1. Introduction
Cloud microphysical properties are major drivers of cloud–radiation interactions, through complex processes that are still a challenge to accurately simulate in large-scale models. The vertical distribution of ice water content (IWC) inside nonprecipitating and deep convective clouds plays a central role in the interaction between clouds and incoming and outgoing radiation (e.g., Stephens et al. 1990). Different climate models still produce a very different ice water path, spanning up to an order of magnitude difference (Waliser et al. 2009; Li et al. 2012). New global datasets (Delanoë and Hogan 2010; Deng et al. 2013) offer new avenues to shed more light on the global and regional properties of nonprecipitating ice cloud microphysics, the cloud–radiation interactions, and the relationship between cloud properties and the large-scale environment (e.g., Su et al. 2008; Protat et al. 2011).
Although the retrieval of IWC in nonprecipitating ice clouds has been found to be reasonably accurate (Mace 2010; Protat et al. 2010a; Deng et al. 2013; Delanoë et al. 2013; Avery et al. 2012), there are reasons to believe this is not the case for convective cloud systems. The CloudSat IWC retrieval techniques currently rely on an assumed single statistical relationship between 95-GHz radar reflectivity (denoted as Z95) and IWC, sometimes with temperature T as an additional constraint (e.g., Hogan et al. 2006; Protat et al. 2007, hereinafter referred to as P07). These IWC–Z95 and IWC–Z95–T relationships were derived from aircraft in situ microphysical data collected in nonprecipitating ice clouds at midlatitude and tropical locations, and did not include any data collected within and around deep convective cores. Furthermore, these relationships were not derived using direct measurements of IWC and Z95. Rather, IWC was generally estimated from measured particle size distributions (PSDs) and a prescribed single statistical relationship between ice crystal mass and diameter [the so-called m(D) relationship], while Z95 was also simulated using the same PSD measurements and assumed m(D) relationship as inputs into T-matrix (Mishchenko et al. 1996) or simpler non-Rayleigh scattering calculations for spherical particles with corrected densities (e.g., Hogan et al. 2006; P07). The resulting variability around the fitted IWC–Z95 relationship was found to be very large in these studies, with IWCs having up to an order of magnitude difference for a given Z95, as discussed in, for example, Matrosov et al. (2002) and P07. An unknown fraction of this variability could actually be artificially produced by the use of a single m(D) for all ice clouds. More recent studies have used either bulk IWC or Z95 measurements combined with PSD measurements in order to refine m(D) (e.g., A. J. Heymsfield et al. 2010, hereinafter referred to as H10) or to include some of its variability in the calculations (e.g., Fontaine et al. 2014, hereinafter referred to as F14). However, in none of these studies were both bulk IWC and Z95 measurements available to directly characterize the real variability of the IWC–Z95 relationship.
It is also obvious in past studies that the fitted IWC–Z95 power-law relationship does not capture at all the largest IWCs simulated from the PSDs, owing to the non-Rayleigh scattering effects at 95 GHz distorting the IWC–Z95 relationship for high IWCs (see, e.g., the right panels in Fig. 1 in P07). This is why Matrosov and Heymsfield (2008, hereinafter referred to as MH08) developed a specific CloudSat IWC–Z95 relationship using only data points for which Z95 > 0 dBZ. However, this MH08 relationship is still based on IWCs and Z95 derived from measured PSDs and assumes a single m(D) for all ice clouds. In addition, the maximum estimated IWC and Z95 values included in the MH08 study were 2 g m−3 and 14 dBZ, respectively. This relationship cannot be extrapolated to larger values.
High ice water content detrained by deep convection in the upper troposphere is also a significant issue for aviation safety, especially in the tropics and subtropics where jet engines are found to be susceptible to engine power loss and damage in the vicinity of deep convection (e.g., Lawson et al. 1998; Mason et al. 2006; Grzych and Mason 2010; Strapp et al. 2016a), which have been related to a previously not well recognized form of engine icing involving high concentrations of small ice crystals, now referred to as ice crystal icing. Safety concerns related to these engines led the international regulation authorities and scientific community to organize an international airborne field campaign based in Darwin, Northern Territory, Australia, called the High Altitude Ice Crystal (HAIC)–High Ice Water Content (HIWC) campaign (Dezitter et al. 2013; Strapp et al. 2016a, see summary in section 2) during January–March 2014. Data collected during this field experiment include state-of-the-art particle size distribution, bulk IWC (including high values), and multibeam 95-GHz radar reflectivity measurements, providing an unprecedented opportunity to characterize the IWC–Z95 relationship and its true variability by using actual measurements.
The first objective of this paper is to develop and analyze the first ever IWC–Z95 relationship that does not include any assumption on the m(D) relationship and that includes measured IWC values reaching about 5 g m−3 (section 3). We then investigate how accurately IWC can be characterized from Z95 alone or with additional inputs such as temperature and/or location within a convective cloud system (convective or stratiform region). Accordingly, the variability of the IWC–Z95 relationship as a function of temperature and as a function of a convective index is studied in section 4. These IWC–Z95 relationships are finally used in section 5 to derive a statistical representation of the vertical distribution of IWC in and around tropical deep convective cores. Further possible applications of these relationships are discussed in section 6.
2. The HAIC–HIWC Darwin campaign measurements
The HAIC–HIWC field campaign took place from 16 January to 7 March 2014 out of Darwin. Details of the field campaign can be found in Dezitter et al. (2013). Only information relevant to this study is given in this section. Large-scale active monsoon conditions resulting in intense convective activity over the northern part of Australia were well established throughout much of the duration of the campaign, allowing for 23 scientific flights (for a total of 72 flight hours) to be conducted in very favorable conditions. The flight strategy was developed in conjunction with an aviation industry working group and is contained in the High Ice Water Content Project Science Plan (Strapp et al. 2016a). The objective was to fly a survey pattern through mesoscale convective system anvils at scales of approximately 200 km or larger, one that would initially include penetrations as close as possible to deep convective cores at flight altitude if deemed safe by the pilot. At least one convective core penetration and several flight legs in the immediate vicinity of the convective cores were ideally flown. In situ updrafts of up to 23 m s−1 were recorded at flight altitude, with peak updraft speeds exceeding 10 m s−1 in most flights. The maximum measured peak IWC was about 5 g m−3, and water contents exceeding 2 g m−3 for over 60 n mi (111 km) were measured.
The aircraft platform used for this campaign was the French Service des Avions Français Instrumentés de Recherche en Environnement (SAFIRE) Falcon 20, equipped with a suite of in situ microphysics probes, bulk total water content (TWC) probes, and a 95-GHz Doppler cloud radar named Radar Aéroporté et Sol de Télédétection des Propriétés Nuageuses (RASTA; Protat et al. 2004; Protat et al. 2009; Delanoë et al. 2013). The endurance of the Falcon 20 is 3.5 h, its nominal true airspeed is 200 m s−1, and its ceiling is at about −50°C in the tropical atmosphere near Darwin.
a. In situ microphysical measurements
The PSD was measured from 1- to 6400-μm diameter using the Cloud Droplet Probe (CDP, size range 1–50 μm, resolution of 2 μm) from Droplet Measurement Technologies (DMT), the 2D-Stereo Probe [2D-S, size range 10–1280 μm, resolution of 10 μm; Lawson et al. (2006)] from the Stratton Park Engineering Company (SPEC, Inc.), and the Particle Imaging Probe (PIP, size range 100–6400 μm, resolution of 100 μm) from DMT (Baumgardner et al. 2011). These probes were fitted with antishattering tips so as to reduce the shattering of large ice crystals onto the probe tips (e.g., Korolev and Isaac 2005). Remaining shattered particles were then removed by means of software, using the very small interarrival time of shattered particles (e.g., Field et al. 2006; Heymsfield 2007). Both approaches are indeed needed for an efficient mitigation of shattering (e.g., Jackson et al. 2014). In the present paper, we use composite 2D-S–PIP PSDs, which were derived using a simple weighting technique described in F14.
The reference bulk IWC measurement was obtained using a new isokinetic evaporator TWC probe (IKP) that was originally developed between 2007 and 2011 by the National Research Council of Canada (NRC), Environment Canada (EC, now known as Environment and Climate Change Canada), and Science Engineering Associates (SEA). The device was designed to measure high-IWC conditions up to 10 g m−3 at 200 m s−1 true airspeed in summer tropical and subtropical atmospheric conditions from −10° to −50°C, with a designed accuracy of 20%. A downsized version of the probe (IKP2) was then developed for NASA and the FAA in 2013 by SEA and NRC specifically to fit within the operational constraints of the Falcon 20 for the Darwin-2014 HAIC–HIWC flight measurement program. The operating principles of the IKP have been described by Davison et al. (2009), and are the same for the IKP2. The performance of the IKP2 probe has been assessed in multiple wind tunnel tests at four different facilities, and was found to operate without saturation and within 15% for water contents up to 5 g m−3 and airspeeds up to 150 m s−1. More details on this probe can be found in Strapp et al. (2016b) and Davison et al. (2016). Since the IKP2 measures the total water content, in real conditions liquid water and water vapor contributions should be subtracted to obtain IWC. Unfortunately, the hot-wire LWC sensor on the aircraft was unable to measure LWC below about 10% of the IWC in mixed-phase conditions, and LWC levels exceeding this value were very rare. Fortunately, the Goodrich ice detector could be used to detect the presence of liquid water. Two such regions in two very short flight segments were identified at −10°C, and these regions were excluded from the subsequent comparisons. The minimum detectable IWC of the IKP2 is determined by the noise level of the water vapor measurements of the IKP2 and background probes. This resulting noise level of the subtraction of the background humidity from the IKP2 humidity is a function of temperature: it is about 0.1 g m−3 at −10°C, dropping rapidly to about 0.005 g m−3 at −50°C. Since most data were gathered at temperatures colder than about −25°C, a minimum IWC of 0.05 g m−3 was chosen as the threshold to include in our analysis. The IKP2 dataset used in this study is at 1-s resolution and is the official final full dataset.
A second hot-wire bulk IWC probe, the so-called Robust probe developed by SEA for EC and the NRC, was integrated onto the CDP canister. The system provided reliable measurements at high altitude and high IWC during flight tests conducted by Airbus in 2010 and 2011 (Grandin et al. 2014). Based on results from previous hot-wire probes, it was known that the Robust probe’s collection efficiency for ice crystals would be significantly lower than unity. In this paper, we only use the Robust probe measurements to establish that the two very different bulk TWC probes provide highly correlated IWC measurements. Statistical comparisons using all Darwin 2014 HAIC–HIWC flights (not shown) reveal that these two TWC measurements of quite different operating principles track very closely (correlation coefficient = 0.96, standard deviation of the difference between the two probes ranging from 20% at IWC = 1 g m−3 and decreasing roughly linearly down to about 5% at IWC = 4 g m−3), and that the overall efficiency factor for the Robust probe is close to 0.45 in this HIWC environment.
b. Airborne cloud radar measurements
The RASTA 95-GHz airborne cloud radar (Protat et al. 2004, 2009; Delanoë et al. 2013) provides the radar reflectivities used in this study. The unique setup of this instrument includes the multibeam antenna system (three noncollinear antennas looking upward and three noncollinear antennas looking downward), allowing for the 3D wind to be retrieved below and above the aircraft flight altitude in a pseudovertical cross section during straight-line flight patterns. The RASTA radar has been carefully calibrated using accurate measurements of gains and losses through each radar component, remote fixed targets of known backscatter cross sections, and the Li et al. (2005) ocean surface backscatter technique (Bouniol et al. 2008). Quantitative comparisons with the CloudSat spaceborne radar (Protat et al. 2009) also showed that the two radar reflectivities agreed to within 1 dB, while the CloudSat radar reflectivities also agreed statistically within 0.4 dB with cloud radar data from five different ground-based sites. These results give confidence that the RASTA cloud radar is well calibrated, within 1 dB. Radar reflectivities in linear units from the nadir and zenith antennas nearest to the aircraft were linearly spatially interpolated, typically over 360 m (since the first nadir and zenith radar bins are at 180-m range), to produce a time series of Z95 at flight level, with a 1.2-s temporal resolution. Deriving the IWC–Z95 relationships from the nadir or zenith reflectivities instead of the interpolated ones did not result in any change in the coefficients of these relationships. It must be acknowledged that since the RASTA radar frequency (W band, around 95 GHz) is much higher than the frequency of the pilot radars on commercial aircraft (X band, around 10 GHz), the IWC–Z95 relationships derived in the present paper cannot be readily used to mitigate the HIWC threat in real time on commercial aircraft. More work will be done in the near future to derive the same relationships at X band and to evaluate the differences with the relationships from this paper, when data become available.
3. The IWC–Z95 relationship in deep tropical convective clouds
As explained in section 1, the dataset collected during the HAIC–HIWC campaign using the IKP2 probe and the RASTA cloud radar allows us the unprecedented opportunity to characterize the IWC–Z95 relationship without any assumption on the PSD or the ice crystal mass–size relationship and including high values of IWC up to 5 g m−3. For the sake of comparison with earlier approaches for which direct IWC and/or Z95 measurements were not available, we have also estimated IWC and Z95 using the PSD measurements, the single mass–size relationship used in P07 (which is that from Brown and Francis 1995), and T-matrix calculations using the aspect ratios estimated from the projected aspect ratio measured by raw in situ probes. This will be referred to as the PSD approach in the following. The resulting joint distribution of IWC and Z95 using this technique is shown in Fig. 1, using a Z95 and an IWC bin of 1 dB and 0.05 g m−3, respectively. Figure 2 shows the same joint distribution but derived from direct IKP2 IWC and RASTA Z95 measurements. For the sake of comparisons between Figs. 1 and 2, the mean IKP2 IWC in each Z95 bin is also given in both figures. The joint distributions are normalized for each reflectivity bin by the sum of all points in each IWC bin. In other words the sum of IWC frequencies is 1 for each reflectivity bin. Using such normalization allows for changes in the width of the IWC distribution for each Z95 bin to be readily observed.
Figure 2 shows that there is a very well-defined power-law relationship between IWC and Z95, characterized by a narrow IWC distribution width for Z95 of less than 10 dBZ. For Z95 > 10 dBZ the IWC distribution becomes wider, indicating that the retrieval of IWC from radar reflectivity will be characterized by larger errors for larger IWCs. This increase in the variability of IWC as a function of Z95 is consistent with the fact that higher 95-GHz radar reflectivities are more sensitive to the variabilities in the shape and density of the ice particles as non-Rayleigh scattering effects increase. Despite these potential effects though, the relationship is still well defined. It must be noted that there are currently no data available to assess whether this relationship can be applied to other regions of the world. This regional variability will be investigated to some extent in the future by collecting more data in different large-scale environments conducive to deep convection.
Comparison between Figs. 1 and 2 highlights the impact of using a single mass–size relationship and T-matrix calculations versus direct measurements for the first time. For Z95 < 5 dBZ, the widths of the IWC distribution are very similar for any Z95 bin. The differences between the two joint distributions are largest for Z95 > 10 dBZ and IWCs > 1.5 g m−3, where a bimodal distribution of Z95 as a function IWC appears with the PSD approach (Fig. 1; see the two possible values of Z95 for a given IWC for IWC > 1.5 g m−3). The more frequent of the two modes is in good agreement with the distribution obtained with the direct measurements (Fig. 2), with a tendency to slightly overestimate IWC for any Z95. The second mode largely overestimates IWC. The IWC distribution is also generally wider when direct measurements are used. This result shows that the natural variability of the mass–size relationship tends to broaden the range of possible IWCs for any Z95 greater than 10 dBZ.
It is also important to characterize the errors as a function of the reflectivity itself, since that is the way IWC is retrieved from (1). Figures 3c,d show that for Z95 < 15 dBZ, there is a systematic underestimation of IWC by about 10%–20%, with rms differences decreasing linearly from 70% at Z95 = 0 dBZ to 30% for Z95 = 15 dBZ. For Z95 > 15 dBZ, the bias then sharply increases from −10% to about 50% between 15 and 21 dBZ, and the rms differences range from 30% to 55% in that reflectivity range. As observed in Fig. 2, these larger IWC errors for Z95 > 17 dBZ can be attributed to strong departures from the power-law shape in the joint IWC–Z95 distribution.
This fit is shown in Fig. 2 (dashed line). The error analysis as a function of reflectivity (Fig. 4, dashed red) shows that IWCs retrieved using relationship (2) are slightly overestimated (bias less than 20% over the [0; 10] dBZ range) Z95 < 10 dBZ, with a similar rms difference for the results from relationship (1). The main benefit, as expected, is in the large improvement in the IWC retrieval for Z95 > 10 dBZ when compared to relationship (1) (cf. solid and dashed red lines in Fig. 4). The IWC retrieval bias is less than 10% up to Z95 = 19 dBZ, and increases up to only 25% at Z95 = 21 dBZ, which is a factor of 2 lower than when using relationship (1) (Fig. 4b). The rms difference decreases linearly from 65% to 20% between 0 and 20 dBZ, then increases sharply and up to 35% at Z95 = 21 dBZ (Fig. 4), which is again a large improvement over relationship (1), where the rms difference was up to 55% for Z95 = 21 dBZ.
When using IWC–Z95 relationships to retrieve IWC from Z95, it is assumed implicitly that the radar calibration is perfect. As indicated above, we believe from our calibration work that the RASTA cloud radar calibration is accurate to within 1 dB. The effect of a systematic 1-dB offset on the IWC retrieval can simply be estimated by fitting two power-law relationships such as (1) with 1 dB added or subtracted from the measured reflectivities, resulting in biases of +19% and −16%, respectively, over the whole reflectivity range. If the RASTA radar calibration is off by 1 dB, the IWCs produced using relationship (1) will be subject to this additional bias.
4. The variability of the IWC–Z95 relationship
In this section, we investigate two possible sources of the variability in the IWC–Z95 relationship shown in Fig. 2: the ambient temperature and the location within the convective cloud system (convective versus stratiform region). The underlying motivation for this variability study is to potentially use these parameters as additional constraints to the radar retrieval of IWC to reduce errors. It would have also been interesting to investigate the variability introduced by the underlying surface type (land versus ocean); however, too few cases of pure land-based convection were sampled during the HAIC–HIWC campaign. We also compare in this section the obtained relationships with tropical relationships found elsewhere in the literature.
a. Temperature variability
This large variability of the IWC–Z95 relationship with temperature suggests that the ratio of the number of large ice particles to medium/small ice particles changes with temperature, thereby changing the relationship between IWC (less sensitive to the large particles than Z95) and Z95 (very sensitive to the size of the larger ice particles). This is investigated further in Fig. 6, which shows the mean PSD for all HAIC–HIWC flights in the same 10°C temperature intervals as in Fig. 5. The temperature variability of the PSD is characterized by two main signatures. Both signatures are consistent with small ice particle formation and growth through water vapor deposition processes dominating in the upper troposphere, followed by the aggregation process dominating during particle sedimentation at warmer temperatures in convective ice clouds (e.g., Protat et al. 2010b). The first signature is a strong increase in the number of large ice particles in the 2–8-mm maximum diameter range as temperature increases. The second signature is a decrease of similar magnitude in the number of ice particles smaller than 1 mm, with the exception of the −10° ± 5°C temperature interval, where a very interesting increase in the number of particles smaller than 0.1 mm is observed, which may be an important result that can help us to understand the formation of high-IWC regions. This enhancement of the number of small particles may be the result of an efficient secondary ice production mechanism, such as that described by Hallett and Mossop (1974), where ice splinters are produced under certain conditions in a temperature window of −8° to −5°C. Ice crystal growth from supercooled liquid water lifted in ice phase by the convective updraft also potentially contributes to this increase in the number concentration of ice crystals of maximum diameter less than 0.1 mm. These processes will be investigated in more detail in a subsequent study, and are outside the scope of this paper. The main finding in Fig. 6 relevant to our understanding of the variability of the IWC–Z95 relationship with temperature is that the proportion of large to small particles increases with increasing temperature, implying lower IWCs for the same Z95 at warmer temperatures. This is fully consistent with the observed variability of the IWC–Z95 relationship with temperature in Fig. 5, as well as early studies (e.g., Heymsfield et al. 2013).
As observed in Fig. 7, where the IWC–Z95–T relationship is superimposed every 10°C onto the initial overall joint distribution of Z95 and IWC, a large part of the variability in the joint frequency distribution is captured by the spread in the IWC–Z95 relationships for different temperatures. Figures 3a and 3b show that there is indeed a measurable improvement of about 15% in bias for IWC > 1 g m−3 and a slight improvement of about 5% in the rms difference for 0.8 g m−3 < IWC < 2 g m−3 when using temperature as an additional constraint. Overall, Fig. 3 shows that IWC can be retrieved from (1) with a bias of less than 20% and an rms difference of less than 40% for IWC > 0.5 g m−3. The IWC errors as a function of reflectivity (Figs. 3c,d) show that there is indeed an improvement in the IWC bias when using temperature (biases are less than ±5%), but only up to Z95 = 16 dBZ (corresponding to a mean IKP2 IWC of about 2 g m−3). For Z95 > 16 dBZ, the bias and rms difference get slightly larger when using temperature as an additional constraint. As discussed previously, this is due to non-Rayleigh scattering effects altering the relationship between IWC and Z95 at large Z95. Figure 4 also indicates that relationship (2), derived using a nonlinear fit applied to data with Z95 > 0 dBZ, largely outperforms the IWC–Z95–T relationship (3). This result shows that the temperature constraint is actually detrimental to the IWC retrieval for Z95 > 16 dBZ.
The added value of using temperature as an additional constraint depends on the temperature layer and the reflectivity value (Figs. 8–12). There is a clear difference in the errors for reflectivities lower and larger than about 15–16 dBZ, so we will describe the errors for the two reflectivity ranges [0, 16] dBZ and [16, 21] dBZ separately. As discussed previously, this is due to the growing impact of non-Rayleigh scattering on the shape of the IWC–Z95 relationship. We will first describe how the errors vary as a function of temperature for the IWC–Z95 relationship (1) and, then, analyze to what extent temperature helps reduce those errors.
For Z95 < 15–16 dBZ, relationship (1) produces negative IWC biases for low temperatures and positive biases for warmer temperatures. The IWC bias goes from −40% to −20% at T = −50° ± 5°C (Fig. 8) and to −20% at T = −40° ± 5°C (Fig. 9); it then reaches an overall minimum of ±10% at T = −30° ± 5°C (Fig. 10), before increasing to peak overestimations of 20%–40% for T = −20° ± 5°C in the [0, 5] dBZ and [10, 15] dBZ reflectivity intervals. The IWC bias is then largest at T = −10° ± 5°C, reaching peaks of 60%–80% for Z95 < 9 dBZ. When using the nonlinear fit (2) between log(IWC) and Z95, which was designed to produce a better retrieval for large IWC (dashed red curves in Figs. 8–12), the IWC bias and rms difference at Z95 < 15–16 dBZ are degraded when compared with results obtained with relationship (1), except for low temperatures, where some improvement is observed (Figs. 8 and 9). In contrast, when using temperature as an additional constraint for Z95 < 15–16 dBZ (black curves in Figs. 8–12), the IWC bias remains small (<20%) at all temperature intervals, and much smaller than when using the IWC–Z95 relationship, except for the temperature interval T = −30° ± 5°C, where temperature does not have much impact. In terms of rms differences, Figs. 8–12 show that there is a general improvement of about 5% in all individual temperature bins for Z95 < 15–16 dBZ.
Figure 4 showed that the use of temperature as an additional constraint was overall slightly detrimental to the IWC retrieval for Z95 > 16 dBZ. Figures 8–12 further indicate that there is a compensating effect between the largely detrimental effects at low temperatures and the added value at warmer temperatures. The detrimental effect for Z95 > 16 dBZ is indeed only found at lower temperatures [especially T = −50° ± 5°C (Fig. 8) and T = −40° ± 5°C (Fig. 9)]. In these two temperature bins, it is therefore recommended to use IWC–Z95 relationships (1) or (2), not the temperature-dependent relationship (3). Using temperature has very little impact on the IWC retrieval at T = −30° ± 5°C, while at warmer temperatures (T = −20° ± 5°C and T = −10° ± 5°C), the use of temperature does improve the IWC bias and rms difference. Relationship (3) even performs at the same level or slightly better than the nonlinear relationship (2), which was designed for better high IWC retrieval.
In conclusion the addition of the temperature constraint in the IWC–Z95–T relationship (3) is overall largely beneficial, except when Z95 is larger than 16 dBZ for temperatures lower than −25°C. It is advised to use the nonlinear relationship (2) between log(IWC) and Z95 in that case.
b. Convective–stratiform variability
Convective and stratiform regions of tropical deep convective cloud storms are known to be characterized by different drop size distributions [e.g., Bringi et al. (2009), Thurai et al. (2010), and Penide et al. (2013a) for the Darwin region] and ice particle size distributions (Heymsfield et al. 2013). These convective and stratiform regions can be classified with ground-based weather radars using indices derived from reflectivity [magnitude, texture, presence of so-called radar bright band below the 0°C isotherm altitude; e.g., Steiner et al. (1995)] or from the retrieval of the drop size distribution parameters if the radar has dual-polarization capabilities (e.g., Thurai et al. 2010; Penide et al. 2013b). It is therefore of interest to investigate whether some of the variability of the IWC–Z95 relationship is due to microphysical differences between convective and stratiform regions. Overall, the convective region is characterized by updrafts and downdrafts routinely exceeding 5–10 m s−1 above the melting layer in tropical convective cores (e.g., May and Rajopadhyaya 1999; May et al. 2002; G. M. Heymsfield et al. 2010; Giangrande et al. 2013) while the stratiform region is characterized by a slight updraft in ice phase and slight downdraft in liquid phase, generally not exceeding a few tens of centimeters per second [e.g., Protat and Williams (2011) for the Darwin region; Gamache and Houze 1982; Chong et al. 1987; Nishi et al. 2007]. To separate the RASTA cloud radar profiles into convective and stratiform profiles, we have developed a simple convective index based on the maximum of the drafts. The RASTA cloud radar multibeam measurements allow for the vertical profile of the two horizontal wind components and the sum of the vertical velocity w and reflectivity-weighted terminal velocity VT to be retrieved using the three noncollinear Doppler velocity measurements as inputs into a multi-Doppler ground-based radar retrieval technique adapted to the airborne configuration [technique described in Protat and Zawadzki (1999); Collis et al. (2013)]. The criterion we use is that if (VT + w) is greater than 1 m s−1 or smaller than −3 m s−1 for at least 1 km in height above the 0°C isotherm altitude (i.e., in ice phase), then the cloud radar profile is classified as convective. Otherwise, it is classified as stratiform.
From Fig. 13, it is clearly observed that for any given Z95, IWC is systematically larger for convective profiles than for stratiform profiles. For instance, for Z95 = 20 dBZ, the mean IWC is 4.1 g m−3 in convective profiles and 3.2 g m−3 in stratiform profiles (~25% increase in IWC). A much higher frequency of occurrence of IWC > 2 g m−3 is also found in the convective profiles. Differences between convective PSDs and stratiform PSDs (Fig. 6) provide further insights into the microphysical processes involved in the large differences observed between the two IWC–Z95 relationships. Figure 6 shows that convective profiles are characterized by a much larger number of particles of maximum diameter up to about 2 mm than stratiform profiles (an order of magnitude difference for Dmax ~ 0.1 mm), while the number of large particles is similar. This is consistent with larger IWCs for a given Z95 in convective profiles. This large difference in the number of smaller particles in convective profiles suggests again that the production of small ice in convective updrafts through secondary ice formation–multiplication has the potential to generate areas of high IWC with moderate Z95.
Error analysis of IWC derived from the convective IWC–Z95 and IWC–Z95–T relationships (Fig. 14) shows that the bias and rms difference as a function of Z95 are very similar with or without temperature for Z95 > 9 dBZ, and the IWC bias is larger when using temperature for Z95 < 9 dBZ (Figs. 14a,b). Figures 14a,b show that the nonlinear relationship (2) between log(IWC) and Z95 produces the best error statistics overall, with IWC biases less than ±20% over the [2, 21] dBZ range, and rms differences decreasing from about 80% at Z95 = 0 dBZ down to 20%–30% for Z95 > 15 dBZ.
Error analysis of IWC derived from the stratiform IWC–Z95 relationship (7) (Fig. 15) shows that the use of temperature is beneficial to the IWC retrieval. Relationship (3) indeed outperforms relationships (1) and (2), with an IWC bias of less than ±10% over the whole reflectivity range and rms differences reduced by about 5%–10%, except for Z95 > 16 dBZ, where relationships (1) and (2) slightly outperform the temperature-dependent relationship (3). Using relationship (3), the rms difference decreases linearly from 60% at Z95 = 0 dBZ to 30% at Z95 = 15 dBZ, then, is of about 25%–35% for Z95 > 15 dBZ.
Overall, this analysis shows that the nonlinear relationship (2) between log(IWC) and Z95 should be used for convective profiles, and the temperature-dependent relationship (3) should be used for stratiform profiles. There is a large reduction of errors in stratiform IWC retrieval when temperature is used as a constraint, except for the bias in IWCs < 0.8 g m−3. The use of temperature yields improvement in bias by about 10% for IWCs > 0.8 g m−3 and in rms difference by about 30% for stratiform profiles over the whole IWC range.
c. Comparison with published IWC–Z95 relationships
The IWC–Z95 relationships from the HAIC–HIWC field experiment are for the first time derived from actual measurements of both IWC (including high values) and Z95. It is therefore appropriate to compare these new relationships with those developed previously in the literature to assess their accuracy, as these earlier relationships have already been extensively used to derive IWC and build cloud climatologies from satellite measurements (e.g., Delanoë and Hogan 2010; Mace 2010; Deng et al. 2013), and to evaluate the representation of cloud microphysics in numerical weather prediction models (e.g., Illingworth et al. 2007; Bouniol et al. 2010; Delanoë et al. 2011). Below, we describe how these earlier tropical relationships were derived and compare them with the new HAIC–HIWC relationships.
The H10 relationship (10) was obtained in convectively generated ice clouds during the Cirrus Regional Study of Tropical Anvils and Cirrus Layers–Florida-Area Cirrus Experiment (CRYSTAL-FACE; Jensen et al. 2004) and Tropical Composition, Cloud and Climate Coupling (TC4; Toon et al. 2010) tropical field experiments, which were carried out in Florida and Costa Rica, respectively. From these data a single m(D) relationship was derived using PSD measurements and closure with bulk IWC measurements, and Z95 has been simulated from the PSD measurements using Mie calculations. Mostly tropical cirrus clouds generated by deep convection were measured during these experiments. Relationship (12) was also derived in MH08 from the CRYSTAL-FACE dataset and with the same technique as that presented in H10. However, only Z95 > 0 dBZ data were included in the IWC–Z95 power-law fit. Relationship (11) from H10 uses the same technique applied to the NASA African Monsoon Multidisciplinary Analyses (NAMMA; Zipser et al. 2009) dataset. Most data were collected in tropical stratiform clouds and in the vicinity of deep tropical convective cores off the coast of West Africa.
Finally the P07 relationships (13) and (14) were obtained from a very large dataset of PSD measurements compiled from several campaigns conducted in the midlatitudes and in the tropics. This dataset includes a large variety of ice clouds, from thin cirrus to stratiform ice. The Brown and Francis (1995) m(D) relationship was assumed for all clouds. The quantity Z95 was calculated from the PSD measurements assuming spherical particles, but with a refractive index corrected following Oguchi (1983). Relationship (13) was obtained from the whole dataset, while relationship (14) was obtained using only the tropical data.
These relationships are all displayed in linear (Fig. 16a) and logarithmic (Fig. 16b) scales, together with the HAIC–HIWC relationships: in (1) for all profiles, in (6) for convective profiles, and in (7) for stratiform profiles. Each relationship is drawn only within the IWC range that was used to derive them, either simulated from the PSDs or measured by a bulk IWC probe. Interestingly, the convective and stratiform relationships derived from the HAIC–HIWC dataset are bounded by the H10 relationships (10) and (11). For Z95 > 10 dBZ, the lowest IWCs are produced by relationship (10), which indicates that the IWCs in tropical cirrus are much lower for a given Z95 than IWCs closer to the convective cores. Using the equivalent-melted diameter Deq as the definition of the diameter of the ice crystals (e.g., Delanoë et al. 2005; Delanoë et al. 2014), Z95 is proportional to a higher moment of the PSD (sixth moment under the Rayleigh scattering approximation, slightly lower and variable in non-Rayleigh scattering situations) than IWC (third moment), where the nth moment of the PSD is defined as
It is also clearly observed in Fig. 16 that the F14 relationships (8) and (9) produce IWCs that are very similar to the general HAIC–HIWC relationship (1) and the stratiform HAIC–HIWC relationship (7), respectively. The F14 relationships were obtained in tropical stratiform anvils in two very different large-scale environments and over different underlying surfaces (end of the West African monsoon season over land vs weakly forced oceanic convection in the Indian Ocean). In practical terms, this result suggests that the variability of the IWC–Z95 relationship in tropical stratiform anvils as a function of the underlying surface (land versus ocean) cannot be neglected and should be studied further. This is consistent with the reported morphological and microphysical differences of these stratiform regions along the tropical belt in Cetrone and Houze (2009).
In contrast, the P07 tropical relationship (14) is found to produce much larger IWCs than the HAIC–HIWC relationships, including the convective HAIC–HIWC relationship (6), although the dataset used in P07 does not include any measurement in convective clouds. This result suggests that the P07 relationship (14) likely overestimates IWC. This may be related to the use of the Brown and Francis (1995) m(D) relationship, which was later found to overestimate the mass of ice crystals and to fail to capture dependences on temperature and particle size that are a result of the complex ice microphysical processes (H10). In contrast, the P07 relationship (13) obtained using the whole dataset including midlatitude stratiform ice clouds produces IWCs closer to the general HAIC–HIWC relationship (1) for Z95 > 10 dBZ, but produces much larger IWCs for Z95 < 10 dBZ [similar to the HAIC–HIWC convective relationship (6)]. This overestimation is also probably due to the choice of the Brown and Francis (1995) m(D) relationship.
The only dataset other than HAIC–HIWC that includes data close to the convective cores is the NAMMA dataset, although the maximum values reported in this experiment did not exceed 2 g m−3, possibly because of instrumental limitations. The IWC–Z95 relationship (11) derived from the NAMMA dataset appears to produce IWCs larger than the convective HAIC–HIWC relationship (6) in this IWC range.
MH08 only included reflectivities larger than 0 dBZ in an attempt to mitigate the departures from the power-law shape of the IWC–Z95 relationship when fitting a power law using the whole IWC range. As observed in Fig. 16, the MH08 relationship tends to produce lower IWCs than the general [(1)] and convective [(6)] HAIC–HIWC relationships for Z95 < 6 dBZ and Z95 < 12 dBZ, and produces consistent results with the HAIC–HIWC convective relationship (6) between 1 and 2 g m−3. However, the MH08 study does not include any IWC values larger than 2 g m−3. Extrapolating the MH08 relationship above 2 g m−3 is not recommended, as it would result in large overestimations of high IWCs. It is a major added value of the HAIC–HIWC relationships that they are constrained with measured bulk IWC values exceeding 2 g m−3.
5. The vertical distribution of IWC within and around tropical convective cores
One of the primary objectives of the HAIC–HIWC campaign is to characterize the microphysical properties of regions of high IWC produced by deep convective systems and the processes responsible for the formation and maintenance of these regions (Strapp et al. 2016a). Quantitative information about the 99th percentile of the IWC as a function of the distance scale will also be derived from the IKP2 reference IWC measurements at flight altitude in coming studies in order to validate a new ice crystal regulatory envelope (Government Printing Office 2010, appendix D; EASA 2011, appendix P) that has recently become law. The radar-derived IWC dataset has the potential to greatly expand the in situ TWC dataset collected by the IKP2 and therefore the amount of data possibly available for the assessment of the regulatory ice crystal envelope. Although the radar dataset has been demonstrated to contain increased uncertainty relative to in situ measurements, it is hoped that the much larger combined radar–in situ dataset may help reduce the statistical uncertainty of the results from an in situ–only analysis, as well as filling in additional altitudes that have been undersampled by in situ measurements as a result of practical limitations. Below, we examine some preliminary results of remotely detected IWCs from the RASTA radar as a demonstration of how such results could be used to augment in situ measurements after a careful analysis of the data suitability.
Vertical profiles of radar-derived IWCs at ~200-m scale from the HAIC–HIWC dataset matched with ambient temperatures from the European Centre for Medium-Range Weather Forecasts (ECMWF) reanalyses were assembled to characterize for the first time the vertical distribution (or temperature dependence) of high IWC in deep tropical convective clouds. Unlike the reference IKP2 probe, the RASTA airborne cloud radar measured radar reflectivity above and below the aircraft at 60-m vertical resolution, which allows for a first analysis of the vertical distribution of IWC in a high-IWC environment in our dataset over the whole troposphere. It must be noted that RASTA reflectivities are not corrected for attenuation to produce Fig. 17. Underestimations of IWC are therefore expected for vertical profiles that include graupel, in which W-band attenuation is expected to be large. However, graupel produce high X-band pilot radar reflectivity (30 dBZ or more), which does not correspond to HIWC conditions thought to cause engine events (e.g., Mason et al. 2006; Strapp et al. 2016a).
Errors associated with the use of ECMWF temperatures have also been estimated by comparing flight-level temperature measurements. The bias is 0.20°C and the rms difference is 0.74°C. When examining only the convective profiles (stratiform profiles), the bias and rms differences are 0.27° and 0.77°C (0.19° and 0.74°C), respectively. In light of these results, in order to estimate the maximum IWC error due to temperature errors when using the IWC–Z95–T relationship, we have considered a maximum 1°C systematic overestimation, applied our relationship every 5°C in the interval from −10° to −50°C with or without the overestimation, and picked the maximum error produced. The maximum IWC error was less than 3% over the [−10, 20] dBZ range. In other words, the ECMWF temperature errors translate into negligible errors on the IWC retrieval using the proposed IWC–Z95–T relationship.
The statistical distribution of radar-derived IWC as a function of temperature is shown in Fig. 17a. The results indicate that the probability of encountering large values of IWC increases with decreasing temperature up to −35°C. At −35°C, an IWC value of 4 g m−3 was found in 1% of the samples. This frequency of occurrence then quickly dropped for temperatures colder than −35°C. Values of IWC exceeding 4 g m−3 (5 g m−3) were not detected at all at temperatures of −50°C (−35°C) or colder in our radar dataset, which suggests that these values may be rare. Separating these probabilities for convective and stratiform profiles (Fig. 17) using the convective–stratiform separation technique described in section 3b, IWC values greater than 4 g m−3 were exclusively found in convective profiles at all temperatures. IWC values greater than 3 g m−3 were also almost exclusively found in convective profiles and at temperatures colder than −25°C. Interestingly, an enhanced frequency of high IWC at the level from −10° to −5°C is also found in these convective profiles (Fig. 17b). This −10°C level is known to be important for microphysical growth processes, including ice particle growth from supercooled liquid water in convective updrafts and potentially ice multiplication–splintering through the Hallett–Mossop process (Hallett and Mossop 1974) and other secondary ice formation mechanisms. As discussed previously, PSDs in the −10°C layer are clearly characterized by a large increase in the number of ice crystals smaller than 0.1 mm (Fig. 6), which is consistent with secondary ice production in that specific layer.
The highest priority temperature interval for the aviation regulatory interests is the −50° ± 5°C interval (Strapp et al. 2016a), as it corresponds to the typical cruise altitude for many commercial aircraft. At the −50°C level our radar IWC statistics indicate that values greater than approximately 1.5 g m−3 were only found in convective profiles (according to the radar retrievals) during the Darwin 2014 HAIC–HIWC experiment. Practically, this important result suggests that future research should focus on developing convective–stratiform indices from geostationary satellites to detect high IWC and mitigate the high-IWC threat to civil aviation at this flight level.
The IWC statistics of the −50° ± 5°C temperature interval derived from the entirety of the radar-derived IWC profiles are next compared to radar-derived IWCs at flight level from only the −50° ± 5°C temperature interval flight segments, using the same IWC–Z95 relationship. Assuming that there is no bias in the nature of the flight segments executed at the other levels relative to those at −50°C (i.e., the clouds and cloud regions sampled at other altitudes are similar to those comprising the −50°C in situ dataset), and that there are no unidentified range-dependent errors in the radar IWC estimates, the differences in IWC PDFs are most likely due simply to the number of samples. Figure 18 shows the PDFs of IWC as a function of temperature for this temperature interval. The solid lines in Fig. 18 are the PDFs derived from the whole vertical profiles of IWC, and the dashed lines are the PDFs derived from the radar-derived IWCs at flight altitude. The flight-level PDFs are found to match the reference PDFs well down to the 0.1% frequency level, with a slight overestimation of the frequency of occurrence of IWCs of 2–3 g m−3 in the convective profiles, along with an underestimation of the frequency of IWCs larger than 0.7 g m−3 in the stratiform profiles. Figure 18a–c also show that the PDFs at flight level are truncated at frequencies lower than about 0.1%. Since the regulatory objective is to derive 99th percentile values of IWC, this example analysis would suggest that the HAIC–HIWC in situ dataset should be sufficient to achieve this goal.
6. Conclusions
Unprecedented bulk measurements of ice water content up to about 5 g m−3 collocated with 95-GHz radar reflectivities were used in this study to analyze the IWC–Z95 relationship and its variability as a function of temperature and the nature of convection (convective vs stratiform). The unique aspect of this work is that, unlike past studies, these relationships do not include any assumptions about the statistical relationship between crystal mass and maximum dimension or any errors arising from scattering calculations of Z95 from particle size distributions. It is also the first study to include measured IWC values greater than about 2 g m−3 and up to about 5 g m−3.
Our results indicated that using a single power-law IWC–Z95 relationship allows for the radar retrieval of IWC with ~(10%–30%) bias and 40%–70% rms difference, depending on IWC. The IWC is also found to be underestimated by about 10%–20% for reflectivities lower than 15 dBZ, but is largely overestimated for reflectivities larger than 15 dBZ, which is attributed to non-Rayleigh scattering effects distorting the relationship between IWC and Z95 at large Z95. A nonlinear relationship between log(IWC) and Z95 has therefore been developed, which allows for IWC retrievals with biases less than 20% and rms differences of 20%–35% for Z95 > 15 dBZ.
We then showed that the temperature variability of the IWC–Z95 relationship was large and that temperature could be used as an additional constraint to further reduce uncertainties on radar-derived IWCs, except when Z > 16 dBZ for temperatures lower than −25°C, where the nonlinear relationship between log(IWC) and Z95 largely outperforms the temperature-dependent relationship. This variability with temperature has been clearly linked to and is consistent with the natural temperature variability of PSDs measured during the HAIC–HIWC campaign. Our variability study also shows that the nonlinear relationship (2) between log(IWC) and Z95 should be used for convective profiles, and the temperature-dependent relationship (3) should be used for stratiform profiles to minimize IWC retrieval errors.
The radar results will be combined with those from a second just-completed flight program, and then examined for suitability in augmenting in situ IWC data collected for a future assessment of new aircraft certification rules for flight in ice crystals. Some preliminary results from the Darwin flight campaign related to these aviation objectives are reported upon here. Using all profiles collected during the field experiment (72 flight hours), a joint frequency distribution of radar-derived IWC and temperature within and around deep tropical convective cores was constructed. The results showed that IWC values greater than 4 g m−3 on ~200-m-distance scales were exclusively found in convective profiles at all temperatures, and IWC values greater than 3 g m−3 were also almost exclusively found in convective profiles and at temperatures colder than −25°C. At the −50° ± 5°C level, which is the cruise level of many commercial jet aircraft, IWC values greater than 1.5 g m−3 were exclusively found in convective profiles during the HAIC–HIWC experiment. This result suggests that future efforts should be directed toward the development of a convective–stratiform index from geostationary satellites in order to detect and mitigate this type of high-IWC threat to civil aviation at this flight level. Nevertheless, it must be noted that recent analyses have highlighted that in-service engine events are most often associated with traverses across large convective anvils, suggesting that long exposures to moderate values of IWC may be as important as short exposures to high IWC. More studies will be needed to address this potentially different type of HIWC environment.
Acknowledgments
This research has received funding from the Federal Aviation Administration, Aviation Research Division, and Aviation Weather Division, under Agreement CON-I-2901 with the Australian Bureau of Meteorology. The research was also conducted as part of the European Union’s Seventh Framework Program in research, technological development, and demonstration under Grant Agreement ACP2-GA-2012-314314, and the European Aviation Safety Agency Research Program under Service Contract EASA.2013.FC27. Funding to support the development and testing of the isokinetic bulk TWC probe was provided by the FAA, NASA’s Aviation Safety Program, Environment and Climate Change Canada (formerly known as Environment Canada), and the National Research Council of Canada. Funding for the Darwin flight project was provided by the EU Seventh Framework Program agreement and the EASA contract noted above, the FAA, NASA’s Aviation Safety Program, the Boeing Company, Environment and Climate Change Canada, and Transport Canada.
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