1. Introduction
Warm cloud microphysical parameterizations usually divide the droplet spectrum within a cloud into cloud droplets and raindrops by size and calculates their physical quantities separately, following Kessler (1969, hereafter K69). Cloud droplets with small terminal velocity are assumed to remain within a cloud, and larger raindrops with appreciable terminal velocities are assumed to settle gravitationally, causing precipitation. The value of a separation radius




















Meanwhile, various evidence suggests that autoconversion is also influenced by various other factors besides




Autoconversion rates vary much more between schemes than accretion rates, often causing a difference by several orders of magnitude for the same
Considering the difficulty of obtaining reliable observation data, one valuable approach to evaluate cloud microphysics parameterizations is to analyze the results from a model that can simulate the variation of droplet spectrum directly, such as a spectral-bin model (SBM), which solves the stochastic collection equation (SCE). The results of the SBM initialized with observed DSD data (Wood 2005; Hsieh et al. 2009) or with the idealized DSD (Seifert and Beheng 2001; Franklin 2008; Lee and Baik 2017) were used to evaluate parameterizations of A and C. Meanwhile, KK00 and Kogan (2013) developed a formula for A and C from regression analysis of SBM data, when a stratocumulus or cumulus cloud is simulated by large-eddy simulation (LES). LES has an advantage of providing the dynamically balanced DSD within the fine structure of the cloud, which plays an important role in the calculation of A and C from (1) and (2) (Kogan 2013). Evaluations have been carried out usually by the comparison of A and C calculated from the SBM and the parameterization. However, the comparison can be affected by factors that are not represented in the parameterization, such as DSD, TICE, and aging time.
An Eulerian model, such as the SBM, calculates only the averaged values of A and C over the grid size and the time step. Moreover, the numerical diffusion of the droplet spectrum, in both physical and spectral space, can hinder the accurate calculation of A and C. Therefore, probably the ideal approach to calculate A and C is to capture the moment of each Lagrangian droplet growing to a raindrop together with the background condition, as suggested by Straka (2009). Nonetheless, it is possible only when cloud droplets are simulated by Lagrangian particles.
Recently, several groups developed Lagrangian cloud models (LCMs), in which the cloud microphysics of Lagrangian droplets and cloud dynamics are two-way coupled (e.g., Andrejczuk et al. 2010; Shima et al. 2009; Sölch and Kärcher 2010; Riechelmann et al. 2012; Hoffmann et al. 2017). In these models, the flow field is simulated by LES, and the droplets are treated as Lagrangian particles, which undergo cloud microphysics while interacting with the surrounding air.
Hoffmann et al. (2017) applied the LCM to clarify the mechanism of raindrop formation in a shallow cumulus cloud. They found that the rapid collisional growth, leading to raindrop formation, is triggered when droplets with a radius of 20 μm appear in the region near the cloud top that is characterized by large liquid water content, strong turbulence, large mean droplet size, a broad DSD, and high supersaturations. They also found that the rapid collisional growth leading to precipitation can be delayed without the broadening of the DSD, when turbulence is weak. On the other hand, TICE does not accelerate the triggering of the rapid collisional growth, but it enhances the collisional growth rate greatly after the triggering and thus results in faster and stronger precipitation. These results imply that both TICE and the dispersion of DSD are important factors to determine autoconversion and accretion.
The present paper aims to investigate the characteristics of the parameterizations of autoconversion and accretion by analyzing LCM data. For this purpose, we first compare A and C from the existing parameterizations with LCM data. At the next step, we investigate the effects of various other factors, such as the dispersion of the DSD, TICE, and aging time and parameterize their effects with an aim to improve the parameterization.
2. Simulation and analysis
a. Model description








































b. Simulation setup


The average distance between superdroplets is initially 3.4 m, yielding a total number of 7.9 × 108 superdroplets and about 200 superdroplets per grid box, which has been found to be sufficient to represent the collisional growth correctly (Riechelmann et al. 2012; Arabas and Shima 2013; Unterstrasser et al. 2017). Two different initial droplet number concentrations
Two simulations are carried out for each
c. Calculation of autoconversion and accretion





















Grouping of collision event to autoconversion, accretion, and self-collection (⃝: raindrop; ×: cloud droplet).

Here, the critical radius that separates a cloud droplet and a raindrop is given by













It should be mentioned that the calculations of A and C from the LCM and the SBM are somewhat different in nature. First, A and C are calculated by the integral of SCE within a grid in the SBM, but they are calculated at every collision event of Lagrangian droplets in the LCM. It also implies that they are affected by the growth history of Lagrangian droplets in the LCM. Second, the occurrence of autoconversion and accretion is continuous and deterministic in the SBM, but it is intermittent and stochastic in the LCM. Accordingly, the values of
3. Results
a. Distribution of autoconversion and accretion
Figure 1 shows the distributions of autoconversion, accretion,

Distributions of
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
Autoconversion is larger than accretion initially (t = 20 min), but accretion soon dominates the conversion to raindrops (t = 25 min). It also reveals that both autoconversion and accretion appear in the upper part of the cloud initially (t = 20 min), but they appear in the center in the later stage (t = 25 min). It reflects the fact that raindrop formation is triggered near the cloud top that is characterized by strong turbulence and a broad DSD (Hoffmann et al. 2017).
The dominance of autoconversion soon after the triggering of raindrop formation is clearly illustrated in the time series of the total amount of autoconversion and accretion per unit time within the cloud (Fig. 2a). As a result of autoconversion and accretion,

Time series of cloud microphysical variables during the evolution of a cumulus cloud (angle brackets mean the total amount within the cloud; solid: TURB; dotted: GRAV) for (a)
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
Figure 2 also shows that both autoconversion and accretion are smaller in GRAV, although they start to appear at about the same time. It reflects the fact that TICE does not accelerate the timing of the raindrop formation, but it increases the amount of precipitation (Hoffmann et al. 2017). Seifert et al. (2010) also showed, using an SBM, that precipitation increases about 2 times, as
b. Comparison of A and C with parameterizations
Figure 3 shows the variation of A with

Variation of (top) A and (bottom)
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
Autoconversion and accretion formulations for the four parameterizations examined (units are cm−3 for

Remarkably, the results reproduce successfully the Kessler-type autoconversion parameterization, such as (3) and (4), in which the threshold
The closest agreement in the relation
Similarly, we examined the variation of C with

Variation of (top) C and (bottom)
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
Finally, the sensitivity to

Comparison of A and C from different
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
c. Influence of other factors on A and C
As discussed in the introduction, various evidence indicates that autoconversion is influenced not only by
To clarify the influences of these factors, we replot Fig. 3 based on the subgroup of data according to the values of the dissipation rate

Variation of A with
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
It is difficult, however, to identify the effects of
There are at least five variables that can influence autoconversion, such as
First, we examine how

Variations of
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
The variations of

Variations of
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1

Variations of
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1












The existence of the threshold R is attributed to two factors. First, if both R and
Similar to the case of autoconversion, we replot Fig. 4 based on the data regrouped according to the values of

Variation of C with
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
The broader DSD makes K larger in (2), thus producing larger accretion, even if
d. Variations of 
and 


We showed in the previous section that autoconversion varies significantly with
With an aim to provide the information on the evolution of

Time series of the mean variables within a cloud (solid: TURB; dotted: GRAV; blue:
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
The aging process is naturally realized by the initial increase of
Another approach to estimate

Histograms of the number of grids in the (a) ε–qc and (b) σ–qc domains (Δ logε = 3.74 × 10−2 cm2 s−3, Δ logσ = 3.03 × 10−2 μm, and Δ logqc = 1.72 × 10−2 kg kg−1;
Citation: Journal of the Atmospheric Sciences 75, 11; 10.1175/JAS-D-18-0080.1
Contrary to the box collision model, in which
The previous parameterizations only in terms of
4. Conclusions
In the present paper, we applied the LCM to investigate the cloud microphysics parameterization for shallow cumulus clouds, focusing on autoconversion and accretion. Autoconversion and accretion were calculated directly by capturing the moment of the conversion of individual Lagrangian droplets from cloud droplets to raindrops.
The autoconversion rate A and the accretion rate C, calculated from the LCM, were compared with various parameterizations (K69; TC80; B94; KK00). The calculation produced for the first time the formulas of autoconversion and accretion, such as
Furthermore, LCM results help to clarify how
Comparison of TC80 and a new parameterization [a = 1.0 cm−1 μm−1 s−1, b = 8.8 × 10−3 cm−2 s3,

It is important to mention that (1) and (2) to calculate A and C are universal, independent of cloud dynamics and nucleation. Cloud dynamics and nucleation affect the variation of turbulence and DSD, and their effects are realized only in terms of the variation of K and n in (1) and (2) through the variation of
We hope that an improved cloud microphysics parameterization, which takes into account the effect of the dispersion of DSD, TICE, and aging time, can be developed in the future based on the information obtained from the present work. It will be necessary for the application of the parameterization, however, to develop a general method to predict the variation of
This work was funded by the Korea Meteorological Administration Research and Development Program under Grants KMI 2015-10410 and KMI 2018-07210. This LES/LCM used in this study (revision 1891) is publicly available (https://palm.muk.uni-hannover.de/trac/browser/palm?rev=1891). For analysis, the model has been extended, and additional analysis tools have been developed. The code is available from the authors on request. Most of the simulations have been carried out on the Cray XC-30 systems of the North-German Supercomputing Alliance (HLRN) and the supercomputer system supported by the National Center for Meteorological Supercomputer of Korea Meteorological Administration (KMA).
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