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L. L. Pan
,
E. L. Atlas
,
R. J. Salawitch
,
S. B. Honomichl
,
J. F. Bresch
,
W. J. Randel
,
E. C. Apel
,
R. S. Hornbrook
,
A. J. Weinheimer
,
D. C. Anderson
,
S. J. Andrews
,
S. Baidar
,
S. P. Beaton
,
T. L. Campos
,
L. J. Carpenter
,
D. Chen
,
B. Dix
,
V. Donets
,
S. R. Hall
,
T. F. Hanisco
,
C. R. Homeyer
,
L. G. Huey
,
J. B. Jensen
,
L. Kaser
,
D. E. Kinnison
,
T. K. Koenig
,
J.-F. Lamarque
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C. Liu
,
J. Luo
,
Z. J. Luo
,
D. D. Montzka
,
J. M. Nicely
,
R. B. Pierce
,
D. D. Riemer
,
T. Robinson
,
P. Romashkin
,
A. Saiz-Lopez
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S. Schauffler
,
O. Shieh
,
M. H. Stell
,
K. Ullmann
,
G. Vaughan
,
R. Volkamer
, and
G. Wolfe

Abstract

The Convective Transport of Active Species in the Tropics (CONTRAST) experiment was conducted from Guam (13.5°N, 144.8°E) during January–February 2014. Using the NSF/NCAR Gulfstream V research aircraft, the experiment investigated the photochemical environment over the tropical western Pacific (TWP) warm pool, a region of massive deep convection and the major pathway for air to enter the stratosphere during Northern Hemisphere (NH) winter. The new observations provide a wealth of information for quantifying the influence of convection on the vertical distributions of active species. The airborne in situ measurements up to 15-km altitude fill a significant gap by characterizing the abundance and altitude variation of a wide suite of trace gases. These measurements, together with observations of dynamical and microphysical parameters, provide significant new data for constraining and evaluating global chemistry–climate models. Measurements include precursor and product gas species of reactive halogen compounds that impact ozone in the upper troposphere/lower stratosphere. High-accuracy, in situ measurements of ozone obtained during CONTRAST quantify ozone concentration profiles in the upper troposphere, where previous observations from balloonborne ozonesondes were often near or below the limit of detection. CONTRAST was one of the three coordinated experiments to observe the TWP during January–February 2014. Together, CONTRAST, Airborne Tropical Tropopause Experiment (ATTREX), and Coordinated Airborne Studies in the Tropics (CAST), using complementary capabilities of the three aircraft platforms as well as ground-based instrumentation, provide a comprehensive quantification of the regional distribution and vertical structure of natural and pollutant trace gases in the TWP during NH winter, from the oceanic boundary to the lower stratosphere.

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Chelsea R. Thompson
,
Steven C. Wofsy
,
Michael J. Prather
,
Paul A. Newman
,
Thomas F. Hanisco
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Thomas B. Ryerson
,
David W. Fahey
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Eric C. Apel
,
Charles A. Brock
,
William H. Brune
,
Karl Froyd
,
Joseph M. Katich
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Julie M. Nicely
,
Jeff Peischl
,
Eric Ray
,
Patrick R. Veres
,
Siyuan Wang
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Hannah M. Allen
,
Elizabeth Asher
,
Huisheng Bian
,
Donald Blake
,
Ilann Bourgeois
,
John Budney
,
T. Paul Bui
,
Amy Butler
,
Pedro Campuzano-Jost
,
Cecilia Chang
,
Mian Chin
,
Róisín Commane
,
Gus Correa
,
John D. Crounse
,
Bruce Daube
,
Jack E. Dibb
,
Joshua P. DiGangi
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Glenn S. Diskin
,
Maximilian Dollner
,
James W. Elkins
,
Arlene M. Fiore
,
Clare M. Flynn
,
Hao Guo
,
Samuel R. Hall
,
Reem A. Hannun
,
Alan Hills
,
Eric J. Hintsa
,
Alma Hodzic
,
Rebecca S. Hornbrook
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L. Greg Huey
,
Jose L. Jimenez
,
Ralph F. Keeling
,
Michelle J. Kim
,
Agnieszka Kupc
,
Forrest Lacey
,
Leslie R. Lait
,
Jean-Francois Lamarque
,
Junhua Liu
,
Kathryn McKain
,
Simone Meinardi
,
David O. Miller
,
Stephen A. Montzka
,
Fred L. Moore
,
Eric J. Morgan
,
Daniel M. Murphy
,
Lee T. Murray
,
Benjamin A. Nault
,
J. Andrew Neuman
,
Louis Nguyen
,
Yenny Gonzalez
,
Andrew Rollins
,
Karen Rosenlof
,
Maryann Sargent
,
Gregory Schill
,
Joshua P. Schwarz
,
Jason M. St. Clair
,
Stephen D. Steenrod
,
Britton B. Stephens
,
Susan E. Strahan
,
Sarah A. Strode
,
Colm Sweeney
,
Alexander B. Thames
,
Kirk Ullmann
,
Nicholas Wagner
,
Rodney Weber
,
Bernadett Weinzierl
,
Paul O. Wennberg
,
Christina J. Williamson
,
Glenn M. Wolfe
, and
Linghan Zeng

Abstract

This article provides an overview of the NASA Atmospheric Tomography (ATom) mission and a summary of selected scientific findings to date. ATom was an airborne measurements and modeling campaign aimed at characterizing the composition and chemistry of the troposphere over the most remote regions of the Pacific, Southern, Atlantic, and Arctic Oceans, and examining the impact of anthropogenic and natural emissions on a global scale. These remote regions dominate global chemical reactivity and are exceptionally important for global air quality and climate. ATom data provide the in situ measurements needed to understand the range of chemical species and their reactions, and to test satellite remote sensing observations and global models over large regions of the remote atmosphere. Lack of data in these regions, particularly over the oceans, has limited our understanding of how atmospheric composition is changing in response to shifting anthropogenic emissions and physical climate change. ATom was designed as a global-scale tomographic sampling mission with extensive geographic and seasonal coverage, tropospheric vertical profiling, and detailed speciation of reactive compounds and pollution tracers. ATom flew the NASA DC-8 research aircraft over four seasons to collect a comprehensive suite of measurements of gases, aerosols, and radical species from the remote troposphere and lower stratosphere on four global circuits from 2016 to 2018. Flights maintained near-continuous vertical profiling of 0.15–13-km altitudes on long meridional transects of the Pacific and Atlantic Ocean basins. Analysis and modeling of ATom data have led to the significant early findings highlighted here.

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