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L. L. Pan, E. L. Atlas, R. J. Salawitch, S. B. Honomichl, J. F. Bresch, W. J. Randel, E. C. Apel, R. S. Hornbrook, A. J. Weinheimer, D. C. Anderson, S. J. Andrews, S. Baidar, S. P. Beaton, T. L. Campos, L. J. Carpenter, D. Chen, B. Dix, V. Donets, S. R. Hall, T. F. Hanisco, C. R. Homeyer, L. G. Huey, J. B. Jensen, L. Kaser, D. E. Kinnison, T. K. Koenig, J.-F. Lamarque, C. Liu, J. Luo, Z. J. Luo, D. D. Montzka, J. M. Nicely, R. B. Pierce, D. D. Riemer, T. Robinson, P. Romashkin, A. Saiz-Lopez, S. Schauffler, O. Shieh, M. H. Stell, K. Ullmann, G. Vaughan, R. Volkamer, and G. Wolfe

Abstract

The Convective Transport of Active Species in the Tropics (CONTRAST) experiment was conducted from Guam (13.5°N, 144.8°E) during January–February 2014. Using the NSF/NCAR Gulfstream V research aircraft, the experiment investigated the photochemical environment over the tropical western Pacific (TWP) warm pool, a region of massive deep convection and the major pathway for air to enter the stratosphere during Northern Hemisphere (NH) winter. The new observations provide a wealth of information for quantifying the influence of convection on the vertical distributions of active species. The airborne in situ measurements up to 15-km altitude fill a significant gap by characterizing the abundance and altitude variation of a wide suite of trace gases. These measurements, together with observations of dynamical and microphysical parameters, provide significant new data for constraining and evaluating global chemistry–climate models. Measurements include precursor and product gas species of reactive halogen compounds that impact ozone in the upper troposphere/lower stratosphere. High-accuracy, in situ measurements of ozone obtained during CONTRAST quantify ozone concentration profiles in the upper troposphere, where previous observations from balloonborne ozonesondes were often near or below the limit of detection. CONTRAST was one of the three coordinated experiments to observe the TWP during January–February 2014. Together, CONTRAST, Airborne Tropical Tropopause Experiment (ATTREX), and Coordinated Airborne Studies in the Tropics (CAST), using complementary capabilities of the three aircraft platforms as well as ground-based instrumentation, provide a comprehensive quantification of the regional distribution and vertical structure of natural and pollutant trace gases in the TWP during NH winter, from the oceanic boundary to the lower stratosphere.

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Greg M. McFarquhar, Christopher S. Bretherton, Roger Marchand, Alain Protat, Paul J. DeMott, Simon P. Alexander, Greg C. Roberts, Cynthia H. Twohy, Darin Toohey, Steve Siems, Yi Huang, Robert Wood, Robert M. Rauber, Sonia Lasher-Trapp, Jorgen Jensen, Jeffrey L. Stith, Jay Mace, Junshik Um, Emma Järvinen, Martin Schnaiter, Andrew Gettelman, Kevin J. Sanchez, Christina S. McCluskey, Lynn M. Russell, Isabel L. McCoy, Rachel L. Atlas, Charles G. Bardeen, Kathryn A. Moore, Thomas C. J. Hill, Ruhi S. Humphries, Melita D. Keywood, Zoran Ristovski, Luke Cravigan, Robyn Schofield, Chris Fairall, Marc D. Mallet, Sonia M. Kreidenweis, Bryan Rainwater, John D’Alessandro, Yang Wang, Wei Wu, Georges Saliba, Ezra J. T. Levin, Saisai Ding, Francisco Lang, Son C. H. Truong, Cory Wolff, Julie Haggerty, Mike J. Harvey, Andrew R. Klekociuk, and Adrian McDonald

Abstract

Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation, and radiative processes, and their interactions. Projects between 2016 and 2018 used in situ probes, radar, lidar, and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN), and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF–NCAR G-V aircraft flying north–south gradients south of Tasmania, at Macquarie Island, and on the R/V Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multilayered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of dynamics and turbulence that likely drive heterogeneity of cloud phase. Satellite retrievals confirmed low clouds were responsible for radiation biases. The combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.

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