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  • Author or Editor: Chris A. Hostetler x
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Larry K. Berg
,
Carl M. Berkowitz
,
John A. Ogren
,
Chris A. Hostetler
,
Richard A. Ferrare
,
Manvendra K. Dubey
,
Elisabeth Andrews
,
Richard L. Coulter
,
Johnathan W. Hair
,
John M. Hubbe
,
Yin-Nan Lee
,
Claudio Mazzoleni
,
Jason Olfert
, and
Stephen R. Springston

The primary goal of the Cumulus Humilis Aerosol Processing Study (CHAPS) was to characterize and contrast freshly emitted aerosols below, within, and above fields of cumuli, and to study changes to the cloud microphysical structure within these same cloud fields in the vicinity of Oklahoma City during June 2007. CHAPS is one of few studies that have had an aerosol mass spectrometer (AMS) sampling downstream of a counterflow virtual impactor (CVI) inlet on an aircraft, allowing the examination of the chemical composition of activated aerosols within the cumuli. The results from CHAPS provide insights into changes in the aerosol chemical and optical properties as aerosols move through shallow cumuli downwind of a moderately sized city. Three instrument platforms were employed during CHAPS, including the U.S. Department of Energy Gulfstream-1 aircraft, which was equipped for in situ sampling of aerosol optical and chemical properties; the NASA Langley King Air B200, which carried the downward-looking NASA Langley High Spectral Resolution Lidar (HSRL) to measure profiles of aerosol backscatter, extinction, and depolarization between the King Air and the surface; and a surface site equipped for continuous in situ measurements of aerosol optical properties, profiles of aerosol backscatter, and meteorological conditions, including total sky cover and thermodynamic profiles of the atmosphere. In spite of record precipitation over central Oklahoma, a total of 8 research flights were made by the G-l and 18 by the B200, including special satellite verification flights timed to coincide with NASA satellite A-Train overpasses.

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David J. Diner
,
Robert T. Menzies
,
Ralph A. Kahn
,
Theodore L. Anderson
,
Jens Bösenberg
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Robert J. Charlson
,
Brent N. Holben
,
Chris A. Hostetler
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Mark A. Miller
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John A. Ogren
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Graeme L. Stephens
,
Omar Torres
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Bruce A. Wielicki
,
Philip J. Rasch
,
Larry D. Travis
, and
William D. Collins

A comprehensive and cohesive aerosol measurement record with consistent, well-understood uncertainties is a prerequisite to understanding aerosol impacts on long-term climate and environmental variability. Objectives to attaining such an understanding include improving upon the current state-of-the-art sensor calibration and developing systematic validation methods for remotely sensed microphysical properties. While advances in active and passive remote sensors will lead to needed improvements in retrieval accuracies and capabilities, ongoing validation is essential so that the changing sensor characteristics do not mask atmospheric trends. Surface-based radiometer, chemical, and lidar networks have critical roles within an integrated observing system, yet they currently undersample key geographic regions, have limitations in certain measurement capabilities, and lack stable funding. In situ aircraft observations of size-resolved aerosol chemical composition are necessary to provide important linkages between active and passive remote sensing. A planned, systematic approach toward a global aerosol observing network, involving multiple sponsoring agencies and surface-based, suborbital, and spaceborne sensors, is required to prioritize trade-offs regarding capabilities and costs. This strategy is a key ingredient of the Progressive Aerosol Retrieval and Assimilation Global Observing Network (PARAGON) framework. A set of recommendations is presented.

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David J. Diner
,
Thomas P. Ackerman
,
Theodore L. Anderson
,
Jens Bösenberg
,
Amy J. Braverman
,
Robert J. Charlson
,
William D. Collins
,
Roger Davies
,
Brent N. Holben
,
Chris A . Hostetler
,
Ralph A. Kahn
,
John V. Martonchik
,
Robert T. Menzies
,
Mark A. Miller
,
John A. Ogren
,
Joyce E. Penner
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Philip J. Rasch
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Stephen E. Schwartz
,
John H. Seinfeld
,
Graeme L. Stephens
,
Omar Torres
,
Larry D. Travis
,
Bruce A . Wielicki
, and
Bin Yu

Aerosols exert myriad influences on the earth's environment and climate, and on human health. The complexity of aerosol-related processes requires that information gathered to improve our understanding of climate change must originate from multiple sources, and that effective strategies for data integration need to be established. While a vast array of observed and modeled data are becoming available, the aerosol research community currently lacks the necessary tools and infrastructure to reap maximum scientific benefit from these data. Spatial and temporal sampling differences among a diverse set of sensors, nonuniform data qualities, aerosol mesoscale variabilities, and difficulties in separating cloud effects are some of the challenges that need to be addressed. Maximizing the longterm benefit from these data also requires maintaining consistently well-understood accuracies as measurement approaches evolve and improve. Achieving a comprehensive understanding of how aerosol physical, chemical, and radiative processes impact the earth system can be achieved only through a multidisciplinary, interagency, and international initiative capable of dealing with these issues. A systematic approach, capitalizing on modern measurement and modeling techniques, geospatial statistics methodologies, and high-performance information technologies, can provide the necessary machinery to support this objective. We outline a framework for integrating and interpreting observations and models, and establishing an accurate, consistent, and cohesive long-term record, following a strategy whereby information and tools of progressively greater sophistication are incorporated as problems of increasing complexity are tackled. This concept is named the Progressive Aerosol Retrieval and Assimilation Global Observing Network (PARAGON). To encompass the breadth of the effort required, we present a set of recommendations dealing with data interoperability; measurement and model integration; multisensor synergy; data summarization and mining; model evaluation; calibration and validation; augmentation of surface and in situ measurements; advances in passive and active remote sensing; and design of satellite missions. Without an initiative of this nature, the scientific and policy communities will continue to struggle with understanding the quantitative impact of complex aerosol processes on regional and global climate change and air quality.

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Armin Sorooshian
,
Bruce Anderson
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Susanne E. Bauer
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Rachel A. Braun
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Brian Cairns
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Ewan Crosbie
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Hossein Dadashazar
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Glenn Diskin
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Richard Ferrare
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Richard C. Flagan
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Johnathan Hair
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Chris Hostetler
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Haflidi H. Jonsson
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Mary M. Kleb
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Hongyu Liu
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Alexander B. MacDonald
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Allison McComiskey
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Richard Moore
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David Painemal
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Lynn M. Russell
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John H. Seinfeld
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Michael Shook
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William L. Smith Jr
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Kenneth Thornhill
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George Tselioudis
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Hailong Wang
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Xubin Zeng
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Bo Zhang
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Luke Ziemba
, and
Paquita Zuidema

Abstract

We report on a multiyear set of airborne field campaigns (2005–16) off the California coast to examine aerosols, clouds, and meteorology, and how lessons learned tie into the upcoming NASA Earth Venture Suborbital (EVS-3) campaign: Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE; 2019–23). The largest uncertainty in estimating global anthropogenic radiative forcing is associated with the interactions of aerosol particles with clouds, which stems from the variability of cloud systems and the multiple feedbacks that affect and hamper efforts to ascribe changes in cloud properties to aerosol perturbations. While past campaigns have been limited in flight hours and the ability to fly in and around clouds, efforts sponsored by the Office of Naval Research have resulted in 113 single aircraft flights (>500 flight hours) in a fixed region with warm marine boundary layer clouds. All flights used nearly the same payload of instruments on a Twin Otter to fly below, in, and above clouds, producing an unprecedented dataset. We provide here i) an overview of statistics of aerosol, cloud, and meteorological conditions encountered in those campaigns and ii) quantification of model-relevant metrics associated with aerosol–cloud interactions leveraging the high data volume and statistics. Based on lessons learned from those flights, we describe the pragmatic innovation in sampling strategy (dual-aircraft approach with combined in situ and remote sensing) that will be used in ACTIVATE to generate a dataset that can advance scientific understanding and improve physical parameterizations for Earth system and weather forecasting models, and for assessing next-generation remote sensing retrieval algorithms.

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