generated from CloudSat, the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations satellite, and the Aqua satellite, the authors investigated the systematic changes of deep cloud properties and cloud radiative forcing (CRF) with respect to changes in aerosol loading over the entire tropics. Distinct correlations between CRF and aerosol loading were found. Systematic variations in both shortwave and longwave CRF with increasing aerosol index over oceans and aerosol optical depth over land for mixed-phase clouds were identified, but little change was seen in liquid clouds. The systematic changes are consistent with the microphysical effect and the aerosol invigoration effect. Although this study cannot fully exclude the influence of other factors, attempts were made to explore various possibilities to the extent that observation data available can offer. Assuming that the systematic dependence originates from aerosol effects, changes in CRF with respect to aerosol loading were examined using satellite retrievals. Mean changes in shortwave and longwave CRF from very clean to polluted conditions ranged from −192.84 to −296.63 W m−2 and from 18.95 to 46.12 W m−2 over land, respectively, and from −156.12 to −170.30 W m−2 and from 6.76 to 11.67 W m−2 over oceans, respectively.
Abstract
It has been widely recognized that aerosols can modify cloud properties, but it remains uncertain how much the changes and associated variations in cloud radiative forcing are related to aerosol loading. Using 4 yr of A-Train satellite products generated from CloudSat, the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations satellite, and the Aqua satellite, the authors investigated the systematic changes of deep cloud properties and cloud radiative forcing (CRF) with respect to changes in aerosol loading over the entire tropics. Distinct correlations between CRF and aerosol loading were found. Systematic variations in both shortwave and longwave CRF with increasing aerosol index over oceans and aerosol optical depth over land for mixed-phase clouds were identified, but little change was seen in liquid clouds. The systematic changes are consistent with the microphysical effect and the aerosol invigoration effect. Although this study cannot fully exclude the influence of other factors, attempts were made to explore various possibilities to the extent that observation data available can offer. Assuming that the systematic dependence originates from aerosol effects, changes in CRF with respect to aerosol loading were examined using satellite retrievals. Mean changes in shortwave and longwave CRF from very clean to polluted conditions ranged from −192.84 to −296.63 W m−2 and from 18.95 to 46.12 W m−2 over land, respectively, and from −156.12 to −170.30 W m−2 and from 6.76 to 11.67 W m−2 over oceans, respectively.
Abstract
Cloud droplet effective radius (DER) and liquid water path (LWP) are two key parameters for the quantitative assessment of cloud effects on the exchange of energy and water. Chang and Li presented an algorithm using multichannel measurements made at 3.7, 2.1, and 1.6 μm to retrieve a cloud DER vertical profile for improved cloud LWP estimation. This study applies the multichannel algorithm to the NASA Moderate Resolution Imaging Spectroradiometer (MODIS) data on the Aqua satellite, which also carries the Advanced Microwave Scanning Radiometer (AMSR-E) for measuring cloud LWP and precipitation. By analyzing one day of coincident MODIS and AMSR-E observations over the tropical oceans between 40°S and 40°N for overcast warm clouds (>273 K) having optical depths between 3.6 and 23, the effects of DER vertical variation on the MODIS-derived LWP are reported. It is shown that the LWP tends to be overestimated if the DER increases with height within the cloud and underestimated if the DER decreases with height within the cloud. Despite the uncertainties in both MODIS and AMSR-E retrievals, the result shows that accounting for the DER vertical variation reduces the mean biases and root-mean-square errors between the MODIS- and AMSR-E–derived LWPs. Besides, the manner in which the DER changes with height has the potential for differentiating precipitative and nonprecipitative warm clouds. For precipitating clouds, the DER at the cloud top is substantially smaller than the DER at the cloud base. For nonprecipitating clouds, however, the DER differences between the cloud top and the cloud base are much less.
Abstract
Cloud droplet effective radius (DER) and liquid water path (LWP) are two key parameters for the quantitative assessment of cloud effects on the exchange of energy and water. Chang and Li presented an algorithm using multichannel measurements made at 3.7, 2.1, and 1.6 μm to retrieve a cloud DER vertical profile for improved cloud LWP estimation. This study applies the multichannel algorithm to the NASA Moderate Resolution Imaging Spectroradiometer (MODIS) data on the Aqua satellite, which also carries the Advanced Microwave Scanning Radiometer (AMSR-E) for measuring cloud LWP and precipitation. By analyzing one day of coincident MODIS and AMSR-E observations over the tropical oceans between 40°S and 40°N for overcast warm clouds (>273 K) having optical depths between 3.6 and 23, the effects of DER vertical variation on the MODIS-derived LWP are reported. It is shown that the LWP tends to be overestimated if the DER increases with height within the cloud and underestimated if the DER decreases with height within the cloud. Despite the uncertainties in both MODIS and AMSR-E retrievals, the result shows that accounting for the DER vertical variation reduces the mean biases and root-mean-square errors between the MODIS- and AMSR-E–derived LWPs. Besides, the manner in which the DER changes with height has the potential for differentiating precipitative and nonprecipitative warm clouds. For precipitating clouds, the DER at the cloud top is substantially smaller than the DER at the cloud base. For nonprecipitating clouds, however, the DER differences between the cloud top and the cloud base are much less.
Abstract
The present study investigates the interdecadal variation of precipitation over the Hengduan Mountains (HM) during rainy seasons from various reanalysis and observational datasets. Based on a moving t test and Lepage test, an obvious rainfall decrease is identified around 2004/05. The spatial distribution of the rainfall changes exhibits large and significant precipitation deficits over the southern HM, with notable anomalous lower-level easterly divergent winds along the southern foothills of the Himalayas (SFH). The anomalous easterlies are located at the northern edge of two cyclones, with two centers of positive rainfall anomalies over the west coast of India (WCI) and the Bay of Bengal (BOB). Observational evidence and numerical experiments demonstrate that the decadal changes of SST over the WP and WIO suppress rainfall over the eastern Indian Ocean (EIO) through large-scale circulation adjustment. The EIO dry anomalies trigger the cross-equatorial anticyclonic wind anomalies as a Rossby wave response, and further cause anomalous meridional circulation and moisture transport over the WCI and BOB, favoring the rainfall increase there. The anomalous easterlies at the northern edge of two cyclones induced by the wet anomalies–related heating cause the divergence anomalies along the SFH, resulting in the reduction of precipitation in the HM. In turn, the two anomalous cyclones and dry anomalies have positive feedback on the wet and easterly wind anomalies, respectively, emphasizing the importance of the circulation–heating interaction.
Abstract
The present study investigates the interdecadal variation of precipitation over the Hengduan Mountains (HM) during rainy seasons from various reanalysis and observational datasets. Based on a moving t test and Lepage test, an obvious rainfall decrease is identified around 2004/05. The spatial distribution of the rainfall changes exhibits large and significant precipitation deficits over the southern HM, with notable anomalous lower-level easterly divergent winds along the southern foothills of the Himalayas (SFH). The anomalous easterlies are located at the northern edge of two cyclones, with two centers of positive rainfall anomalies over the west coast of India (WCI) and the Bay of Bengal (BOB). Observational evidence and numerical experiments demonstrate that the decadal changes of SST over the WP and WIO suppress rainfall over the eastern Indian Ocean (EIO) through large-scale circulation adjustment. The EIO dry anomalies trigger the cross-equatorial anticyclonic wind anomalies as a Rossby wave response, and further cause anomalous meridional circulation and moisture transport over the WCI and BOB, favoring the rainfall increase there. The anomalous easterlies at the northern edge of two cyclones induced by the wet anomalies–related heating cause the divergence anomalies along the SFH, resulting in the reduction of precipitation in the HM. In turn, the two anomalous cyclones and dry anomalies have positive feedback on the wet and easterly wind anomalies, respectively, emphasizing the importance of the circulation–heating interaction.
Advanced, robust, yet inexpensive observational platforms and networks of platforms will make revolutionary Earth science observations possible in the next 30 years. One new platform concept that is needed is a long-duration stratospheric balloon flying in a near-space environment and capable of remaining aloft for a year carrying a half ton of payload. We dub these platforms StratoSats for stratospheric satellites because they usually orbit the Earth in the stratosphere with an orbit period of 10–20 days. StratoSats can complement space satellites or play a completely independent role in Earth observation. Constellations of these platforms could steer themselves to desired locations and perform coordinated in situ and remote sensing observations of the Earth and its atmosphere. In principle, such constellations could easily surpass the capabilities of a single satellite for far less cost. NASA has defined stratospheric science measurement requirements and platform capabilities for several Earth science disciplines, including atmospheric chemistry, Earth radiation budget, geomagnetism, and weather. StratoSats can satisfy these measurement requirements and platform capabilities. Key enabling technologies for StratoSats include very long-life, sealed super-pressure balloons and techniques for balloon guidance. These key technologies are relatively mature, having achieved successful prototype and model tests in relevant environments, although a final push in engineering development is needed with a focus on meeting Earth science platform needs.
Advanced, robust, yet inexpensive observational platforms and networks of platforms will make revolutionary Earth science observations possible in the next 30 years. One new platform concept that is needed is a long-duration stratospheric balloon flying in a near-space environment and capable of remaining aloft for a year carrying a half ton of payload. We dub these platforms StratoSats for stratospheric satellites because they usually orbit the Earth in the stratosphere with an orbit period of 10–20 days. StratoSats can complement space satellites or play a completely independent role in Earth observation. Constellations of these platforms could steer themselves to desired locations and perform coordinated in situ and remote sensing observations of the Earth and its atmosphere. In principle, such constellations could easily surpass the capabilities of a single satellite for far less cost. NASA has defined stratospheric science measurement requirements and platform capabilities for several Earth science disciplines, including atmospheric chemistry, Earth radiation budget, geomagnetism, and weather. StratoSats can satisfy these measurement requirements and platform capabilities. Key enabling technologies for StratoSats include very long-life, sealed super-pressure balloons and techniques for balloon guidance. These key technologies are relatively mature, having achieved successful prototype and model tests in relevant environments, although a final push in engineering development is needed with a focus on meeting Earth science platform needs.
Abstract
A significant reduction in precipitation in the past decades has been documented over many mountain ranges such as those in central and eastern China. Consistent with the increase of air pollution in these regions, it has been argued that the precipitation trend is linked to the aerosol microphysical effect on suppressing warm rain. Rigorous quantitative investigations on the reasons responsible for the precipitation reduction are lacking. In this study, an improved Weather Research and Forecasting (WRF) Model with online coupled chemistry (WRF-Chem) is applied and simulations are conducted at the convection-permitting scale to explore the major mechanisms governing changes in precipitation from orographic clouds in the Mt. Hua area in central China. It is found that anthropogenic pollution contributes to a ~40% reduction of precipitation over Mt. Hua during the 1-month summertime period. The reduction is mainly associated with precipitation events associated with valley–mountain circulation and a mesoscale cold-front event. In this paper (Part I), the mechanism leading to a significant reduction for the cases associated with valley–mountain circulation is scrutinized. It is found that the valley breeze is weakened by aerosols as a result of absorbing aerosol-induced warming aloft and cooling near the surface as a result of aerosol–radiation interaction (ARI). The weakened valley breeze and the reduced water vapor in the valley due to reduced evapotranspiration as a result of surface cooling significantly reduce the transport of water vapor from the valley to mountain and the relative humidity over the mountain, thus suppressing convection and precipitation in the mountain.
Abstract
A significant reduction in precipitation in the past decades has been documented over many mountain ranges such as those in central and eastern China. Consistent with the increase of air pollution in these regions, it has been argued that the precipitation trend is linked to the aerosol microphysical effect on suppressing warm rain. Rigorous quantitative investigations on the reasons responsible for the precipitation reduction are lacking. In this study, an improved Weather Research and Forecasting (WRF) Model with online coupled chemistry (WRF-Chem) is applied and simulations are conducted at the convection-permitting scale to explore the major mechanisms governing changes in precipitation from orographic clouds in the Mt. Hua area in central China. It is found that anthropogenic pollution contributes to a ~40% reduction of precipitation over Mt. Hua during the 1-month summertime period. The reduction is mainly associated with precipitation events associated with valley–mountain circulation and a mesoscale cold-front event. In this paper (Part I), the mechanism leading to a significant reduction for the cases associated with valley–mountain circulation is scrutinized. It is found that the valley breeze is weakened by aerosols as a result of absorbing aerosol-induced warming aloft and cooling near the surface as a result of aerosol–radiation interaction (ARI). The weakened valley breeze and the reduced water vapor in the valley due to reduced evapotranspiration as a result of surface cooling significantly reduce the transport of water vapor from the valley to mountain and the relative humidity over the mountain, thus suppressing convection and precipitation in the mountain.
Abstract
Many efforts have been taken to investigate aerosol–cloud interactions from space, but only a few studies have examined the response of vertical cloud structure to aerosol perturbations. Three-dimensional cloud climatologies of eight different cloud types identified from the CloudSat level-2 cloud product during the warm season (May–September) in 2008–10 over eastern China were first generated and analyzed. Using visibility as a proxy for cloud condensation nuclei, in combination with satellite-observed radar reflectivity, normalized contoured frequency by altitude diagrams of the differences in cloud radar reflectivity Z profiles under polluted and clean conditions were constructed. For shallow cumulus clouds (shallow Cu) Z tends to be inhibited, and it is enhanced in the upper layers for deep cumulus (deep Cu), nimbostratus (Ns), and deep convective clouds (DCC) under polluted conditions. Overall, analyses of the modified center of gravity (MCOG) and cloud-top height (CTH) also point to a similar aerosol effect, except for the nonsignificant changes in MCOGs and CTHs in deep Cu. The impacts of environmental factors such as lower-tropospheric stability and vertical velocity are also discussed for these types of clouds. Although consistent aerosol-induced elevations in MCOGs and CTHs for Ns and DCC clouds are observed, the effect of meteorology cannot be completely ruled out, which merits further analysis.
Abstract
Many efforts have been taken to investigate aerosol–cloud interactions from space, but only a few studies have examined the response of vertical cloud structure to aerosol perturbations. Three-dimensional cloud climatologies of eight different cloud types identified from the CloudSat level-2 cloud product during the warm season (May–September) in 2008–10 over eastern China were first generated and analyzed. Using visibility as a proxy for cloud condensation nuclei, in combination with satellite-observed radar reflectivity, normalized contoured frequency by altitude diagrams of the differences in cloud radar reflectivity Z profiles under polluted and clean conditions were constructed. For shallow cumulus clouds (shallow Cu) Z tends to be inhibited, and it is enhanced in the upper layers for deep cumulus (deep Cu), nimbostratus (Ns), and deep convective clouds (DCC) under polluted conditions. Overall, analyses of the modified center of gravity (MCOG) and cloud-top height (CTH) also point to a similar aerosol effect, except for the nonsignificant changes in MCOGs and CTHs in deep Cu. The impacts of environmental factors such as lower-tropospheric stability and vertical velocity are also discussed for these types of clouds. Although consistent aerosol-induced elevations in MCOGs and CTHs for Ns and DCC clouds are observed, the effect of meteorology cannot be completely ruled out, which merits further analysis.