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David R. Smith, William A. Krayer, Kathryn M. Ginger, Michael A. Rosenthal, Jo Ann P. Mulvany, Walter Sanford, Juanita J. Matkins, Loisteen E. Harrell, Bonnie Smith, G. Jayne Koester, Richard L. Lees, John D. Moore, and Frankie C. Vann

Project ATMOSPHERE Atmospheric Education Resource Agents (AERAs) from the mid-Atlantic states conducted their second annual regional workshop for teachers. The focus of this conference was hazardous weather. Over 150 educators from 10 states and the District of Columbia attended this one-day event held in Silver Spring, Maryland. The workshop included presentations by meteorologists and scientists from the National Oceanic and Atmospheric Administration, the Environmental Protection Agency, private corporations, and universities as well as by the AERAs themselves. The presentations were designed to develop basic understandings about hazardous weather and to provide guidance about how to deal with its effects. The orientation of the program was hands on, including a number of activities for teachers to implement in the classroom. This conference demonstrates how educators and scientists can form partnerships to improve science education.

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Christina S. McCluskey, Thomas C. J. Hill, Francesca Malfatti, Camille M. Sultana, Christopher Lee, Mitchell V. Santander, Charlotte M. Beall, Kathryn A. Moore, Gavin C. Cornwell, Douglas B. Collins, Kimberly A. Prather, Thilina Jayarathne, Elizabeth A. Stone, Farooq Azam, Sonia M. Kreidenweis, and Paul J. DeMott

Abstract

Emission rates and properties of ice nucleating particles (INPs) are required for proper representation of aerosol–cloud interactions in atmospheric models. Few investigations have quantified marine INP emissions, a potentially important INP source for remote oceanic regions. Previous studies have suggested INPs in sea spray aerosol (SSA) are linked to oceanic biological activity. This proposed link was explored in this study by measuring INP emissions from nascent SSA during phytoplankton blooms during two mesocosm experiments. In a Marine Aerosol Reference Tank (MART) experiment, a phytoplankton bloom was produced with chlorophyll-a (Chl a) concentrations reaching 39 μg L−1, while Chl a concentrations more representative of natural ocean conditions were obtained during the Investigation into Marine Particle Chemistry and Transfer Science (IMPACTS; peak Chl a of 5 μg L−1) campaign, conducted in the University of California, San Diego, wave flume. Dynamic trends in INP emissions occurred for INPs active at temperatures > −30°C. Increases in INPs active between −25° and −15°C lagged the peak in Chl a in both studies, suggesting a consistent population of INPs associated with the collapse of phytoplankton blooms. Trends in INP emissions were also compared to aerosol composition, abundances of microbes, and enzyme activity. In general, increases in INP concentrations corresponded to increases in organic species in SSA and the emissions of heterotrophic bacteria, suggesting that both microbes and biomolecules contribute to marine INP populations. INP trends were not directly correlated with a single biological marker in either study. Direct measurements of INP chemistry are needed to accurately identify particles types contributing to marine INP populations.

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Greg M. McFarquhar, Christopher S. Bretherton, Roger Marchand, Alain Protat, Paul J. DeMott, Simon P. Alexander, Greg C. Roberts, Cynthia H. Twohy, Darin Toohey, Steve Siems, Yi Huang, Robert Wood, Robert M. Rauber, Sonia Lasher-Trapp, Jorgen Jensen, Jeffrey L. Stith, Jay Mace, Junshik Um, Emma Järvinen, Martin Schnaiter, Andrew Gettelman, Kevin J. Sanchez, Christina S. McCluskey, Lynn M. Russell, Isabel L. McCoy, Rachel L. Atlas, Charles G. Bardeen, Kathryn A. Moore, Thomas C. J. Hill, Ruhi S. Humphries, Melita D. Keywood, Zoran Ristovski, Luke Cravigan, Robyn Schofield, Chris Fairall, Marc D. Mallet, Sonia M. Kreidenweis, Bryan Rainwater, John D’Alessandro, Yang Wang, Wei Wu, Georges Saliba, Ezra J. T. Levin, Saisai Ding, Francisco Lang, Son C. H. Truong, Cory Wolff, Julie Haggerty, Mike J. Harvey, Andrew R. Klekociuk, and Adrian McDonald

Abstract

Weather and climate models are challenged by uncertainties and biases in simulating Southern Ocean (SO) radiative fluxes that trace to a poor understanding of cloud, aerosol, precipitation, and radiative processes, and their interactions. Projects between 2016 and 2018 used in situ probes, radar, lidar, and other instruments to make comprehensive measurements of thermodynamics, surface radiation, cloud, precipitation, aerosol, cloud condensation nuclei (CCN), and ice nucleating particles over the SO cold waters, and in ubiquitous liquid and mixed-phase clouds common to this pristine environment. Data including soundings were collected from the NSF–NCAR G-V aircraft flying north–south gradients south of Tasmania, at Macquarie Island, and on the R/V Investigator and RSV Aurora Australis. Synergistically these data characterize boundary layer and free troposphere environmental properties, and represent the most comprehensive data of this type available south of the oceanic polar front, in the cold sector of SO cyclones, and across seasons. Results show largely pristine environments with numerous small and few large aerosols above cloud, suggesting new particle formation and limited long-range transport from continents, high variability in CCN and cloud droplet concentrations, and ubiquitous supercooled water in thin, multilayered clouds, often with small-scale generating cells near cloud top. These observations demonstrate how cloud properties depend on aerosols while highlighting the importance of dynamics and turbulence that likely drive heterogeneity of cloud phase. Satellite retrievals confirmed low clouds were responsible for radiation biases. The combination of models and observations is examining how aerosols and meteorology couple to control SO water and energy budgets.

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Chelsea R. Thompson, Steven C. Wofsy, Michael J. Prather, Paul A. Newman, Thomas F. Hanisco, Thomas B. Ryerson, David W. Fahey, Eric C. Apel, Charles A. Brock, William H. Brune, Karl Froyd, Joseph M. Katich, Julie M. Nicely, Jeff Peischl, Eric Ray, Patrick R. Veres, Siyuan Wang, Hannah M. Allen, Elizabeth Asher, Huisheng Bian, Donald Blake, Ilann Bourgeois, John Budney, T. Paul Bui, Amy Butler, Pedro Campuzano-Jost, Cecilia Chang, Mian Chin, RóISíN Commane, Gus Correa, John D. Crounse, Bruce Daube, Jack E. Dibb, Joshua P. Digangi, Glenn S. Diskin, Maximilian Dollner, James W. Elkins, Arlene M. Fiore, Clare M. Flynn, Hao Guo, Samuel R. Hall, Reem A. Hannun, Alan Hills, Eric J. Hintsa, Alma Hodzic, Rebecca S. Hornbrook, L. Greg Huey, Jose L. Jimenez, Ralph F. Keeling, Michelle J. Kim, Agnieszka Kupc, Forrest Lacey, Leslie R. Lait, Jean-Francois Lamarque, Junhua Liu, Kathryn Mckain, Simone Meinardi, David O. Miller, Stephen A. Montzka, Fred L. Moore, Eric J. Morgan, Daniel M. Murphy, Lee T. Murray, Benjamin A. Nault, J. Andrew Neuman, Louis Nguyen, Yenny Gonzalez, Andrew Rollins, Karen Rosenlof, Maryann Sargent, Gregory Schill, Joshua P. Schwarz, Jason M. St. Clair, Stephen D. Steenrod, Britton B. Stephens, Susan E. Strahan, Sarah A. Strode, Colm Sweeney, Alexander B. Thames, Kirk Ullmann, Nicholas Wagner, Rodney Weber, Bernadett Weinzierl, Paul O. Wennberg, Christina J. Williamson, Glenn M. Wolfe, and Linghan Zeng

Abstract

This article provides an overview of the NASA Atmospheric Tomography (ATom) mission and a summary of selected scientific findings to date. ATom was an airborne measurements and modeling campaign aimed at characterizing the composition and chemistry of the troposphere over the most remote regions of the Pacific, Southern, Atlantic, and Arctic Oceans, and examining the impact of anthropogenic and natural emissions on a global scale. These remote regions dominate global chemical reactivity and are exceptionally important for global air quality and climate. ATom data provide the in situ measurements needed to understand the range of chemical species and their reactions, and to test satellite remote sensing observations and global models over large regions of the remote atmosphere. Lack of data in these regions, particularly over the oceans, has limited our understanding of how atmospheric composition is changing in response to shifting anthropogenic emissions and physical climate change. ATom was designed as a global-scale tomographic sampling mission with extensive geographic and seasonal coverage, tropospheric vertical profiling, and detailed speciation of reactive compounds and pollution tracers. ATom flew the NASA DC-8 research aircraft over four seasons to collect a comprehensive suite of measurements of gases, aerosols, and radical species from the remote troposphere and lower stratosphere on four global circuits from 2016 to 2018. Flights maintained near-continuous vertical profiling of 0.15 – 13 km altitudes on long meridional transects of the Pacific and Atlantic Ocean basins. Analysis and modeling of ATom data have led to the significant early findings highlighted here.

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