1. Introduction
A key parameter in predicting future climate change and in explaining past climate changes is climate sensitivity. The equilibrium climate sensitivity, for example, is defined as the global-mean surface warming in response to a doubling of CO2 after the system has reached a new steady state (Knutti and Hegerl 2008). Recent, authoritative estimates suggest that the equilibrium climate sensitivity is likely to be in the range 1.5°–4.5°C (Bindoff et al. 2013; Knutti and Hegerl 2008). This uncertainty range has remained virtually unchanged despite decades of research (Mitchell et al. 1990; Knutti and Hegerl 2008). Estimates of climate sensitivity based on instrumental records are limited by significant uncertainties in observations, especially in ocean heat uptake and the magnitude of aerosol radiative forcing (Knutti et al. 2002; Hansen et al. 2005).
A significant challenge in inferring climate sensitivity from observations is to disentangle greenhouse gas warming from internal variability and from the response to other forcings, particularly anthropogenic aerosols. For instance, some aerosols directly cool Earth by enhancing scattering of solar radiation to space, whereas others, such as black carbon, absorb solar radiation and thereby warm the atmosphere, altering the general circulation. Aerosols also can serve as cloud condensation nuclei and thereby alter cloud properties. In particular, aerosols increase the number of small liquid cloud droplets, causing an increase in total droplet surface area and an increase in the albedo of liquid clouds, leading to a cooling effect (Boucher et al. 2013). Most studies find that, overall, anthropogenic aerosols have cooled the planet (Boucher et al. 2013), implying that they have masked some of the global warming that would have occurred in their absence.
Stott et al. (2006) applied optimal fingerprinting techniques to estimate the cooling effects of aerosols and the warming effects of anthropogenic greenhouse gases. Both spatial and temporal aspects of the observed temperature change were necessary to constrain the relative roles of greenhouse gas warming and sulfate cooling over the twentieth century. In particular, the analysis exploited distinctive differences between the different forcings, especially the differential warming rates between the hemispheres, between land and ocean, and between mid- and low latitudes.
Recent studies have revealed another difference between greenhouse gas warming and sulfate cooling—namely, their hydrological sensitivity (Hansen et al. 1997; Allen and Ingram 2002; Lambert and Faull 2007; Andrews et al. 2009; Bala et al. 2010; O’Gorman et al. 2012). Hydrological sensitivity is defined as the change in global-mean precipitation per degree of global-mean temperature. Climate models suggest that the hydrological sensitivity for greenhouse gas forcing is less than that of sulfate aerosols. This difference has been explained in terms of differences in the response on fast time scales (Bala et al. 2010; Andrews et al. 2009, 2010). Specifically, numerical experiments reveal that precipitation initially decreases in response to an instantaneous change in CO2. The initial decrease can be explained by the fact that an increase in greenhouse gas forcing reduces radiative cooling in the troposphere, and since on monthly time scales energy is balanced above the atmospheric boundary layer, a decrease in radiative cooling requires a reduction in condensational heating from convection (Yang et al. 2003; Andrews et al. 2009; Takahashi 2009). After this initial “fast” adjustment, precipitation then increases with increasing sea surface temperatures on “slow” multiyear time scales. Thus, the fast and slow time-scale responses are in opposite directions for warming due to greenhouse gases. In contrast, an increase in sulfate aerosol forcing enhances solar reflectivity, which only modestly impacts the atmospheric energy balance on fast time scales, leaving the slow response to dominate the total hydrological sensitivity. Interestingly, the hydrological sensitivity on slow time scales tends to be independent of forcing (Andrews et al. 2010). Thus, the total hydrological sensitivity, because of the combined effect of fast and slow responses, is less for greenhouse gas warming than for sulfate cooling. Because different forcings share a common slow response, their hydrological sensitivities tend to be similar and hence difficult to distinguish.
The purpose of this paper is to demonstrate that anthropogenic aerosol cooling can be separated from the response to all other forcings using just their hydrological sensitivities. This result is demonstrated using temperature and precipitation data generated by climate models, rather than from observations, because global precipitation observations are too uncertain (as will be shown). We further show that this result is reproducible across different climate models and demonstrate that aerosol cooling can be estimated without using any spatial or temporal gradient information in the response, provided temperature data are augmented by precipitation data. In addition, this paper clarifies that previous regression methods for estimating hydrological sensitivities do not account for temperature–precipitation (T–P) relations that occur through internal variability and are not optimized to detect specific forcings. This paper proposes an alternative method for estimating hydrological sensitivity that overcomes these limitations. Finally, this paper presents a stark contrast between hydrological sensitivities between models and observations but also presents strong arguments that these discrepancies are very likely due to observational errors. The data used in this paper are discussed in section 2. Our methodology is explained in section 3, with mathematical details relegated to an appendix. The results of our analysis on model simulations and observations are discussed in section 4. We conclude with a summary and discussion of our results.
2. Data
Four types of simulations are used in our analysis: historical, AA, noAA, and control. Historical runs refer to simulations that include both natural and anthropogenic forcings. The AA runs refer to simulations that include only anthropogenic aerosols. The noAA runs refer to simulations that include all forcings except anthropogenic aerosol forcing. Control runs refer to simulations in which natural and anthropogenic forcing does not vary from year to year. The historical, AA, and noAA runs were analyzed over the period 1900–2004. We only consider models if they have at least 500 years of control simulations. We use only the last 500 years of each control run.
Only two models from the CMIP5 archive have all four runs—namely, CSIRO Mk3.6.0 and IPSL-CM5A-LR, denoted CSIRO and IPSL, respectively. We focus on results from these two models in the main text. We also consider four additional models that have AA runs (but not noAA runs) and at least 500 years of control simulations. These models are GFDL-ESM2M, NorESM1-M, GFDL CM3, and CCSM4. Results from these models are discussed in the appendix and confirm results from CSIRO and IPSL. Table 1 also indicates the models that include the first indirect effect of aerosols [as documented in Wilcox et al. (2013)], which is the tendency for aerosols to increase droplet concentration and decrease droplet size, making clouds more reflective.
Summary of CMIP5 model attributes used in this study. The AA and noAA response parameters for the CMIP5 models are based on global-mean temperature and precipitation. Sensitivities are expressed as ensemble mean plus or minus interensemble standard deviation (zero standard deviation implies only one member was available). Models that include the first indirect effect of aerosols are indicated by “Y” in the “first indirect” column.
Observational estimates of global precipitation were obtained from the Global Precipitation Climatology Project (GPCP), version 2 (http://www.esrl.noaa.gov/psd/data/gridded/data.gpcp.html) and from the Climate Prediction Center (CPC) Merged Analysis of Precipitation (CMAP; Xie and Arkin 1997; http://www.esrl.noaa.gov/psd/data/gridded/data.cmap.html).
Observational estimates of global temperature were obtained from the Hadley Centre/Climatic Research Unit, version 4 (HadCRUT4; downloaded from http://www.cru.uea.ac.uk/cru/data/temperature/). Annual means were computed when at least 10 months per calendar year were available. A grid point is included only when annual means are available for every year in the period 1979–2014. The resulting map of available grid points covers 75% of the surface area of the globe and was used to analyze both observations and model output of temperature.
3. Methodology
a. Estimating hydrological sensitivity









We estimate hydrological sensitivity (i.e., γ) and response time series
One may question whether hydrological sensitivity can be treated as a constant. Indeed, noAA represents a mix of forcings (e.g., greenhouse gases, ozone, and volcanoes), so assuming a constant sensitivity effectively assumes that the temperature–precipitation response to these different forcings follows a constant ratio. If the constant-ratio assumption is not appropriate, then the regression model should be expanded to include additional sensitivities
b. Estimating the response time series




A standard approach to estimating the response to external forcing using observations is to introduce scaling factors for each forcing and then choose the scaling factors to best fit observations using generalized least squares methods. This approach, called optimal fingerprinting, uses the full spatiotemporal structure of the response to inform the estimation. Instead, we directly estimate the time series
4. Results
The estimated sensitivities for AA and noAA forcing are shown in Fig. 1 (and listed in Table 1). These estimates generally are larger than those reported previously (Andrews et al. 2010), owing partly to differences in estimation method [e.g., (3) implies our estimate will be larger than the least squares estimate; see also the appendix, especially Fig. A1]. As anticipated in the introduction, the sensitivity to noAA forcing is consistently less than that of AA in the same model. Moreover, for each model, the sensitivity of AA forcing is clearly separated from that of noAA forcing.
Hydrological sensitivity associated with anthropogenic aerosol forcing (AA) and with all forcings except anthropogenic aerosols (noAA), estimated by ML methods from CMIP5 simulations. Each estimate is derived from a single ensemble member of a single-forcing simulation for 1900–2004 and 500 years of a control run from each model. Different points for the same model indicate estimates from different ensemble members.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
The estimated sensitivities are distinct in each model but nevertheless may be so close as to cause multicollinearity problems. As discussed in the appendix, the angle between the AA and noAA response vectors emerges naturally as a measure of collinearity from generalized least squares. This measure is effectively the angle between the vectors in “whitened space” and can be interpreted as a kind of “pattern correlation” between the two response vectors. These pattern correlations, as well as their corresponding condition numbers, are listed in Table 1. The largest condition number is 5.7, which is less than 10 and hence implies that multicollinearity is not a serious problem.
We test our methodology by applying it to historical simulations containing both anthropogenic and natural forcings. The response time series estimated from the historical simulations are shown in Fig. 2 as green and red curves, while those derived from the AA and noAA runs are shown in blue and black curves. The latter time series were estimated for each year separately, with no temporal smoothing, which can be done accurately because only one type of forcing exists (i.e., no separation of responses is required). Different curves of the same color show results for different ensemble members. The response time series estimated from the historical runs are in excellent agreement with each other and with response time series estimated from the AA and noAA runs. This result demonstrates the remarkable fact that the hydrological sensitivity parameter is sufficient to recover the correct (multidecadal) time history of the response to both AA and noAA forcings simultaneously. Moreover, time series estimated from different ensemble members of the same forcing are close to each other relative to the secular changes, indicating that the estimates are not sensitive to different realizations of internal variability.
Changes in global-average temperature due to AA and noAA, estimated from historical simulations containing both anthropogenic and natural forcings (red and green curves) and from individual-forcing runs containing only those forcings (blue and black curves) in (top) CSIRO and (bottom) IPSL. The temperature changes are estimated using the technique described in the appendix, which uses the joint covariability between temperature and precipitation. Estimates from AA and noAA simulations are obtained for each year separately, while those from the historical simulations are obtained from a polynomial fit. Different curves of the same color show estimates based on different ensemble members. The black and gray curves before 1900 show the projection of the AA and noAA response vectors in the preindustrial control run, respectively.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
Performing the same fingerprinting procedure on historical simulations that lack a corresponding noAA simulation gives similar results (see appendix). Also, when the response time series for AA and noAA are regressed out from those respective runs, the residual contains no statistically significant detectable component in most cases, indicating that the two hydrological sensitivities are sufficient to capture practically the whole climate change signal (not shown). We also considered the “imperfect model” case in which response vectors from one model are used to detect AA and noAA responses in another model. For these two models, temperature changes derived from the perfect and imperfect cases are close to each other (not shown). This robustness is not surprising because the only information used in fingerprinting are the hydrological sensitivities, which are nearly the same for the two models (see Fig. 1). (Technically, fingerprinting also depends on the covariances of internal variability, but swapping covariances from different models produces nearly identical results.) Thus, differences between inferred time series can be attributed solely to differences in hydrological sensitivities. Of course, greater disagreement can be found by choosing models with greater differences in hydrological sensitivities. Also, this approach does not tell the whole story because models differ not only in their response to forcing but also in the nature and magnitude of the forcing itself. Nevertheless, these issues do not affect our main conclusion, which is that hydrological sensitivities for AA and noAA forcings are sufficiently distinct in each model that they can be used to infer time series for anthropogenic cooling and greenhouse gas warming in that model.
Having established that the methodology works in climate models, we now consider observations. Unfortunately, global precipitation data are limited to the satellite era (i.e., since the 1970s). Repeating the above analysis on climate models but for the shorter period 1979–2004 (not shown) yields time series consistent with those shown above but with larger uncertainties because of the smaller sample size. It should be recognized that global anthropogenic aerosol forcing varies weakly over the period 1979–2004 (Myhre et al. 2013, their Fig. 8.18), so the response to aerosols over this period is likely to have small trend (as can be seen in Fig. 2).
To visualize the situation, we construct a scatterplot of all the data in temperature–precipitation space, as in Fig. 3. The AA and noAA simulations (blue and red circles, respectively) are seen to be displaced from each other. However, this displacement is not relevant for distinguishing the two forcings because the time series will be centered prior to analysis (to remove model bias). Instead, the relevant feature is the slope of the variability, which corresponds to hydrological sensitivity. For reference, the hydrological sensitivities of the AA and noAA simulations determined by maximum likelihood are indicated in the lower-right corner of each panel. These values differ slightly from those in Table 1 because the sensitivities were computed from model data whose spatial grid was masked in such a way to mimic missing data in the temperature observations.
Scatterplot of annual-mean, global-mean temperature and precipitation in simulations from (top) CSIRO and (bottom) IPSL and observations (green symbols). Simulations are shown with AA (blue), with noAA (red), with both natural and anthropogenic forcings (gold symbols), and with no natural and anthropogenic forcing (gray symbols). Also shown are observations based on GPCP (green filled circles) and CMAP (green crosses). Temperature in the historical run and observations are centered to have zero mean over the common period 1979–2004, while other simulations are shown relative to the mean of the historical run over this period. Precipitation in the historical run and observations are normalized by their respective means over the period 1979–2004, while other simulations are normalized by the mean of the historical run over the same period. The solid curves show the projection of a low-pass time series of the respective runs. The two lines in the lower-right corner indicate the hydrological sensitivities estimated from the AA and noAA simulations.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
The historical and control runs also are shown in Fig. 3. The historical runs (gold circles) trace a path that cannot be explained by internal variability (gray circles). Geometrically, optimal fingerprinting represents each year of the historical run as a linear combination of the response vectors shown in the lower-right corner. The observations are shown as green dots and green crosses (after aligning their mean with that of the historical run over the same period). The figure reveals that observations vary over a region in T–P space outside that of any of the climate simulations. To highlight differences between models and observations further, we show in Fig. 4 (see also Fig. A3) the sensitivity estimated from observations against a histogram of hydrological sensitivities computed for every 36-yr period in historical simulations. The sensitivity estimated from observations are very unlikely relative to the sensitivities found in the historical simulations.
Histogram of the hydrological sensitivity computed for every 36-yr period in historical simulations over the period 1900–2004 (gray bars) in four CMIP5 models. The sensitivity computed from GPCP in the period 1979–2014 is indicated by the red dot; the error bar indicates one standard error. All sensitivities were computed from OLS.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
Note that the two observational datasets differ even between themselves. These differences are due entirely to differences in precipitation datasets [e.g., global-mean, annual-mean temperature shows little sensitivity to estimation method; see Fig. 2.14 in Hartmann et al. (2013)]. Indeed, the correlation between the annual-mean, global-mean precipitation time series for CMAP and GPCP over 1979–2014 is 0.24, which is not statistically significant at the 5% level. Previous attempts to estimate hydrological sensitivity from observations have yielded negative values (Arkin et al. 2010), values around 2% K−1 (Adler et al. 2008), and values around 7% K−1 (Wentz et al. 2007; Liepert and Previdi 2009), clearly indicating sensitivity to data source, estimation method, and time period. Yin et al. (2004) document additional differences between GPCP and CMAP precipitation datasets and show that certain trends are clear artifacts of changes in satellite data input and sampling of atoll data.
5. Summary and discussion
This paper shows that, in climate models, differences in hydrological sensitivity can be used to separate the cooling effects of aerosols from the effects of other forcings. The proposed methodology for doing this uses both temperature and precipitation data and requires estimates of the hydrological sensitivity associated with different forcings. We introduce a new estimate for hydrological sensitivity that accounts for temperature–precipitation covariability due to internal variability and converges to the “true sensitivity” [the sensitivity in the model in (2)] in the limit of large sample sizes, in contrast to the linear regression estimate. This method is formally equivalent to finding the response vector that maximizes detectability (Jia and DelSole 2012). Finally, the fingerprinting method is generalized to infer the multidecadal evolution due to different forcings. Applying this methodology to historical simulations containing both anthropogenic and natural forcings yields response time series that closely match those obtained from individual forcing runs. This result demonstrates that greenhouse gas warming and aerosol cooling can be estimated without using any spatial or temporal gradient information in the response, provided temperature data are augmented by precipitation data. This result also highlights the fact that hydrological sensitivity is important not only for predicting future climates but also has implications for attributing past climate changes to man.
This study also reveals striking inconsistencies between models and observations. Specifically, over the late twentieth century, climate models predict a robust positive relation between global-mean, annual-mean temperature and precipitation that differs significantly from that of observations. Whether this discrepancy can be attributed to observational error, which is substantial as different estimates of global-mean precipitation are not even significantly correlated with each other, or to model error is not clear. Because global-mean temperature and precipitation are fundamental indices of climate change, this clear discrepancy between models and observations seems serious. Previous attempts to estimate hydrological sensitivity from global observational datasets yield results that are sensitive to data source, estimation method, and time period. Moreover, precipitation estimates can differ by as much as 20% in the tropics and as much as 50% in midlatitudes (Adler et al. 2012). Such differences are not surprising given well-known sensitivity of precipitation estimates to changes in satellite and gauge data input. Precipitation estimates over land are considered to be more accurate owing to the availability of rain gauge measurements for calibration purposes. Using land-average precipitation in our model-only analysis does not yield accurate estimates of aerosol-forced signals (not shown). A more comprehensive analysis that includes spatial variations in land precipitation will be discussed in future work.
Acknowledgments
This work was sponsored by National Science Foundation Grant ATM1338427 (TD and XY), National Aeronautics and Space Administration Grant NNX14AM19G (TD and XY), National Oceanic and Atmospheric Administration Grant NA14OAR4310160 (TD and XY), Department of Energy Grant ER65095 (TD and XY), and Office of Naval Research Grant N00014-16-1-2073 (MKT). We acknowledge the World Climate Research Programme’s Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups for producing and making available their model output. For CMIP the U.S. Department of Energy’s Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals.
APPENDIX
Calculation Details and Additional Information
a. Maximum likelihood estimates of the signal parameters





The model in (A1) is known as an errors-in-variables model (Fuller 1980). There exist a variety of methods for estimating parameters of such models. Here, we estimate












In practice, the covariance matrix
Comparison of the OLS and ML estimates of hydrological sensitivity for AA and noAA forcing computed from simulations from the CMIP5 archive. The solid line shows y = x.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
b. Model for combined forcings








c. Analysis of models without noAA runs
In the CMIP5 archive, at least four models have AA runs without a corresponding noAA run. In such cases, the noAA signal can be estimated by subtracting one ensemble member of the AA run from one ensemble member of the historical run, and then determining the maximum likelihood estimates of the signal parameters of the noAA signal from (A7) and (A11) (where
Results of applying optimal fingerprinting to historical simulations of four different models, but with the noAA parameters determined from the residual between historical and AA runs. The noAA response time series is shown as the blue curve, and the AA response time series (determined from the AA run) is shown as the black curve. The green and red curves show time series of AA and noAA response time series estimated from each ensemble member of the historical simulations. Different curves of the same color show results from different ensemble members. The black and gray curves before the year 1900 show estimates of the amplitude of the AA and noAA signal vector, respectively, in the control run. Each time series is obtained as anomalies with respect to the mean of the full period but is offset by a constant for display purposes.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
For completeness, we show in Fig. A3 the sensitivity estimated from observations against a histogram of hydrological sensitivities computed for every 36-yr period in historical simulations.
Histogram of the hydrological sensitivity computed for every 36-yr period in historical simulations over the period 1900–2004 (gray bars) in four CMIP5 models. The sensitivity computed from GPCP in the period 1979–2014 is indicated by the red dot; the error bar indicates one standard error. All sensitivities were computed from OLS.
Citation: Journal of Climate 29, 17; 10.1175/JCLI-D-15-0364.1
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