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V. Eyring, N. R. P. Harris, M. Rex, T. G. Shepherd, D. W. Fahey, G. T. Amanatidis, J. Austin, M. P. Chipperfield, M. Dameris, P. M. De F. Forster, A. Gettelman, H. F. Graf, T. Nagashima, P. A. Newman, S. Pawson, M. J. Prather, J. A. Pyle, R. J. Salawitch, B. D. Santer, and D. W. Waugh

Accurate and reliable predictions and an understanding of future changes in the stratosphere are major aspects of the subject of climate change. Simulating the interaction between chemistry and climate is of particular importance, because continued increases in greenhouse gases and a slow decrease in halogen loading are expected. These both influence the abundance of stratospheric ozone. In recent years a number of coupled chemistry–climate models (CCMs) with different levels of complexity have been developed. They produce a wide range of results concerning the timing and extent of ozone-layer recovery. Interest in reducing this range has created a need to address how the main dynamical, chemical, and physical processes that determine the long-term behavior of ozone are represented in the models and to validate these model processes through comparisons with observations and other models. A set of core validation processes structured around four major topics (transport, dynamics, radiation, and stratospheric chemistry and microphysics) has been developed. Each process is associated with one or more model diagnostics and with relevant datasets that can be used for validation. This approach provides a coherent framework for validating CCMs and can be used as a basis for future assessments. Similar efforts may benefit other modeling communities with a focus on earth science research as their models increase in complexity.

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L. L. Pan, E. L. Atlas, R. J. Salawitch, S. B. Honomichl, J. F. Bresch, W. J. Randel, E. C. Apel, R. S. Hornbrook, A. J. Weinheimer, D. C. Anderson, S. J. Andrews, S. Baidar, S. P. Beaton, T. L. Campos, L. J. Carpenter, D. Chen, B. Dix, V. Donets, S. R. Hall, T. F. Hanisco, C. R. Homeyer, L. G. Huey, J. B. Jensen, L. Kaser, D. E. Kinnison, T. K. Koenig, J.-F. Lamarque, C. Liu, J. Luo, Z. J. Luo, D. D. Montzka, J. M. Nicely, R. B. Pierce, D. D. Riemer, T. Robinson, P. Romashkin, A. Saiz-Lopez, S. Schauffler, O. Shieh, M. H. Stell, K. Ullmann, G. Vaughan, R. Volkamer, and G. Wolfe

Abstract

The Convective Transport of Active Species in the Tropics (CONTRAST) experiment was conducted from Guam (13.5°N, 144.8°E) during January–February 2014. Using the NSF/NCAR Gulfstream V research aircraft, the experiment investigated the photochemical environment over the tropical western Pacific (TWP) warm pool, a region of massive deep convection and the major pathway for air to enter the stratosphere during Northern Hemisphere (NH) winter. The new observations provide a wealth of information for quantifying the influence of convection on the vertical distributions of active species. The airborne in situ measurements up to 15-km altitude fill a significant gap by characterizing the abundance and altitude variation of a wide suite of trace gases. These measurements, together with observations of dynamical and microphysical parameters, provide significant new data for constraining and evaluating global chemistry–climate models. Measurements include precursor and product gas species of reactive halogen compounds that impact ozone in the upper troposphere/lower stratosphere. High-accuracy, in situ measurements of ozone obtained during CONTRAST quantify ozone concentration profiles in the upper troposphere, where previous observations from balloonborne ozonesondes were often near or below the limit of detection. CONTRAST was one of the three coordinated experiments to observe the TWP during January–February 2014. Together, CONTRAST, Airborne Tropical Tropopause Experiment (ATTREX), and Coordinated Airborne Studies in the Tropics (CAST), using complementary capabilities of the three aircraft platforms as well as ground-based instrumentation, provide a comprehensive quantification of the regional distribution and vertical structure of natural and pollutant trace gases in the TWP during NH winter, from the oceanic boundary to the lower stratosphere.

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