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Abstract
Updated analyses of in situ microphysical properties of three Arctic cloud systems sampled by aircraft in July 1998 during the Surface Heat Budget of the Arctic Ocean (SHEBA)/First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment–Arctic Clouds Experiment (FIRE–ACE) are examined in detail and compared with surface-based millimeter Doppler radar. A fourth case is given a cursory examination. The clouds were at 78°N over a melting ice surface, in distinctly different yet typical synoptic conditions. The cases comprise a midlevel all-ice cloud on 8 July; a deep, weakly forced, layered, mixed-phase stratus cloud system with pockets of drizzle, large dendrites, rimed ice and aggregates on 18 July; and a deep, mixed-phase cloud system with embedded convection on 28 July followed by an all-water boundary layer cloud on 29 July. The new observations include measured ice water content exceeding 2 g m−3 on 18 and 28 July and 3-cm snowflakes and 5-mm graupel particles on 28 July, unexpected in clouds close to the North Pole. Radar–aircraft agreement in reflectivity and derived microphysical parameters was reasonably good for the all-water and all-ice cases. In contrast, agreement in radar–aircraft reflectivity and derived parameters was generally inconsistent and sometimes poor for the two mixed-phase cases. The inconsistent agreement in radar–aircraft retrievals may be a result of large uncertainties in both instrument platforms and the algorithms used to retrieve derived parameters. The data also suggest that (single-wavelength) radar alone may not be capable of accurately retrieving the microphysical effects of cloud drops and drizzle in mixed-phase clouds, especially radiative properties such as extinction, albedo, and optical depth. However, more research is required before this generalization can be considered conclusive.
Abstract
Updated analyses of in situ microphysical properties of three Arctic cloud systems sampled by aircraft in July 1998 during the Surface Heat Budget of the Arctic Ocean (SHEBA)/First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment–Arctic Clouds Experiment (FIRE–ACE) are examined in detail and compared with surface-based millimeter Doppler radar. A fourth case is given a cursory examination. The clouds were at 78°N over a melting ice surface, in distinctly different yet typical synoptic conditions. The cases comprise a midlevel all-ice cloud on 8 July; a deep, weakly forced, layered, mixed-phase stratus cloud system with pockets of drizzle, large dendrites, rimed ice and aggregates on 18 July; and a deep, mixed-phase cloud system with embedded convection on 28 July followed by an all-water boundary layer cloud on 29 July. The new observations include measured ice water content exceeding 2 g m−3 on 18 and 28 July and 3-cm snowflakes and 5-mm graupel particles on 28 July, unexpected in clouds close to the North Pole. Radar–aircraft agreement in reflectivity and derived microphysical parameters was reasonably good for the all-water and all-ice cases. In contrast, agreement in radar–aircraft reflectivity and derived parameters was generally inconsistent and sometimes poor for the two mixed-phase cases. The inconsistent agreement in radar–aircraft retrievals may be a result of large uncertainties in both instrument platforms and the algorithms used to retrieve derived parameters. The data also suggest that (single-wavelength) radar alone may not be capable of accurately retrieving the microphysical effects of cloud drops and drizzle in mixed-phase clouds, especially radiative properties such as extinction, albedo, and optical depth. However, more research is required before this generalization can be considered conclusive.
Abstract
The spacing of cloud droplets observed along an approximately horizontal line through a cloud may be analyzed using a variety of techniques to reveal structure on small scales, sometimes called clustering, if such structure exists. A number of techniques have been applied and others have been suggested but not yet rigorously defined and applied. In this paper techniques are studied and evaluated using synthetic droplet spacing data. For the type of small-scale structure (clustering) modeled in this study, the most promising analysis approach is to use a combination of the power spectrum and the fishing statistic. Standard deviations and confidence intervals are determined for the power spectrum, the pair correlation function, and a modified fishing statistic. The clustering index and the volume-averaged pair correlation are shown to be less usefully normalized forms of the fishing statistic.
Abstract
The spacing of cloud droplets observed along an approximately horizontal line through a cloud may be analyzed using a variety of techniques to reveal structure on small scales, sometimes called clustering, if such structure exists. A number of techniques have been applied and others have been suggested but not yet rigorously defined and applied. In this paper techniques are studied and evaluated using synthetic droplet spacing data. For the type of small-scale structure (clustering) modeled in this study, the most promising analysis approach is to use a combination of the power spectrum and the fishing statistic. Standard deviations and confidence intervals are determined for the power spectrum, the pair correlation function, and a modified fishing statistic. The clustering index and the volume-averaged pair correlation are shown to be less usefully normalized forms of the fishing statistic.
Abstract
The microphysical properties of wave clouds based on data collected during 17 missions flown by a Learjet research aircraft are presented and discussed. This extensive dataset expands upon previous aircraft studies of wave clouds and introduces some new findings. While most aspects of the observations are consistent with basic cloud physics, some aspects remain difficult to interpret. Most notable among these are ice nucleation and aspects of the dynamical structure of wave clouds. A new hypothesis to explain the ice nucleation behavior is presented.
The average and standard deviation of bulk microphysical parameters are presented for various locations within the wave clouds. Using digital imagery from a cloud particle imager (CPI), the shapes of ice particles are studied and crystal habits are classified. For certain categories—rosette shapes, columns, and irregular shapes—power-law parameterizations of particle area from particle length are presented. Polycrystals with rosette shapes dominate the ice mass while small spheroidal and irregularly shaped crystals dominate the ice number concentration.
The concept and difficulties of using wave clouds as natural cloud physics laboratories are discussed and evaluated. A study of the riming threshold size of columns is in good agreement with the results of previous studies, showing that column width is the predominate factor in determining riming threshold. The first reported studies of the riming threshold size of rosette shapes and the threshold size for side-plane growth are presented.
Abstract
The microphysical properties of wave clouds based on data collected during 17 missions flown by a Learjet research aircraft are presented and discussed. This extensive dataset expands upon previous aircraft studies of wave clouds and introduces some new findings. While most aspects of the observations are consistent with basic cloud physics, some aspects remain difficult to interpret. Most notable among these are ice nucleation and aspects of the dynamical structure of wave clouds. A new hypothesis to explain the ice nucleation behavior is presented.
The average and standard deviation of bulk microphysical parameters are presented for various locations within the wave clouds. Using digital imagery from a cloud particle imager (CPI), the shapes of ice particles are studied and crystal habits are classified. For certain categories—rosette shapes, columns, and irregular shapes—power-law parameterizations of particle area from particle length are presented. Polycrystals with rosette shapes dominate the ice mass while small spheroidal and irregularly shaped crystals dominate the ice number concentration.
The concept and difficulties of using wave clouds as natural cloud physics laboratories are discussed and evaluated. A study of the riming threshold size of columns is in good agreement with the results of previous studies, showing that column width is the predominate factor in determining riming threshold. The first reported studies of the riming threshold size of rosette shapes and the threshold size for side-plane growth are presented.
Abstract
The rapid glaciation of tropical cumulus clouds has been an enigma and has been debated in the literature for over 60 years. Possible mechanisms responsible for the rapid freezing have been postulated, but until now direct evidence has been lacking. Recent high-speed photography of electrostatically suspended supercooled drops in the laboratory has shown that freezing events produce small secondary ice particles. Aircraft observations from the Ice in Clouds Experiment–Tropical (ICE-T), strongly suggest that the drop-freezing secondary ice production mechanism is operating in strong, tropical cumulus updraft cores. The result is the production of small ice particles colliding with large supercooled drops (hundreds of microns up to millimeters in diameter), producing a cascading process that results in rapid glaciation of water drops in the updraft. The process was analyzed from data collected using state-of-the-art cloud particle probes during 54 Learjet penetrations of strong cumulus updraft cores over open ocean in a temperature range from 5° to −20°C. Repeated Learjet penetrations of an updraft core containing 3–5 g m−3 supercooled liquid showed an order-of-magnitude decrease in liquid mass concentration 3 min later at an elevation 1–1.5 km higher in the cloud. The aircraft observations were simulated using a one-dimensional cloud model with explicit bin microphysics. The model was initialized with drop and ice particle size distributions observed prior to rapid glaciation. Simulations show that the model can explain the observed rapid glaciation by the drop-freezing secondary ice production process and subsequent riming, which results when large supercooled drops collide with ice particles.
Abstract
The rapid glaciation of tropical cumulus clouds has been an enigma and has been debated in the literature for over 60 years. Possible mechanisms responsible for the rapid freezing have been postulated, but until now direct evidence has been lacking. Recent high-speed photography of electrostatically suspended supercooled drops in the laboratory has shown that freezing events produce small secondary ice particles. Aircraft observations from the Ice in Clouds Experiment–Tropical (ICE-T), strongly suggest that the drop-freezing secondary ice production mechanism is operating in strong, tropical cumulus updraft cores. The result is the production of small ice particles colliding with large supercooled drops (hundreds of microns up to millimeters in diameter), producing a cascading process that results in rapid glaciation of water drops in the updraft. The process was analyzed from data collected using state-of-the-art cloud particle probes during 54 Learjet penetrations of strong cumulus updraft cores over open ocean in a temperature range from 5° to −20°C. Repeated Learjet penetrations of an updraft core containing 3–5 g m−3 supercooled liquid showed an order-of-magnitude decrease in liquid mass concentration 3 min later at an elevation 1–1.5 km higher in the cloud. The aircraft observations were simulated using a one-dimensional cloud model with explicit bin microphysics. The model was initialized with drop and ice particle size distributions observed prior to rapid glaciation. Simulations show that the model can explain the observed rapid glaciation by the drop-freezing secondary ice production process and subsequent riming, which results when large supercooled drops collide with ice particles.
Abstract
The Canadian Atlantic Storms Program (CASP II) field experiment was conducted near St. John’s, Newfoundland, Canada, during January–March 1992, and it focused on the nature of winter storms. Analyses of CASP II aircraft, surface, satellite, and radar observations collected during an intensive study of the origin and development of 9 mm h−1 precipitation containing 4–5-cm diameter snowflakes are compared in this article with results of the MM5 (mesoscale) and Mitchell (microphysical) models. MM5 simulations of the thermal, kinematic, and bulk microphysical fields were in good agreement with the observations; this comparison provided the basis for extending the spatial and temporal scales of the aircraft observations to a larger-scale domain using the model results. The Mitchell analytical–numerical model was used to improve the understanding of the microphysical processes that led to the development of the very large snowflakes. A synthesis of results using the different techniques leads to the conclusion that the snowflakes originated as 3–5-mm dendritic crystals in an area of weak convective instability at 5 km and were transported downwind in a strongly sheared airflow. The dendrites aggregated, fell into an existing snowzone (supported in some regions by vertical motion with velocities ranging from 0.2–0.6 m s−1), and continued to descend along a deep, downward sloping layer with temperatures near 0°C. Rapid aggregation occurred in the near 0°C region in particular and without appreciable particle breakup. An exponential fit to the particle size distribution in the region of very large snowflakes had a slope parameter on the order of 100 m−1.
Abstract
The Canadian Atlantic Storms Program (CASP II) field experiment was conducted near St. John’s, Newfoundland, Canada, during January–March 1992, and it focused on the nature of winter storms. Analyses of CASP II aircraft, surface, satellite, and radar observations collected during an intensive study of the origin and development of 9 mm h−1 precipitation containing 4–5-cm diameter snowflakes are compared in this article with results of the MM5 (mesoscale) and Mitchell (microphysical) models. MM5 simulations of the thermal, kinematic, and bulk microphysical fields were in good agreement with the observations; this comparison provided the basis for extending the spatial and temporal scales of the aircraft observations to a larger-scale domain using the model results. The Mitchell analytical–numerical model was used to improve the understanding of the microphysical processes that led to the development of the very large snowflakes. A synthesis of results using the different techniques leads to the conclusion that the snowflakes originated as 3–5-mm dendritic crystals in an area of weak convective instability at 5 km and were transported downwind in a strongly sheared airflow. The dendrites aggregated, fell into an existing snowzone (supported in some regions by vertical motion with velocities ranging from 0.2–0.6 m s−1), and continued to descend along a deep, downward sloping layer with temperatures near 0°C. Rapid aggregation occurred in the near 0°C region in particular and without appreciable particle breakup. An exponential fit to the particle size distribution in the region of very large snowflakes had a slope parameter on the order of 100 m−1.
Abstract
Since cirrus clouds have a substantial influence on the global energy balance that depends on their microphysical properties, climate models should strive to realistically characterize the cirrus ice particle size distribution (PSD), at least in a climatological sense. To date, the airborne in situ measurements of the cirrus PSD have contained large uncertainties due to errors in measuring small ice crystals (D ≲ 60 μm). This paper presents a method to remotely estimate the concentration of the small ice crystals relative to the larger ones using the 11- and 12-μm channels aboard several satellites. By understanding the underlying physics producing the emissivity difference between these channels, this emissivity difference can be used to infer the relative concentration of small ice crystals. This is facilitated by enlisting temperature-dependent characterizations of the PSD (i.e., PSD schemes) based on in situ measurements.
An average cirrus emissivity relationship between 12 and 11 μm is developed here using the Moderate Resolution Imaging Spectroradiometer (MODIS) satellite instrument and is used to “retrieve” the PSD based on six different PSD schemes. The PSDs from the measurement-based PSD schemes are compared with corresponding retrieved PSDs to evaluate differences in small ice crystal concentrations. The retrieved PSDs generally had lower concentrations of small ice particles, with total number concentration independent of temperature. In addition, the temperature dependence of the PSD effective diameter De and fall speed Vf for these retrieved PSD schemes exhibited less variability relative to the unmodified PSD schemes. The reduced variability in the retrieved De and Vf was attributed to the lower concentrations of small ice crystals in the retrieved PSD.
Abstract
Since cirrus clouds have a substantial influence on the global energy balance that depends on their microphysical properties, climate models should strive to realistically characterize the cirrus ice particle size distribution (PSD), at least in a climatological sense. To date, the airborne in situ measurements of the cirrus PSD have contained large uncertainties due to errors in measuring small ice crystals (D ≲ 60 μm). This paper presents a method to remotely estimate the concentration of the small ice crystals relative to the larger ones using the 11- and 12-μm channels aboard several satellites. By understanding the underlying physics producing the emissivity difference between these channels, this emissivity difference can be used to infer the relative concentration of small ice crystals. This is facilitated by enlisting temperature-dependent characterizations of the PSD (i.e., PSD schemes) based on in situ measurements.
An average cirrus emissivity relationship between 12 and 11 μm is developed here using the Moderate Resolution Imaging Spectroradiometer (MODIS) satellite instrument and is used to “retrieve” the PSD based on six different PSD schemes. The PSDs from the measurement-based PSD schemes are compared with corresponding retrieved PSDs to evaluate differences in small ice crystal concentrations. The retrieved PSDs generally had lower concentrations of small ice particles, with total number concentration independent of temperature. In addition, the temperature dependence of the PSD effective diameter De and fall speed Vf for these retrieved PSD schemes exhibited less variability relative to the unmodified PSD schemes. The reduced variability in the retrieved De and Vf was attributed to the lower concentrations of small ice crystals in the retrieved PSD.
Abstract
A Learjet research aircraft was used to collect microphysical data, including cloud particle imager (CPI) measurements of ice particle size and shape, in 22 midlatitude cirrus clouds. The dataset was collected while the aircraft flew 104 horizontal legs, totaling over 15 000 km in clouds. Cloud temperatures ranged from −28° to −61°C.
The measurements show that cirrus particle size distributions are mostly bimodal, displaying a maximum in number concentration, area, and mass near 30 μm and another smaller maximum near 200–300 μm. CPI images show that particles with rosette shapes, which include mixed-habit rosettes and platelike polycrystals, constitute over 50% of the surface area and mass of ice particles >50 μm in cirrus clouds. Approximately 40% of the remaining mass of ice particles >50 μm are found in irregular shapes, with a few percent each in columns and spheroidal shapes. Plates account for <1% of the total mass. Particles <50 μm account for 99% of the total number concentration, 69% of the shortwave extinction, and 40% of the mass in midlatitude cirrus. Plots and average equations for area versus particle size are shown for various particle habits, and can be used in studies involving radiative transfer.
The average particle concentration in midlatitude cirrus is on the order of 1 cm−3 with occasional 10-km averages exceeding 5 cm−3. There is a strong similarity of microphysical properties of ice particles between wave clouds and cirrus clouds, suggesting that, like wave clouds, cirrus ice particles first experience conversion to liquid water and/or solution drops before freezing.
Abstract
A Learjet research aircraft was used to collect microphysical data, including cloud particle imager (CPI) measurements of ice particle size and shape, in 22 midlatitude cirrus clouds. The dataset was collected while the aircraft flew 104 horizontal legs, totaling over 15 000 km in clouds. Cloud temperatures ranged from −28° to −61°C.
The measurements show that cirrus particle size distributions are mostly bimodal, displaying a maximum in number concentration, area, and mass near 30 μm and another smaller maximum near 200–300 μm. CPI images show that particles with rosette shapes, which include mixed-habit rosettes and platelike polycrystals, constitute over 50% of the surface area and mass of ice particles >50 μm in cirrus clouds. Approximately 40% of the remaining mass of ice particles >50 μm are found in irregular shapes, with a few percent each in columns and spheroidal shapes. Plates account for <1% of the total mass. Particles <50 μm account for 99% of the total number concentration, 69% of the shortwave extinction, and 40% of the mass in midlatitude cirrus. Plots and average equations for area versus particle size are shown for various particle habits, and can be used in studies involving radiative transfer.
The average particle concentration in midlatitude cirrus is on the order of 1 cm−3 with occasional 10-km averages exceeding 5 cm−3. There is a strong similarity of microphysical properties of ice particles between wave clouds and cirrus clouds, suggesting that, like wave clouds, cirrus ice particles first experience conversion to liquid water and/or solution drops before freezing.
Abstract
Understanding ice development in cumulus congestus (CuCg) clouds, which are ubiquitous globally, is critical for improving our knowledge of cloud physics, precipitation and climate prediction models. Results presented here are representative of data collected in 1008 penetrations of moderate to strong updrafts in CuCg clouds by five research aircraft in six geographic locations. The results show that CuCg with warm (∼23°C) cloud-base temperatures, such as in tropical marine environments, experience a strong collision–coalescence process. Development of coalescence is also correlated with drop effective radius >∼12 to 14 μm in diameter. Increasing the cloud-base drop concentration with diameters from 15 to 35 μm and decreasing the drop concentration < 15 μm appears to enhance coalescence. While the boundary layer aerosol population is not a determinate factor in development of coalescence in most tropical marine environments, its impact on coalescence is not yet fully determined. Some supercooled large drops generated via coalescence fracture when freezing, producing a secondary ice process (SIP) with production of copious small ice particles that naturally seed the cloud. The SIP produces an avalanche effect, freezing the majority of supercooled liquid water before fresh updrafts reach the −16°C level. Conversely, CuCg with cloud-base temperatures ≤ ∼8°C develop significant concentrations of ice particles at colder temperatures, so that small supercooled water drops are lofted to higher elevations before freezing. Recirculation of ice in downdrafts at the edges of updrafts appears to be the primary mechanism for development of precipitation in CuCg with colder cloud-base temperatures.
Significance Statement
Cumulus congestus clouds occur globally and account for a significant amount of precipitation in the tropics. The physics underlying the warm rain process and development of ice in cumulus congestus clouds are fundamental to a better understanding of precipitation formation. The collected data show that the strength of collision–coalescence is strongly influenced by cloud-base temperature, and that millimeter-diameter supercooled cloud drops will form in convective clouds with base temperatures warmer than 20°C. When supercooled large drops form, there is a secondary ice process that rapidly freezes the large majority of supercooled cloud water before updrafts reach the −16°C level. Incorporating results from the observations will improve cloud-resolving and climate prediction models.
Abstract
Understanding ice development in cumulus congestus (CuCg) clouds, which are ubiquitous globally, is critical for improving our knowledge of cloud physics, precipitation and climate prediction models. Results presented here are representative of data collected in 1008 penetrations of moderate to strong updrafts in CuCg clouds by five research aircraft in six geographic locations. The results show that CuCg with warm (∼23°C) cloud-base temperatures, such as in tropical marine environments, experience a strong collision–coalescence process. Development of coalescence is also correlated with drop effective radius >∼12 to 14 μm in diameter. Increasing the cloud-base drop concentration with diameters from 15 to 35 μm and decreasing the drop concentration < 15 μm appears to enhance coalescence. While the boundary layer aerosol population is not a determinate factor in development of coalescence in most tropical marine environments, its impact on coalescence is not yet fully determined. Some supercooled large drops generated via coalescence fracture when freezing, producing a secondary ice process (SIP) with production of copious small ice particles that naturally seed the cloud. The SIP produces an avalanche effect, freezing the majority of supercooled liquid water before fresh updrafts reach the −16°C level. Conversely, CuCg with cloud-base temperatures ≤ ∼8°C develop significant concentrations of ice particles at colder temperatures, so that small supercooled water drops are lofted to higher elevations before freezing. Recirculation of ice in downdrafts at the edges of updrafts appears to be the primary mechanism for development of precipitation in CuCg with colder cloud-base temperatures.
Significance Statement
Cumulus congestus clouds occur globally and account for a significant amount of precipitation in the tropics. The physics underlying the warm rain process and development of ice in cumulus congestus clouds are fundamental to a better understanding of precipitation formation. The collected data show that the strength of collision–coalescence is strongly influenced by cloud-base temperature, and that millimeter-diameter supercooled cloud drops will form in convective clouds with base temperatures warmer than 20°C. When supercooled large drops form, there is a secondary ice process that rapidly freezes the large majority of supercooled cloud water before updrafts reach the −16°C level. Incorporating results from the observations will improve cloud-resolving and climate prediction models.
Abstract
For nonconvective, steady light rain with rain rates <5 mm h−1 the mean Doppler velocity of raindrop spectra was found to be constant below the melting band, when the drop-free fall speed was adjusted for pressure. The Doppler radar–weighted raindrop diameters varied from case to case from 1.5 to 2.5 mm while rain rates changed from 1.2 to 2.9 mm h−1. Significant changes of advected velocity moments were observed over periods of 4 min.
These findings were corroborated by three independent systems: a Doppler radar for establishing vertical air speed and mean terminal drop speeds [using extended Velocity Azimuth Display (EVAD) analyses], a Joss–Waldvogel disdrometer at the ground, and a Particle Measuring System (PMS) 2-DP probe flown on an aircraft. These measurements were supported by data from upper-air soundings. The reason why inferred raindrop spectra do not change with height is the negligible interaction rate between raindrops at low rain rates. At low rain rates, numerical box models of drop collisions strongly support this interpretation. It was found that increasing characteristic drop diameters are correlated with increasing rain rates.
Abstract
For nonconvective, steady light rain with rain rates <5 mm h−1 the mean Doppler velocity of raindrop spectra was found to be constant below the melting band, when the drop-free fall speed was adjusted for pressure. The Doppler radar–weighted raindrop diameters varied from case to case from 1.5 to 2.5 mm while rain rates changed from 1.2 to 2.9 mm h−1. Significant changes of advected velocity moments were observed over periods of 4 min.
These findings were corroborated by three independent systems: a Doppler radar for establishing vertical air speed and mean terminal drop speeds [using extended Velocity Azimuth Display (EVAD) analyses], a Joss–Waldvogel disdrometer at the ground, and a Particle Measuring System (PMS) 2-DP probe flown on an aircraft. These measurements were supported by data from upper-air soundings. The reason why inferred raindrop spectra do not change with height is the negligible interaction rate between raindrops at low rain rates. At low rain rates, numerical box models of drop collisions strongly support this interpretation. It was found that increasing characteristic drop diameters are correlated with increasing rain rates.
On the Susceptibility of Cold Tropical Cirrus to Ice Nuclei AbundanceAbstract
Numerical simulations of cirrus formation in the tropical tropopause layer (TTL) during boreal wintertime are used to evaluate the impact of heterogeneous ice nuclei (IN) abundance on cold cloud microphysical properties and occurrence frequencies. The cirrus model includes homogeneous and heterogeneous ice nucleation, deposition growth/sublimation, and sedimentation. Reanalysis temperature and wind fields with high-frequency waves superimposed are used to force the simulations. The model results are constrained by comparison with in situ and satellite observations of TTL cirrus and relative humidity. Temperature variability driven by high-frequency waves has a dominant influence on TTL cirrus microphysical properties and occurrence frequencies, and inclusion of these waves is required to produce agreement between the simulated and observed abundance of TTL cirrus. With homogeneous freezing only and small-scale gravity waves included in the temperature curtains, the model produces excessive ice concentrations compared with in situ observations. Inclusion of relatively numerous heterogeneous ice nuclei (N IN ≥ 100 L−1) in the simulations improves the agreement with observed ice concentrations. However, when IN contribute significantly to TTL cirrus ice nucleation, the occurrence frequency of large supersaturations with respect to ice is less than indicated by in situ measurements. The model results suggest that the sensitivity of TTL cirrus extinction and ice water content statistics to heterogeneous ice nuclei abundance is relatively weak. The simulated occurrence frequencies of TTL cirrus are quite insensitive to ice nuclei abundance, both in terms of cloud frequency height distribution and regional distribution throughout the tropics.
Abstract
Numerical simulations of cirrus formation in the tropical tropopause layer (TTL) during boreal wintertime are used to evaluate the impact of heterogeneous ice nuclei (IN) abundance on cold cloud microphysical properties and occurrence frequencies. The cirrus model includes homogeneous and heterogeneous ice nucleation, deposition growth/sublimation, and sedimentation. Reanalysis temperature and wind fields with high-frequency waves superimposed are used to force the simulations. The model results are constrained by comparison with in situ and satellite observations of TTL cirrus and relative humidity. Temperature variability driven by high-frequency waves has a dominant influence on TTL cirrus microphysical properties and occurrence frequencies, and inclusion of these waves is required to produce agreement between the simulated and observed abundance of TTL cirrus. With homogeneous freezing only and small-scale gravity waves included in the temperature curtains, the model produces excessive ice concentrations compared with in situ observations. Inclusion of relatively numerous heterogeneous ice nuclei (N IN ≥ 100 L−1) in the simulations improves the agreement with observed ice concentrations. However, when IN contribute significantly to TTL cirrus ice nucleation, the occurrence frequency of large supersaturations with respect to ice is less than indicated by in situ measurements. The model results suggest that the sensitivity of TTL cirrus extinction and ice water content statistics to heterogeneous ice nuclei abundance is relatively weak. The simulated occurrence frequencies of TTL cirrus are quite insensitive to ice nuclei abundance, both in terms of cloud frequency height distribution and regional distribution throughout the tropics.
