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- Author or Editor: Olivier Jourdan x
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Abstract
Observations of halos and related phenomena due to ice crystals are commonly reported from ground observations and presented in the literature. Nevertheless, ice crystal characteristics have only been poorly documented from in situ measurements performed in halo-producing cirrus with simultaneous observations of optical phenomena. Using the Polar Nephelometer, a new instrument for in situ measuring of the scattering phase function of cloud droplets and ice particles, 22° and 46° halo features have been evidenced during a cirrus uncinus cloud case study between −30°C and −38°C. Simultaneous microphysical measurements were made with a 2D-C probe manufactured by Particle Measuring Systems Inc. (PMS). The results show that ice crystal properties derived from 2D-C measurements do not present substantial differences when comparing cirrus cloud samples with and without halos. Consequently, the cloud scattering properties appear to be dominated by small ice particles (smaller than about 100 μm), which are poorly documented with conventional PMS probes. The halo occurrences are observed in only a few cloud portions (2%), which are characterized by small horizontal scales (100–400 m). Furthermore, the observed 22° and 46° peak features are smoothed out with regard to modeling results relative to geometric pristine-crystal shape. These differences are discussed by using the new Inhomogeneous Hexagonal Monocrystal theoretical model of light scattering.
Abstract
Observations of halos and related phenomena due to ice crystals are commonly reported from ground observations and presented in the literature. Nevertheless, ice crystal characteristics have only been poorly documented from in situ measurements performed in halo-producing cirrus with simultaneous observations of optical phenomena. Using the Polar Nephelometer, a new instrument for in situ measuring of the scattering phase function of cloud droplets and ice particles, 22° and 46° halo features have been evidenced during a cirrus uncinus cloud case study between −30°C and −38°C. Simultaneous microphysical measurements were made with a 2D-C probe manufactured by Particle Measuring Systems Inc. (PMS). The results show that ice crystal properties derived from 2D-C measurements do not present substantial differences when comparing cirrus cloud samples with and without halos. Consequently, the cloud scattering properties appear to be dominated by small ice particles (smaller than about 100 μm), which are poorly documented with conventional PMS probes. The halo occurrences are observed in only a few cloud portions (2%), which are characterized by small horizontal scales (100–400 m). Furthermore, the observed 22° and 46° peak features are smoothed out with regard to modeling results relative to geometric pristine-crystal shape. These differences are discussed by using the new Inhomogeneous Hexagonal Monocrystal theoretical model of light scattering.
Abstract
A methodology of employing statistical procedures, specifically the principal component analysis (PCA) technique, to assess cirrus cloud data reliability is described. The approach is demonstrated by an example of a study of optical and microphysical characteristics measured during two campaigns performed at midlatitudes in the pristine Southern (SH) and polluted Northern (NH) Hemispheres within the international INCA project (Interhemispheric Differences in Cirrus Cloud Properties from Anthropogenic Emissions). The datasets were obtained by using state-of-the-art airborne instruments including the polar nephelometer and PMS particle size spectrometers for the ice-particle characterization. The approach is applied to both the measured angular scattering intensities and the ice-particle size distributions. It is shown that the PCA technique allows for impartial elimination of nonreliable channels of instruments. Furthermore, this technique is efficient in a study if the dataset is statistically homogeneous, and provides the possibility of removing specific records corresponding to distinguishing statistical ensembles. The results, expressed in terms of significant components and corresponding eigenvalues, show that the Southern and Northern Hemisphere datasets are in good agreement and they can be considered as statistically representative of the sampled cirrus. Furthermore, the frequency distributions of the cirrus cloud microphysical and optical properties can be regarded as arbitrary positive quantities, which are lognormally distributed. The validation of the measurements is provided by intercomparison of parameters estimated from different and independent techniques. The statistical relationships between quantities derived from angular scattering intensities and from ice-particle distributions as well as the similarity of the results obtained for the Southern and Northern Hemisphere cases serve as proof of the reliability of the measured cloud properties.
Abstract
A methodology of employing statistical procedures, specifically the principal component analysis (PCA) technique, to assess cirrus cloud data reliability is described. The approach is demonstrated by an example of a study of optical and microphysical characteristics measured during two campaigns performed at midlatitudes in the pristine Southern (SH) and polluted Northern (NH) Hemispheres within the international INCA project (Interhemispheric Differences in Cirrus Cloud Properties from Anthropogenic Emissions). The datasets were obtained by using state-of-the-art airborne instruments including the polar nephelometer and PMS particle size spectrometers for the ice-particle characterization. The approach is applied to both the measured angular scattering intensities and the ice-particle size distributions. It is shown that the PCA technique allows for impartial elimination of nonreliable channels of instruments. Furthermore, this technique is efficient in a study if the dataset is statistically homogeneous, and provides the possibility of removing specific records corresponding to distinguishing statistical ensembles. The results, expressed in terms of significant components and corresponding eigenvalues, show that the Southern and Northern Hemisphere datasets are in good agreement and they can be considered as statistically representative of the sampled cirrus. Furthermore, the frequency distributions of the cirrus cloud microphysical and optical properties can be regarded as arbitrary positive quantities, which are lognormally distributed. The validation of the measurements is provided by intercomparison of parameters estimated from different and independent techniques. The statistical relationships between quantities derived from angular scattering intensities and from ice-particle distributions as well as the similarity of the results obtained for the Southern and Northern Hemisphere cases serve as proof of the reliability of the measured cloud properties.
Abstract
This study illustrates the high potential of RALI, the French airborne radar–lidar instrument, for studying cloud processes and evaluating satellite products when satellite overpasses are available. For an Arctic nimbostratus ice cloud collected on 1 April 2008 during the Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols, and Transport (POLARCAT) campaign, the capability of this synergistic instrument to retrieve cloud properties and to characterize the cloud phase at scales smaller than a kilometer, which is crucial for cloud process analysis, is demonstrated. A variational approach, which combines radar and lidar, is used to retrieve the ice-water content (IWC), extinction, and effective radius. The combination of radar and lidar is shown to provide better retrievals than do stand-alone methods and, in general, the radar overestimates and the lidar underestimates IWC. As the sampled ice cloud was simultaneously observed by CloudSat and Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellites, a new way to assess satellite cloud products by combining in situ and active remote sensing measurements is identified. It was then possible to compare RALI to three satellite ice cloud products: CloudSat, CALIPSO, and the Cloud-Aerosol-Water-Radiation Interactions (ICARE) center’s radar–lidar project (DARDAR).
Abstract
This study illustrates the high potential of RALI, the French airborne radar–lidar instrument, for studying cloud processes and evaluating satellite products when satellite overpasses are available. For an Arctic nimbostratus ice cloud collected on 1 April 2008 during the Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols, and Transport (POLARCAT) campaign, the capability of this synergistic instrument to retrieve cloud properties and to characterize the cloud phase at scales smaller than a kilometer, which is crucial for cloud process analysis, is demonstrated. A variational approach, which combines radar and lidar, is used to retrieve the ice-water content (IWC), extinction, and effective radius. The combination of radar and lidar is shown to provide better retrievals than do stand-alone methods and, in general, the radar overestimates and the lidar underestimates IWC. As the sampled ice cloud was simultaneously observed by CloudSat and Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellites, a new way to assess satellite cloud products by combining in situ and active remote sensing measurements is identified. It was then possible to compare RALI to three satellite ice cloud products: CloudSat, CALIPSO, and the Cloud-Aerosol-Water-Radiation Interactions (ICARE) center’s radar–lidar project (DARDAR).
Abstract
Homogeneous freezing of supercooled droplets occurs in convective systems in low and midlatitudes. This droplet-freezing process leads to the formation of a large amount of small ice particles, so-called frozen droplets, that are transported to the upper parts of anvil outflows, where they can influence the cloud radiative properties. However, the detailed microphysics and, thus, the scattering properties of these small ice particles are highly uncertain. Here, the link between the microphysical and optical properties of frozen droplets is investigated in cloud chamber experiments, where the frozen droplets were formed, grown, and sublimated under controlled conditions. It was found that frozen droplets developed a high degree of small-scale complexity after their initial formation and subsequent growth. During sublimation, the small-scale complexity disappeared, releasing a smooth and near-spherical ice particle. Angular light scattering and depolarization measurements confirmed that these sublimating frozen droplets scattered light similar to spherical particles: that is, they had angular light-scattering properties similar to water droplets. The knowledge gained from this laboratory study was applied to two case studies of aircraft measurements in midlatitude and tropical convective systems. The in situ aircraft measurements confirmed that the microphysics of frozen droplets is dependent on the humidity conditions they are exposed to (growth or sublimation). The existence of optically spherical frozen droplets can be important for the radiative properties of detraining convective outflows.
Abstract
Homogeneous freezing of supercooled droplets occurs in convective systems in low and midlatitudes. This droplet-freezing process leads to the formation of a large amount of small ice particles, so-called frozen droplets, that are transported to the upper parts of anvil outflows, where they can influence the cloud radiative properties. However, the detailed microphysics and, thus, the scattering properties of these small ice particles are highly uncertain. Here, the link between the microphysical and optical properties of frozen droplets is investigated in cloud chamber experiments, where the frozen droplets were formed, grown, and sublimated under controlled conditions. It was found that frozen droplets developed a high degree of small-scale complexity after their initial formation and subsequent growth. During sublimation, the small-scale complexity disappeared, releasing a smooth and near-spherical ice particle. Angular light scattering and depolarization measurements confirmed that these sublimating frozen droplets scattered light similar to spherical particles: that is, they had angular light-scattering properties similar to water droplets. The knowledge gained from this laboratory study was applied to two case studies of aircraft measurements in midlatitude and tropical convective systems. The in situ aircraft measurements confirmed that the microphysics of frozen droplets is dependent on the humidity conditions they are exposed to (growth or sublimation). The existence of optically spherical frozen droplets can be important for the radiative properties of detraining convective outflows.
Abstract
The goal of the Sea2Cloud project is to study the interplay between surface ocean biogeochemical and physical properties, fluxes to the atmosphere, and ultimately their impact on cloud formation under minimal direct anthropogenic influence. Here we present an interdisciplinary approach, combining atmospheric physics and chemistry with marine biogeochemistry, during a voyage between 41° and 47°S in March 2020. In parallel to ambient measurements of atmospheric composition and seawater biogeochemical properties, we describe semicontrolled experiments to characterize nascent sea spray properties and nucleation from gas-phase biogenic emissions. The experimental framework for studying the impact of the predicted evolution of ozone concentration in the Southern Hemisphere is also detailed. After describing the experimental strategy, we present the oceanic and meteorological context including provisional results on atmospheric thermodynamics, composition, and flux measurements. In situ measurements and flux studies were carried out on different biological communities by sampling surface seawater from subantarctic, subtropical, and frontal water masses. Air–Sea-Interface Tanks (ASIT) were used to quantify biogenic emissions of trace gases under realistic environmental conditions, with nucleation observed in association with biogenic seawater emissions. Sea spray continuously generated produced sea spray fluxes of 34% of organic matter by mass, of which 4% particles had fluorescent properties, and which size distribution resembled the one found in clean sectors of the Southern Ocean. The goal of Sea2Cloud is to generate realistic parameterizations of emission flux dependences of trace gases and nucleation precursors, sea spray, cloud condensation nuclei, and ice nuclei using seawater biogeochemistry, for implementation in regional atmospheric models.
Abstract
The goal of the Sea2Cloud project is to study the interplay between surface ocean biogeochemical and physical properties, fluxes to the atmosphere, and ultimately their impact on cloud formation under minimal direct anthropogenic influence. Here we present an interdisciplinary approach, combining atmospheric physics and chemistry with marine biogeochemistry, during a voyage between 41° and 47°S in March 2020. In parallel to ambient measurements of atmospheric composition and seawater biogeochemical properties, we describe semicontrolled experiments to characterize nascent sea spray properties and nucleation from gas-phase biogenic emissions. The experimental framework for studying the impact of the predicted evolution of ozone concentration in the Southern Hemisphere is also detailed. After describing the experimental strategy, we present the oceanic and meteorological context including provisional results on atmospheric thermodynamics, composition, and flux measurements. In situ measurements and flux studies were carried out on different biological communities by sampling surface seawater from subantarctic, subtropical, and frontal water masses. Air–Sea-Interface Tanks (ASIT) were used to quantify biogenic emissions of trace gases under realistic environmental conditions, with nucleation observed in association with biogenic seawater emissions. Sea spray continuously generated produced sea spray fluxes of 34% of organic matter by mass, of which 4% particles had fluorescent properties, and which size distribution resembled the one found in clean sectors of the Southern Ocean. The goal of Sea2Cloud is to generate realistic parameterizations of emission flux dependences of trace gases and nucleation precursors, sea spray, cloud condensation nuclei, and ice nuclei using seawater biogeochemistry, for implementation in regional atmospheric models.
Abstract
The THINICE field campaign, based from Svalbard in August 2022, provided unique observations of summertime Arctic cyclones, their coupling with cloud cover, and interactions with tropopause polar vortices and sea ice conditions. THINICE was motivated by the need to advance our understanding of these processes and to improve coupled models used to forecast weather and sea ice, as well as long-term projections of climate change in the Arctic. Two research aircraft were deployed with complementary instrumentation. The Safire ATR42 aircraft, equipped with the RALI (RAdar-LIdar) remote sensing instrumentation and in-situ cloud microphysics probes, flew in the mid-troposphere to observe the wind and multi-phase cloud structure of Arctic cyclones. The British Antarctic Survey MASIN aircraft flew at low levels measuring sea-ice properties, including surface brightness temperature, albedo and roughness, and the turbulent fluxes that mediate exchange of heat and momentum between the atmosphere and the surface. Long duration instrumented balloons, operated by WindBorne Systems, sampled meteorological conditions within both cyclones and tropospheric polar vortices across the Arctic. Several novel findings are highlighted. Intense, shallow low-level jets along warm fronts were observed within three Arctic cyclones using the Doppler radar and turbulence probes. A detailed depiction of the interweaving layers of ice crystals and supercooled liquid water in mixed-phase clouds is revealed through the synergistic combination of the Doppler radar, the lidar and in-situ microphysical probes. Measurements of near-surface turbulent fluxes combined with remote sensing measurements of sea ice properties are being used to characterize atmosphere-sea ice interactions in the marginal ice zone.
Abstract
The THINICE field campaign, based from Svalbard in August 2022, provided unique observations of summertime Arctic cyclones, their coupling with cloud cover, and interactions with tropopause polar vortices and sea ice conditions. THINICE was motivated by the need to advance our understanding of these processes and to improve coupled models used to forecast weather and sea ice, as well as long-term projections of climate change in the Arctic. Two research aircraft were deployed with complementary instrumentation. The Safire ATR42 aircraft, equipped with the RALI (RAdar-LIdar) remote sensing instrumentation and in-situ cloud microphysics probes, flew in the mid-troposphere to observe the wind and multi-phase cloud structure of Arctic cyclones. The British Antarctic Survey MASIN aircraft flew at low levels measuring sea-ice properties, including surface brightness temperature, albedo and roughness, and the turbulent fluxes that mediate exchange of heat and momentum between the atmosphere and the surface. Long duration instrumented balloons, operated by WindBorne Systems, sampled meteorological conditions within both cyclones and tropospheric polar vortices across the Arctic. Several novel findings are highlighted. Intense, shallow low-level jets along warm fronts were observed within three Arctic cyclones using the Doppler radar and turbulence probes. A detailed depiction of the interweaving layers of ice crystals and supercooled liquid water in mixed-phase clouds is revealed through the synergistic combination of the Doppler radar, the lidar and in-situ microphysical probes. Measurements of near-surface turbulent fluxes combined with remote sensing measurements of sea ice properties are being used to characterize atmosphere-sea ice interactions in the marginal ice zone.
Abstract
Clouds play an important role in Arctic amplification. This term represents the recently observed enhanced warming of the Arctic relative to the global increase of near-surface air temperature. However, there are still important knowledge gaps regarding the interplay between Arctic clouds and aerosol particles, and surface properties, as well as turbulent and radiative fluxes that inhibit accurate model simulations of clouds in the Arctic climate system. In an attempt to resolve this so-called Arctic cloud puzzle, two comprehensive and closely coordinated field studies were conducted: the Arctic Cloud Observations Using Airborne Measurements during Polar Day (ACLOUD) aircraft campaign and the Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and Aerosol (PASCAL) ice breaker expedition. Both observational studies were performed in the framework of the German Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC) 3 project. They took place in the vicinity of Svalbard, Norway, in May and June 2017. ACLOUD and PASCAL explored four pieces of the Arctic cloud puzzle: cloud properties, aerosol impact on clouds, atmospheric radiation, and turbulent dynamical processes. The two instrumented Polar 5 and Polar 6 aircraft; the icebreaker Research Vessel (R/V) Polarstern; an ice floe camp including an instrumented tethered balloon; and the permanent ground-based measurement station at Ny-Ă…lesund, Svalbard, were employed to observe Arctic low- and mid-level mixed-phase clouds and to investigate related atmospheric and surface processes. The Polar 5 aircraft served as a remote sensing observatory examining the clouds from above by downward-looking sensors; the Polar 6 aircraft operated as a flying in situ measurement laboratory sampling inside and below the clouds. Most of the collocated Polar 5/6 flights were conducted either above the R/V Polarstern or over the Ny-Ă…lesund station, both of which monitored the clouds from below using similar but upward-looking remote sensing techniques as the Polar 5 aircraft. Several of the flights were carried out underneath collocated satellite tracks. The paper motivates the scientific objectives of the ACLOUD/PASCAL observations and describes the measured quantities, retrieved parameters, and the applied complementary instrumentation. Furthermore, it discusses selected measurement results and poses critical research questions to be answered in future papers analyzing the data from the two field campaigns.
Abstract
Clouds play an important role in Arctic amplification. This term represents the recently observed enhanced warming of the Arctic relative to the global increase of near-surface air temperature. However, there are still important knowledge gaps regarding the interplay between Arctic clouds and aerosol particles, and surface properties, as well as turbulent and radiative fluxes that inhibit accurate model simulations of clouds in the Arctic climate system. In an attempt to resolve this so-called Arctic cloud puzzle, two comprehensive and closely coordinated field studies were conducted: the Arctic Cloud Observations Using Airborne Measurements during Polar Day (ACLOUD) aircraft campaign and the Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and Aerosol (PASCAL) ice breaker expedition. Both observational studies were performed in the framework of the German Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC) 3 project. They took place in the vicinity of Svalbard, Norway, in May and June 2017. ACLOUD and PASCAL explored four pieces of the Arctic cloud puzzle: cloud properties, aerosol impact on clouds, atmospheric radiation, and turbulent dynamical processes. The two instrumented Polar 5 and Polar 6 aircraft; the icebreaker Research Vessel (R/V) Polarstern; an ice floe camp including an instrumented tethered balloon; and the permanent ground-based measurement station at Ny-Ă…lesund, Svalbard, were employed to observe Arctic low- and mid-level mixed-phase clouds and to investigate related atmospheric and surface processes. The Polar 5 aircraft served as a remote sensing observatory examining the clouds from above by downward-looking sensors; the Polar 6 aircraft operated as a flying in situ measurement laboratory sampling inside and below the clouds. Most of the collocated Polar 5/6 flights were conducted either above the R/V Polarstern or over the Ny-Ă…lesund station, both of which monitored the clouds from below using similar but upward-looking remote sensing techniques as the Polar 5 aircraft. Several of the flights were carried out underneath collocated satellite tracks. The paper motivates the scientific objectives of the ACLOUD/PASCAL observations and describes the measured quantities, retrieved parameters, and the applied complementary instrumentation. Furthermore, it discusses selected measurement results and poses critical research questions to be answered in future papers analyzing the data from the two field campaigns.
