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Liqi Chen, Wei Li, Jianqiong Zhan, Jianjun Wang, Yuanhui Zhang, and Xulin Yang

Abstract

To investigate the concentrations, sources, and temporal variations of atmospheric black carbon (BC) in the summer Arctic, routine ground-level observations of BC by optical absorption were made in the summer from 2005 to 2008 at the Chinese Arctic “Yellow River” Station (78°55′N, 11°56′E) at Ny-Ålesund on the island of Spitsbergen in the Svalbard Archipelago. Methods of the ensemble empirical-mode decomposition analysis and back-trajectory analysis were employed to assess temporal variation embedded in the BC datasets and airmass transport patterns. The 10th-percentile and median values of BC concentrations were 7.2 and 14.6 ng m−3, respectively, and hourly average BC concentrations ranged from 2.5 to 54.6 ng m−3. A gradual increase was found by 4 ng m−3 a−1. This increase was not seen in the Zeppelin Station and it seemed to contrast with the prevalent conception of generally decreasing BC concentration since 1989 in the Arctic. Factors responsible for this increase such as changes in emissions and atmospheric transport were taken into consideration. The result indicated that BC from local emissions was mostly responsible for the observed increase from 2005 to 2008. BC temporal variation in the summer was controlled by the atmospheric circulation, which presented a significant 6–14-day variation and coherent with 1–3- and 2–5-day and longer cycle variation. Although the atmospheric circulation changes from 2005 to 2008, there was not a marked trend in long-range transportation of BC. This study suggested that local emissions might have significant implication for the regional radiative energy balance at Ny-Ålesund.

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Jianqiong Zhan, Wenyuan Chang, Wei Li, Yanming Wang, Liqi Chen, and Jinpei Yan

Abstract

Fujian Province in southeastern coastal China is a relatively clean region with low emissions, as its high altitude isolates it from the rest of the country. However, the region experienced haze episodes on 3–14 December 2013. The authors performed simulations using the Weather Research and Forecasting Model coupled with chemistry (WRF-Chem) to examine the impacts of meteorological conditions, aerosol radiative feedbacks (ARFs; including aerosol direct and nearly first indirect effect), and internal and external emissions reduction scenarios on particulate matter smaller than 2.5 μm (PM2.5) concentrations. To the best of the authors’ knowledge, this is the first time the WRF-Chem model has been used to study air quality in this region. The model reasonably reproduced the meteorological conditions and PM2.5 concentrations. The analysis demonstrated that the highest-PM2.5 event was associated with a cold surge that promoted the impingement of northern pollutants on the region, and PM2.5 concentrations were sensitive to the emissions from the Yangtze River delta (16.6%) and the North China Plain (12.1%). This suggests that efforts toward coastal air quality improvement require regional cooperation to reduce emissions. Noticeably, ARFs were unlikely to increase PM2.5 concentrations in the coastal region, which was in contrast to the case in northern China. ARFs induced strong clean wind anomalies in the coastal region and also lowered the inland planetary boundary layer, which enhanced the blocking of northern pollutants crossing the high terrain in the north of Fujian Province. This indicates that ARFs tend to weaken the haze intensity in the southeastern coastal region.

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