1. Introduction
Clouds are very important elements in the earth–atmosphere radiative balance because of their role in the interaction with shortwave (SW) (or solar) and longwave (LW) (or thermal) radiation. On one hand, they reflect and absorb part of the incoming SW radiation; on the other hand, they absorb LW radiation emitted from the earth’s surface and, in turn, reemit LW radiation back to the earth and to space. Thus, clouds are the dominant modulators of radiation, both at the surface and at the top of the atmosphere (TOA) (Dong et al. 2006). A way of quantifying the cloud radiation effects at the surface and at the TOA is the cloud radiative forcing (CRF), which is defined as an instantaneous change in net total radiation (SW plus LW; in W m−2) obtained under cloudy conditions and its clear-sky counterpart; CRF can produce a cooling (negative CRF) or a warming (positive CRF) effect on the earth–atmosphere system.
CRF has been a research topic over the last decades because of its importance in understanding the effects of clouds on the radiative balance, which controls the earth–atmosphere temperature; Ramanathan et al. (1989) and Harrison et al. (1990) were the first to estimate the global CRF and the seasonal effects of clouds on the radiation budget from Earth Radiation Budget Experiment (ERBE) data. Since then, with the improvement of satellites, ground-based instruments, and radiative transfer and climate models, many other studies dedicated to the radiative effects of clouds were developed (Mace et al. 2006; Dong et al. 2006; Kassianov et al. 2011; Berg et al. 2011; Liu et al. 2011), both at the surface and at the TOA. The calculation of CRF at the surface can be done through ground-based observations, and the information gathered at different sites all over the globe constitutes valuable information for validation purposes. The description of the cloud effects on the surface radiation budget is a critical component for understanding the current climate and an important step toward simulating potential climate change (Dong et al. 2006).
In this work, the shortwave cloud radiative forcing (CRFSW), defined as the difference between the SW net fluxes (downward minus upward SW fluxes) obtained under both all-sky and clear-sky conditions, is calculated from irradiance measurements taken at the surface in the Geophysics Centre of Évora, which is located in the south of Portugal, about 100 km east from the Atlantic coast. Studies on the shortwave radiative forcing in this region, both at the TOA and surface levels, have already been made but mostly using atmospheric modeling and concentrating on the radiative effect of aerosols and of contaminated clouds by desert dust aerosols (Santos et al. 2008, 2013). However, no investigation of the cloud radiative effects in the shortwave spectral range has been done at the site using the long time series of surface SW irradiance measurements taken during the period 2003–10.
These studies can be extremely useful to validate satellite assessments of radiative forcing or model calculations, particularly over a region of potential interest that is affected by contrasting air masses (Raes et al. 2000), and thus offers opportunities for studying not only clouds, but also their interaction with aerosols from different origins. During the winter season, the large-scale atmospheric circulation in Portugal is primarily determined by the location and intensity of the Icelandic Low. The area is on the track of front systems typical of midlatitude regions, brought from the Atlantic Ocean by the westerly circulation and carrying moist air. These fronts affect the region more often in winter and spring, before the polar front moves northward. When this happens, the synoptic circulation becomes constrained by the Azores anticyclone (during late spring and summer), which transports dry warm air from north or northeast into the region and is associated with clear-sky conditions. Besides, in the warm season, the intense surface heating of inland regions results frequently in the development of a thermal low pressure system at the Iberia scale, with shallow convection originating mostly in the afternoon (Costa et al. 2010).
In this study, the CRF estimates are relative only to the SW spectral range and involve global SW irradiance measurements in two different spectral bands obtained for all cloudy-sky conditions, in terms of cloud type and cloud fraction (from partially cloudy to overcast), taken from ground-based instruments. Other authors have studied the variations of CRF for several sky conditions and for specific types of clouds (Dong et al. 2006; Berg et al. 2011; Liu et al. 2011). Berg et al. (2011) found a shortwave CRF average value of −45.5 W m−2 for shallow cumuli; Dong et al. (2006) studied the seasonal and monthly variations of CRF for a midlatitude site and showed that CRFSW at the surface exhibited minimum values in spring and had a spring seasonal average of −61.3 W m−2 for all-sky conditions. This study also analyzes the seasonal and monthly variability of the surface CRFSW for all-sky conditions over a midlatitude site in southwestern Europe, aiming to contribute to the understanding of the cloud impact on Earth’s radiation balance, which is important for climate and climate change studies (Ramanathan et al. 1989).
The next section describes the methodology as well as the data used to estimate the shortwave cloud radiative forcing at the ground surface. Section 3 presents the results of this study, and section 4 summarizes the work and the main results.
2. Data and methodology
a. Instruments and data
The measurements used here are recorded with two field instruments, a multifilter rotating shadowband radiometer (MFRSR) (Harrison et al. 1994) and an Eppley black and white pyranometer, both operating since 2003 at the Atmospheric Physics Observatory of Geophysics Center of Évora (CGE; 38°34’N, 7°54’W, 300 m above mean sea level). The MFRSR is an instrument that provides automatic measurements of global and diffuse components of the spectral and broadband hemispherical shortwave irradiances with a temporal sampling of 1 min. It has seven channels, covering the visible and partly the near-infrared spectral regions (415, 500, 615, 673, 870, and 940 nm), with 10 nm of bandwidth and a broadband channel (300–1100 nm), used in this study. The Eppley black and white pyranometer provides measurements of hemispherical shortwave global irradiances, corresponding to the spectral region between 285 and 2800 nm, with a temporal sampling of 1 min and providing 10-min averages. The instruments are regularly calibrated, and their uncertainties are estimated at 5%.
MFRSR broadband irradiance measurements taken from August 2003 to August 2010 have considerable gaps within the period, as listed in Table 1. Only the periods where coincident shortwave irradiance measurements from both instruments occur are used in the study. These measurements cover all-sky situations in terms of cloud type and cloud fraction. The two sets of data from the MFRSR and Eppley instruments are used because the spectral bands of the instruments cover different fractions of the solar radiation spectrum at the surface (the MFRSR broadband channel covers approximately 73.5%, and the Eppley pyranometer covers roughly 95%). This allows comparison of the SW cloud radiative forcing at the surface obtained with two different sets of observed data for the same time period, geographic location, and atmospheric conditions and allows us to estimate the relative contribution of the MFRSR forcing to the total forcing (Eppley).
MFRSR data available in Évora (cells with X) for the period 2003–10.

Aerosol optical thickness (AOT) and precipitable water vapor (PWV) data obtained from direct sun measurements continuously taken at the observatory of the Évora Geophysics Centre as part of the Aerosol Robotic Network (AERONET) (Holben et al. 2001) are also used in the study, as explained in the next subsection.
b. Clear-sky irradiance
The calculation of the SW cloud radiative forcing, which is described in the next subsection, requires irradiance values for clear-sky conditions; these values are not possible to obtain from measurements during cloudy periods. Long and Ackerman (2000) proposed a method to identify and produce continuous estimates of clear-sky irradiance values at the surface based on the empirical fit of clear-sky irradiance functions using the cosine of the solar zenith angle as the independent variable. While this method provides very good estimates of clear-sky irradiance at the surface for the day of the fitting, it ignores changes in atmospheric variables, such as PWV and AOT, between clear-sky days and therefore may introduce errors in the clear-sky irradiance estimates. A different approach is proposed here, based on radiative transfer (RT) calculations. The clear-sky irradiances corresponding to each measurement are calculated using the Library for Radiative transfer (LibRadtran) package (Mayer and Kylling 2005), taking into account both the MFRSR and Eppley spectral response functions. The surface is considered as a Lambertian reflector, with an albedo value of 0.22 for Eppley simulations (http://speclib.jpl.nasa.gov/) and 0.27 for MFRSR broadband channel simulations obtained from spectral reflectance ground-based measurements with a portable spectroradiometer (described by Potes et al. 2012). A midlatitude type of atmospheric vertical profile for winter or summer (McClatchey et al. 1971) was considered, according to the season. PWV and AOT values of 15 kg m−2 and 0.1 were used, respectively, corresponding to the average of AERONET measurements for the 7-yr period and therefore considered representative of the conditions over Évora. Aerosols are assumed to be described by the Shettle (1989) default properties, with rural-type aerosols in the boundary layer, background aerosols above 2 km, spring–summer or fall–winter conditions (according to the season), and 50-km visibility. The radiative transfer equation is numerically solved using the discrete ordinate method (Stamnes et al. 2000) with 16 quadrature angles.





Conversion functions accounting for (a) AOT variations on MFRSR irradiances, (b) PWV variations on MFRSR irradiances, (c) AOT variations on Eppley irradiances, and (d) PWV variations on Eppley irradiances.
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1



Relative error (%) associated with the solar irradiance calculation using the conversion factors, as a function of solar zenith angle.
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1
Statistics of the comparisons between exact radiative transfer calculations of clear-sky irradiance and the corresponding approximation using the conversion factors.

The clear-sky irradiances obtained applying the described methodology are checked against clear-sky observations and are also compared to those obtained applying the method proposed by Long and Ackerman (2000). Figure 3 shows an example of the performance of the method for a case of moderately high values of AOT and PWV (0.47 and 24.6 kg m−2, respectively) on 10 August 2010 for MFRSR and Eppley measurements. The clear-sky irradiance obtained from RT considering an AOT of 0.1 and PWV of 15 kg m−2 clearly overestimates the measurements; however, when the conversion factors are applied [Eq. (2)] accounting for the actual AOT and PWV values, a very good match between RT calculations and measurements is obtained in both cases, especially from around 1000 UTC until the end of the day. Small differences between observations and RT calculations may also be due to variations in the AOT and PWV during the day, since daily averages are used to get the conversion factors for a certain solar zenith angle. The fit line obtained from the Long and Ackerman (2000) method also adjusts very well to the experimental points. However, this method requires a minimum number of clear-sky measurements over a considerable range of solar zenith angles to guarantee a statistically accurate calculation (Long and Ackerman 2000), which is not always available. Under cloudy conditions, the fits obtained with this method must be interpolated, introducing additional uncertainties in the clear-sky irradiance. To compare the uncertainties introduced by the different methods, periods of at least four successive clear-sky days were selected from the complete dataset (2003–10), in order to test the effect of the interpolation of the fit coefficients in a similar way to that followed by Long and Ackerman (2000), as well as to test the effect of the RT-based methods. A total number of 64 days were found fulfilling the conditions mentioned before. Figure 4 shows the corresponding frequency histogram of relative differences between Eppley measured and estimated clear-sky irradiance using actually fitted coefficients (diagonal striped bars), interpolated coefficients (solid gray bars), RT calculations (solid black bars), and RT calculations combined with the conversion factors (checkered bars). Of the data obtained with the fitting method (Long and Ackerman 2000), 83% are within 3% of the clear-sky measurements, whereas, when the fitting coefficients are interpolated, only 58% of the data are within the same threshold (about the same percentage for the uncorrected RT method). The value increases to 70% when considering the method proposed here (RTM corrected). Similar results were obtained for the MFRSR data (plot not shown here), with 84% of the fitted clear-sky irradiances within 3% of the observations and 70% of the RT-corrected irradiances within the same limit.

Global solar irradiance measurements (dots) and corresponding calculations using the Long and Ackerman (2000) method (line), the RT approach for fixed AOT and PWV values (triangles), and the RT approach combined with the conversion functions (squares) for 10 August 2010: (a) MFRSR and (b) Eppley.
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1

Frequency histogram of relative differences between Eppley 1-min measured and estimated clear-sky irradiance using actually fitted coefficients (diagonal striped bars), interpolated coefficients (solid gray bars), RT calculations (solid black bars), and RT calculations combined with the conversion factors (checkered bars).
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1
Although the fitting method presents the best performance (NRMSE of 2%), the proposed method constitutes a valid alternative (NRMSE of 3%), especially useful while clear-sky measurements are not available (preventing the use of the fitting method), as frequently happens during relatively long periods (more than 4 successive days) in autumn, winter, and even springtime, when day-to-day changes in columnar aerosols and water vapor are also frequent. Since the main scope of this study is the analysis of the cloud radiative forcing at the surface, the clear-sky irradiance is estimated using the RT-corrected method, which introduces an uncertainty of 3% (NRMSE), comparable to the uncertainty of the measurements (~5%).
c. Cloud radiative forcing








The (normalized) cloud radiative forcing calculated using the MFRSR broadband data and the Eppley pyranometer data are referred to hereinafter as MFRSR (N)CRFSW and Eppley (N)CRFSW, respectively.
3. Results and discussion
The CRFSW as well as the NCRFSW are calculated using data from the MFRSR broadband channel and from the Eppley pyranometer measurements [Eq. (4)], both corresponding to 10-min averages. The results correspond to the whole period of measurements indicated in Table 1 for all-sky conditions. Discarding the clear-sky periods, the data corresponds to a total of 28 061 cloud occurrences (10-min bins) in 963 days (240 in winter, 238 in spring, 251 in summer, and 234 in autumn), considering all cloud situations in terms of type and fraction. The daily-mean values of the CRFSW and NCRFSW are calculated by integrating the 10-min averaged values of CRFSW and NCRFSW over the day (24 h) and dividing by this period, obtaining the all-sky CRFSW. The cloudy periods, in hours per day, are also estimated from the 10-min averaged data bins; those containing clouds (CRFSW < 0), in each day, are summed up to yield the cloudy period (in min), then converted to hours per day and averaged for all years of the study (2003–10; Table 1), for each season, and for each month. The use of this threshold to detect clouds constitutes a limitation with respect to enhancement events associated with broken cloud conditions (Piedehierro et al. 2014). These episodes exhibit CRFSW > 0, and thus, according to the classification adopted here, they are not considered cloudy, which may introduce additional uncertainty in the lower limits of the CRF statistics. Nevertheless, as the calculations are done using the 10-min averages, the number of these enhancement events is expected to be small and the effect in the daily averages even smaller.
Overall CRFSW results are represented in the probability distribution function (pdf) and cumulative distribution function (cdf) of Fig. 5 and correspond to the 963 days. MFRSR results are represented by the solid line and Eppley pyranometer values by the dashed line. The distribution is clearly skewed to the left, with a long tail, reflecting in a few values with low daily-mean CRFSW, with the minimum MFRSR (Eppley) CRFSW of −139.5 W m−2 (−198.4 W m−2) and the median −18.9 W m−2 (−13.0 W m−2). Yet, the interquartile range that contains 50% of the values is only 42.2 W m−2 (47.6 W m−2), and the 10th and 90th percentiles are −73.1 and −2.0 W m−2 (−84.3 and −0.8 W m−2), respectively, indicating a relatively low spread of the majority of the values in the sample. About 25% of the clouds exert a CRFSW lower than −50 W m−2, and only 3% (7%) present CRFSW values lower than −100 W m−2. Comparing the overall results obtained from MFRSR and Eppley data, only a minor change is observed in the central values; nevertheless, a great difference is obtained in the lower extreme, with a decrease from −139.5 W m−2 (MFRSR) to −198.4 W m−2 (Eppley).

Pdf and cdf of MFRSR (solid line) and Eppley (dashed line) daily averaged CRF at Évora site during the 7-yr period.
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1
The monthly-mean cloud periods, as well as the all-sky CRFSW variability on a daily basis are shown in Fig. 6. Note that only days with at least one cloud occurrence (cloudy days) are represented (963 days in the 7-yr period). A considerable spread of the daily-mean CRFSW and cloudy periods can be noted in March, April, and May. This indicates a large variability in springtime because of the large dispersion that occurs for all months of this season, with interquartile ranges of the MFRSR (Eppley) CRFSW between 58.3 and 73.5 W m−2 (55.6 and 82.2 W m−2) and relative errors of the daily-mean cloudy periods ranging between 43% and 47%, hinting at a greater variability in the sky conditions with respect to the other months. Autumn and winter months present very similar distributions, and the cloudy periods present little variation. The summer season (June, July, and August) presents the lowest interquartile distance (MFRSR CRFSW: 24.4 W m−2; Eppley CRFSW: 17.0 W m−2), and the minima are −129.8 W m−2 (MFRSR CRFSW) and −177.1 W m−2 (Eppley CRFSW), which occur in the month of June. The cloudy periods represented in Fig. 6a show higher variability (higher interquartile ranges) for the spring and autumn months than for winter and summer, when it scarcely varies, suggesting that these are transition months with highly variable conditions in terms of cloud occurrences. In fact, during the spring (autumn) season, the synoptic conditions are determined by the northerly (southerly) migration of the polar front, which determines the passage of Atlantic frontal systems over the area. On the other hand, in these seasons the region is sometimes affected also by northward drifts of the Azores anticyclone, which brings warm dry air into the region and is associated with clear-sky periods. The variability in the cloud occurrences originates from the occurrence of these synoptic patterns, as is typical of the transition seasons.

Box plots showing the monthly variation of the (a) mean cloudy periods and (b) daily-mean MFRSR CRFSW (black) and Eppley CRFSW (dotted gray filled).
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1
The all-sky daily CRFSW is seasonally and annually averaged (considering also clear-sky days), and the results obtained using the Eppley measurements are compared with those reported by Dong et al. (2006) for another midlatitude site. Seasonal and annual CRF averages are also obtained under the conditions of total cloud, as described by Dong et al. (2006). The comparisons are summarized in Table 3 and show, in general, similar CRFSW annual cycles. The all-sky CRFSW presents lower absolute values for this study, and the lowest CRF values (more negative) are obtained for spring in both studies. Dong et al. (2006) estimate a springtime average CRFSW for all-sky conditions of −61.3 W m−2, whereas in this study, the estimated mean value for the CRFSW is −45.5 W m−2. The annual average obtained here of −29.8 W m−2 is also lower (absolute value) than that estimated by Dong et al. (2006), who present a value of −41.5 W m−2. As for the CRF for total cloud conditions (also shown in Table 3), it presents very similar results for both studies, with slightly more negative CRFSW obtained here for winter and summer and slightly less negative values for spring and autumn, with respect to Dong et al. (2006). Overall total CRFSW is very similar in both sites. The dissimilarities of all-sky CRF and similarities of total CRF also hint at the occurrence of more clear-sky days in Évora. Berg et al. (2011) reported a value of −45.5 W m−2 for summertime shallow cumuli, which is thus not directly comparable with the CRFSW obtained here. Mateos et al. (2013) also estimated the CRFSW for another south Iberian site, obtaining average values of −78 W m−2 and −50.0 W m−2, for solar zenith angles of 30° and 60°, respectively.
Seasonal and annual averages of CRF (all-sky and total cloud; W m−2), where S denotes this study and D denotes Dong et al. (2006).

Figure 7 presents the pdf and cdf of the daily-mean MFRSR NCRFSW and Eppley NCRFSW. The median present moderately low values of 7.8% for the MFRSR NCRFSW and 4.2% for the Eppley NCRFSW. The interquartile range of the MFRSR (Eppley) NCRFSW is 15.9% (13%), and the 10th and 90th percentiles are 0.8% and 26.5% (0.0% and 23.1%), respectively, indicating once again a relatively low variability of the majority of the values in the sample. The distance between the 75th percentile and the maximum is quite large (MFRSR NCRFSW: 22.8%; Eppley NCRFSW: 26.8%), significantly higher than the interquartile range (MFRSR NCRFSW: 15.9%; Eppley NCRFSW: 13.0%); yet, according to the pdfs, the high extreme values presented in the sample are only a small number. In fact, barely 3% of the data presents a daily-mean MFRSR NCRFSW above 30% and even less for the Eppley NCRFSW. Eppley broad band decreases the variability of the central values by about 3% relative to MFRSR data; nevertheless, in terms of total variability, there is practically no change, with the maximum in both cases around 40%, as in the findings of Liu et al. (2011).

As in Fig. 5, but for the daily-mean NCRFSW.
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1
The monthly variability of the daily-mean MFRSR NCRFSW and Eppley NCRFSW is presented in Fig. 8. The season with the largest interquartile range of MFRSR (Eppley) NCRFSW is again spring with 19.7% (16.5%), contrasting with summer with only 7.6% (5.5%), which is probably related to the longest cloudy periods in spring (6.9 h day−1) and the shortest in summer (3.6 h day−1) (Fig. 6a). Nevertheless, in summer, the low variability in the central values oppose to the rather large upper extremes, which are as high as about 39.5% (originated in June). Autumn and winter present very similar distributions, skewed to the right, with moderately high upper whiskers (maxima of roughly 36% and 35%, respectively).

As in Fig. 6a, but for the monthly variation of the daily-mean MFRSR NCRFSW (black) and Eppley NCRFSW (dotted gray filled).
Citation: Journal of Climate 27, 20; 10.1175/JCLI-D-13-00696.1


4. Summary
The main purpose of this work was the calculation of the SW cloud radiative forcing at the surface, using surface irradiance measurements taken at a midlatitude site (Évora), with a multifilter rotating shadowband radiometer (MFRSR CRFSW) and an Eppley black and white pyranometer (Eppley CRFSW), for all-sky situations in terms of cloud type and fraction. A new methodology to estimate the clear-sky irradiance is also proposed, based on the correction of the values obtained from radiative transfer calculations, using conversion functions to account for day-to-day atmospheric changes (aerosols and water vapor). It is shown that the clear-sky irradiances obtained in this way present a small uncertainty (~3%), constituting a fast tool to estimate this variable.
Overall results of CRFSW show a large variability of the springtime values with respect to the other seasons and the lowest variability in summer for both absolute and normalized values; it is also in spring that the cloud occurrence presents the highest values and variability. Minimum values of −139.5 and −198.4 W m−2 for MFRSR CRFSW and Eppley CRFSW, respectively, were obtained considering the complete dataset (Table 1). Yet for this dataset, it was found that the interquartile range (containing 50% of the values) is only 42.2 and 47.6 W m−2 for MFRSR CRFSW and Eppley CRFSW, respectively.
The NCRFSW presents an amplitude range of approximately 40%, considering the complete dataset (Table 1). This implies that, in this study, clouds may attenuate (by absorption or scattering) up to about 40% of the solar radiation on a daily basis, or in other words, 40% less solar radiation reaches the surface because of the cloud effects. Considering the NCRFSW results, the spring is the season with the largest variability, contrasted with summer, which presents the lowest variability, and probably this is related to the cloudy periods occurred in spring (6.9 h day−1) and in summer (3.6 h day−1). The same relation, between cloudy periods and CRFSW, was verified showing that the variability of the cloudy periods is proportional to the variability of the cloud radiative forcing with its maximum value in springtime.
The use of two different instruments (MFRSR and Eppley) that cover different fractions of the solar radiation spectrum reveals some differences, with respect to the distributions of the daily-mean CRFSW and NCRFSW. Curiously, there is only a minor change in the central values of the CRFSW distributions, both from MFRSR and Eppley instruments; nevertheless, there is a strong decrease of the minimum value for the case where most of the solar radiation is included (Eppley). On the other hand, the total variability of the NCRFSW remains practically unchanged, both for MFRSR and Eppley instruments, although the variability of central values decreases by about 3% in the Eppley case. A mathematical equation is derived, expressing the relationship between the CRFSW obtained in the two spectral bands, which may constitute a useful tool under any cloud conditions for different locations where only one of the instruments is present, or may even be applicable to modeled data.
This work is financed through FCT grant SFRH/BD/88669/2012 and through FEDER [Programa Operacional Factores de Competitividade (COMPETE)] and National funding through Fundação para a Ciência e a Tecnologia (FCT) in the framework of projects FCOMP-01-0124-FEDER-009303 (PTDC/CTE-ATM/102142/2008), FCOMP-01-0124-FEDER-014024 (PTDC/AAC-CLI/114031/2009) and provided by the Évora Geophysics Centre, Portugal, under the contract with FCT, PEst-OE/CTE/UI0078/2014. The authors also acknowledge the project and support of the European Community—Research Infrastructure Action under the FP7 “Capacities” specific program for Integrating Activities, ACTRIS Grant Agreement 262254. Thanks are due to Sérgio Pereira and Samuel Bárias for maintaining radiometric instrumentation used in this work.
The authors thank the anonymous reviewers for their valuable comments and suggestions to improve the paper.
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