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  • Author or Editor: J. R. Minder x
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Ronald B. Smith, Justin R. Minder, Alison D. Nugent, Trude Storelvmo, Daniel J. Kirshbaum, Robert Warren, Neil Lareau, Philippe Palany, Arlington James, and Jeffrey French

The Dominica Experiment (DOMEX) took place in the eastern Caribbean from 4 April to 10 May 2011 with 21 research flights of the Wyoming King Air and several other observing systems. The goal was an improved understanding of the physics of convective orographic precipitation in the tropics. Two types of convection were found. During a period of weak trade winds, diurnal thermal convection was seen over Dominica. This convection caused little precipitation but carried aloft air with island-derived aerosol and depleted CO2. During periods of strong trades, mechanically forced convection over the windward slopes brought heavy rain to the high terrain. This convection was “seeded” by trade-wind cumuli or neutrally buoyant cool wet patches of air. In this mechanically forced convection, air parcels did not touch the island surface to gain buoyancy so no island-derived tracers were lofted. With fewer aerosols, the mean cloud droplet diameter increased from 15 to 25 μm. Plunging airflow and a wake were found in the lee of Dominica. The DOMEX dataset will advance our understanding and test our theories of cumulus triggering and aerosol influence on precipitation.

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Sara Lance, Jie Zhang, James J. Schwab, Paul Casson, Richard E. Brandt, David R. Fitzjarrald, Margaret J. Schwab, John Sicker, Cheng-Hsuan Lu, Sheng-Po Chen, Jeongran Yun, Jeffrey M. Freedman, Bhupal Shrestha, Qilong Min, Mark Beauharnois, Brian Crandall, Everette Joseph, Matthew J. Brewer, Justin R. Minder, Daniel Orlowski, Amy Christiansen, Annmarie G. Carlton, and Mary C. Barth

Abstract

Aqueous chemical processing within cloud and fog water is thought to be a key process in the production and transformation of secondary organic aerosol mass, found abundantly and ubiquitously throughout the troposphere. Yet, significant uncertainty remains regarding the organic chemical reactions taking place within clouds and the conditions under which those reactions occur, owing to the wide variety of organic compounds and their evolution under highly variable conditions when cycled through clouds. Continuous observations from a fixed remote site like Whiteface Mountain (WFM) in New York State and other mountaintop sites have been used to unravel complex multiphase interactions in the past, particularly the conversion of gas-phase emissions of SO2 to sulfuric acid within cloud droplets in the presence of sunlight. These scientific insights led to successful control strategies that reduced aerosol sulfate and cloud water acidity substantially over the following decades. This paper provides an overview of observations obtained during a pilot study that took place at WFM in August 2017 aimed at obtaining a better understanding of Chemical Processing of Organic Compounds within Clouds (CPOC). During the CPOC pilot study, aerosol cloud activation efficiency, particle size distribution, and chemical composition measurements were obtained below-cloud for comparison to routine observations at WFM, including cloud water composition and reactive trace gases. Additional instruments deployed for the CPOC pilot study included a Doppler lidar, sun photometer, and radiosondes to assist in evaluating the meteorological context for the below-cloud and summit observations.

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