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  • Author or Editor: Thaopaul V. Bui x
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David A. Peterson
,
Laura H. Thapa
,
Pablo E. Saide
,
Amber J. Soja
,
Emily M. Gargulinski
,
Edward J. Hyer
,
Bernadett Weinzierl
,
Maximilian Dollner
,
Manuel Schöberl
,
Philippe P. Papin
,
Shobha Kondragunta
,
Christopher P. Camacho
,
Charles Ichoku
,
Richard H. Moore
,
Johnathan W. Hair
,
James H. Crawford
,
Philip E. Dennison
,
Olga V. Kalashnikova
,
Christel E. Bennese
,
Thaopaul P. Bui
,
Joshua P. DiGangi
,
Glenn S. Diskin
,
Marta A. Fenn
,
Hannah S. Halliday
,
Jose Jimenez
,
John B. Nowak
,
Claire Robinson
,
Kevin Sanchez
,
Taylor J. Shingler
,
Lee Thornhill
,
Elizabeth B. Wiggins
,
Edward Winstead
, and
Chuanyu Xu

Abstract

The 2019 Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) field experiment obtained a diverse set of in situ and remotely sensed measurements before and during a pyrocumulonimbus (pyroCb) event over the Williams Flats fire in Washington State. This unique dataset confirms that pyroCb activity is an efficient vertical smoke transport pathway into the upper troposphere and lower stratosphere (UTLS). The magnitude of smoke plumes observed in the UTLS has increased significantly in recent years, following unprecedented wildfire and pyroCb activity observed worldwide. The FIREX-AQ pyroCb dataset is therefore extremely relevant to a broad community, providing the first measurements of fresh smoke exhaust in the upper troposphere, including from within active pyroCb cloud tops. High-resolution remote sensing reveals that three plume cores linked to localized fire fronts, burning primarily in dense forest fuels, contributed to four total pyroCb “pulses.” Rapid changes in fire geometry and spatial extent dramatically influenced the magnitude, behavior, and duration of pyroCb activity. Cloud probe measurements and weather radar identify the presence of large ice particles within the pyroCb and hydrometers below cloud base, indicating precipitation development. The resulting feedbacks suggest that vertical smoke transport efficiency was reduced slightly when compared with intense pyroCb events reaching the lower stratosphere. Physical and optical aerosol property measurements in pyroCb exhaust are compared with previous assumptions. A large suite of aerosol and gas-phase chemistry measurements sets a foundation for future studies aimed at understanding the composition of smoke plumes lifted by pyroconvection into the UTLS and their role in the climate system.

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Eric J. Jensen
,
Leonhard Pfister
,
David E. Jordan
,
Thaopaul V. Bui
,
Rei Ueyama
,
Hanwant B. Singh
,
Troy D. Thornberry
,
Andrew W. Rollins
,
Ru-Shan Gao
,
David W. Fahey
,
Karen H. Rosenlof
,
James W. Elkins
,
Glenn S. Diskin
,
Joshua P. DiGangi
,
R. Paul Lawson
,
Sarah Woods
,
Elliot L. Atlas
,
Maria A. Navarro Rodriguez
,
Steven C. Wofsy
,
Jasna Pittman
,
Charles G. Bardeen
,
Owen B. Toon
,
Bruce C. Kindel
,
Paul A. Newman
,
Matthew J. McGill
,
Dennis L. Hlavka
,
Leslie R. Lait
,
Mark R. Schoeberl
,
John W. Bergman
,
Henry B. Selkirk
,
M. Joan Alexander
,
Ji-Eun Kim
,
Boon H. Lim
,
Jochen Stutz
, and
Klaus Pfeilsticker

Abstract

The February–March 2014 deployment of the National Aeronautics and Space Administration (NASA) Airborne Tropical Tropopause Experiment (ATTREX) provided unique in situ measurements in the western Pacific tropical tropopause layer (TTL). Six flights were conducted from Guam with the long-range, high-altitude, unmanned Global Hawk aircraft. The ATTREX Global Hawk payload provided measurements of water vapor, meteorological conditions, cloud properties, tracer and chemical radical concentrations, and radiative fluxes. The campaign was partially coincident with the Convective Transport of Active Species in the Tropics (CONTRAST) and the Coordinated Airborne Studies in the Tropics (CAST) airborne campaigns based in Guam using lower-altitude aircraft (see companion articles in this issue). The ATTREX dataset is being used for investigations of TTL cloud, transport, dynamical, and chemical processes, as well as for evaluation and improvement of global-model representations of TTL processes. The ATTREX data are publicly available online (at https://espoarchive.nasa.gov/).

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